{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T13:55:48Z","timestamp":1785851748690,"version":"3.56.0"},"reference-count":75,"publisher":"American Chemical Society (ACS)","issue":"30","license":[{"start":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T00:00:00Z","timestamp":1784592000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by-nc-nd\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001691","name":"Japan Society for the Promotion of Science","doi-asserted-by":"publisher","award":["25K01580"],"award-info":[{"award-number":["25K01580"]}],"id":[{"id":"10.13039\/501100001691","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/na","name":"Research Association of Automotive Internal Combustion Engines","doi-asserted-by":"publisher","award":["NA"],"award-info":[{"award-number":["NA"]}],"id":[{"id":"10.13039\/na","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,4]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>NOx and hydrocarbons coexist in the exhaust of diesel engines under conditions relevant to the passive NOx adsorber (PNA). However, the influence of hydrocarbons on NOx adsorption and desorption on Pd-zeolites as a PNA is not clearly understood and appears to depend strongly on the properties of the Pd-zeolites. In this study, the effect of propylene (C3H6), a representative light hydrocarbon, on the NOx adsorption\u2013desorption behavior of Pd-loaded zeolites with different framework structures was systematically investigated to elucidate the role of hydrocarbons. NOx adsorption and desorption test results revealed that the presence of C3H6 increased the total amount of adsorbed NOx while lowering the desorption temperature. In addition, Pd\/MFI and Pd\/BEA exhibited a new low-temperature NOx desorption peak below 300 \u00b0C, contrasting with the previously reported high-temperature shift induced by C3H6. Various NOx-TPD and FT-IR analyses demonstrated that the coadsorption of NO and C3H6 generated organic nitrite (R\u2013ONO) and nitro (R\u2013NO2) species, which decompose below 300 \u00b0C to release NOx. These results provide new mechanistic insights into the C3H6-induced low-temperature NOx desorption on Pd-loaded zeolites, offering a basis for optimizing PNA materials and operating strategies suitable for low exhaust temperatures typical of diesel engines.<\/jats:p>","DOI":"10.1021\/acs.est.6c02256","type":"journal-article","created":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T13:04:13Z","timestamp":1784639053000},"page":"20901-20912","source":"Crossref","is-referenced-by-count":0,"title":["NO\n                    <i>x<\/i>\n                    -Propylene Co-Adsorption\nEnables Low-Temperature NO\n                    <i>x<\/i>\n                    Desorption\nvia Organic Nitrite\/Nitro Species on Pd-Loaded Zeolites"],"prefix":"10.1021","volume":"60","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-6943-7689","authenticated-orcid":true,"given":"Takeshi","family":"Ohtsu","sequence":"first","affiliation":[{"name":"Nagoya University , , Furo-cho, Chikusa-ku , ,","place":["Nagoya, Japan, 464-8603"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hiroki","family":"Miyazaki","sequence":"additional","affiliation":[{"name":"Nagoya University , , Furo-cho, Chikusa-ku , ,","place":["Nagoya, Japan, 464-8603"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nao","family":"Tsunoji","sequence":"additional","affiliation":[{"name":"Tottori University , , 4-101 Koyama-cho Minami , ,","place":["Tottori, Japan, 680-8552"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Akira","family":"Oda","sequence":"additional","affiliation":[{"name":"Hokkaido University , , Kita21, Nishi10, Kita-ku , , ,","place":["Sapporo, Hokkaido, Japan, 001-0021"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6946-7678","authenticated-orcid":true,"given":"Atsushi","family":"Satsuma","sequence":"additional","affiliation":[{"name":"Nagoya University , , Furo-cho, Chikusa-ku , ,","place":["Nagoya, Japan, 464-8603"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,21]]},"reference":[{"issue":"9","key":"2026080409311056000_cit1","doi-asserted-by":"publisher","first-page":"1706","DOI":"10.1007\/s10562-016-1794-6","article-title":"Low Temperature NO Storage of Zeolite\nSupported Pd for Low Temperature Diesel Engine Emission Control","volume":"146","author":"Chen","year":"2016","journal-title":"Catal. Lett."},{"key":"2026080409311056000_cit2","doi-asserted-by":"publisher","first-page":"1","DOI":"10.1016\/j.apcata.2018.10.036","article-title":"Passive NOx Adsorber: An Overview of Catalyst Performance\nand Reaction Chemistry","volume":"570","author":"Gu","year":"2019","journal-title":"Appl. Catal., A"},{"key":"2026080409311056000_cit3","doi-asserted-by":"publisher","first-page":"397","DOI":"10.1016\/j.apcatb.2018.10.069","article-title":"Vehicle\nEmissions Trapping Materials:\nSuccesses, Challenges, and the Path Forward","volume":"243","author":"Lee","year":"2019","journal-title":"Appl. Catal., B"},{"issue":"3","key":"2026080409311056000_cit4","doi-asserted-by":"publisher","first-page":"1169","DOI":"10.1016\/j.cclet.2021.07.066","article-title":"Recent Progress of Pd\/Zeolite as\nPassive NOx Adsorber: Adsorption Chemistry, Structure-Performance\nRelationships, Challenges and Prospects","volume":"33","author":"Bian","year":"2022","journal-title":"Chin.\nChem. Lett."},{"issue":"3","key":"2026080409311056000_cit5","doi-asserted-by":"publisher","first-page":"1151","DOI":"10.1039\/D4CS00140K","article-title":"Toward Synergetic\nReduction of Pollutant and Greenhouse Gas Emissions from Vehicles:\nA Catalysis Perspective","volume":"54","author":"Zhang","year":"2025","journal-title":"Chem. Soc. Rev."},{"issue":"18\u201319","key":"2026080409311056000_cit6","doi-asserted-by":"publisher","first-page":"2007","DOI":"10.1007\/s11244-018-1017-z","article-title":"The Effect\nof Si\/Al Ratio for Pd\/BEA and Pd\/SSZ-13 Used as Passive NOx Adsorbers","volume":"61","author":"Mihai","year":"2018","journal-title":"Top. Catal."},{"key":"2026080409311056000_cit7","doi-asserted-by":"publisher","first-page":"283","DOI":"10.1016\/j.apcatb.2015.01.025","article-title":"Al2O3-Based Passive NOx Adsorbers\nfor Low Temperature\nApplications","volume":"170\u2013171","author":"Ji","year":"2015","journal-title":"Appl. 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Solid State Chem."},{"issue":"18\u201319","key":"2026080409311056000_cit17","doi-asserted-by":"publisher","first-page":"2021","DOI":"10.1007\/s11244-018-1045-8","article-title":"Low Temperature NOx\nAdsorption Study on Pd-Promoted Zeolites","volume":"61","author":"Porta","year":"2018","journal-title":"Top.\nCatal."},{"issue":"51","key":"2026080409311056000_cit18","doi-asserted-by":"publisher","first-page":"16672","DOI":"10.1002\/anie.201809343","article-title":"Achieving\nAtomic Dispersion of Highly Loaded Transition Metals in Small-Pore\nZeolite SSZ-13: High-Capacity and High-Efficiency Low-Temperature\nCO and Passive NO x Adsorbers","volume":"57","author":"Khivantsev","year":"2018","journal-title":"Angew.\nChem. Int. 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Technol."},{"issue":"18","key":"2026080409311056000_cit40","doi-asserted-by":"publisher","first-page":"6455","DOI":"10.1021\/acs.iecr.0c05186","article-title":"Integration of an\nOxidation Catalyst with Pd\/Zeolite-Based\nPassive NOx Adsorbers: Impacts on Degradation Resistance and Desorption\nCharacteristics","volume":"60","author":"Gu","year":"2021","journal-title":"Ind. Eng. Chem. Res."},{"key":"2026080409311056000_cit41","doi-asserted-by":"publisher","first-page":"158299","DOI":"10.1016\/j.cej.2024.158299","article-title":"An Oxidation-Adsorption\nSite Separation Strategy for Stabilizing Pd-Pt\/SSZ-13 PNA Materials\nunder High CO Pressure","volume":"503","author":"Wang","year":"2025","journal-title":"Chem. Eng. 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