{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,18]],"date-time":"2026-08-18T16:54:50Z","timestamp":1787072090397,"version":"build-2736575974"},"reference-count":51,"publisher":"American Chemical Society (ACS)","issue":"32","license":[{"start":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T00:00:00Z","timestamp":1785801600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T00:00:00Z","timestamp":1785801600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T00:00:00Z","timestamp":1785801600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2024YFF0725900"],"award-info":[{"award-number":["2024YFF0725900"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,18]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Per- and polyfluoroalkyl substances (PFAS) represent a global environmental threat due to their chemical stability and bioaccumulation. However, the efficacy of current adsorbents in contaminated source remediation is constrained by limited selectivity and the lack of sustainable regenerability. Here we report AR-1, a pore-size-tuned cross-linked polymethacrylate adsorbent for perfluorooctanoic acid (PFOA) capture and water-mediated regeneration. By engineering high-density ester-functionalized amphiphilic microenvironments within nanoconfined channels, AR-1 relies on engineered mesoporous confinement, hydrogen bonding, local polar contacts, and hydrophobic\/fluorocarbon-chain partitioning interactions. These interactions enable selective molecular recognition of PFOA and promote its confined self-assembly into stable intrapore aggregates. Consequently, AR-1 yields a PFOA adsorption capacity of 531.8 mg g\u20131 and a removal efficiency of &amp;gt;99% in industrial wastewater. It maintains high selectivity for PFOA even in the presence of a 10,000-fold excess of competing background ions. Furthermore, pH-responsive modulation of interfacial binding affinity allows for nearly 100% regeneration using water alone. This strategy offers a sustainable, high-performance solution to the critical challenge of PFAS contamination.<\/jats:p>","DOI":"10.1021\/acs.est.6c04782","type":"journal-article","created":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T04:02:12Z","timestamp":1785902532000},"page":"22423-22436","source":"Crossref","is-referenced-by-count":0,"title":["Molecularly\nDesigned\nPolymer Adsorbents for Selective\nRecognition of Perfluorooctanoic Acid and Hydroresponsive Sustainable\nRegeneration"],"prefix":"10.1021","volume":"60","author":[{"given":"Yifan","family":"Shen","sequence":"first","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]},{"name":"Nanjing University , , ,","place":["Yancheng, China, 224000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guizhou","family":"Xu","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2200-1341","authenticated-orcid":true,"given":"Guandao","family":"Gao","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haolin","family":"Liu","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qiancheng","family":"Xia","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tao","family":"Shan","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9158-6216","authenticated-orcid":true,"given":"Wentao","family":"Li","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuming","family":"Yang","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xinyi","family":"Wang","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3333-0458","authenticated-orcid":true,"given":"Peng","family":"Shi","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-3003-2114","authenticated-orcid":true,"given":"Aimin","family":"Li","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7655-9244","authenticated-orcid":true,"given":"Zunyao","family":"Wang","sequence":"additional","affiliation":[{"name":"Nanjing University , , ,","place":["Nanjing, China, 210023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2028-1295","authenticated-orcid":true,"given":"Baoshan","family":"Xing","sequence":"additional","affiliation":[{"name":"University of Massachusetts Amherst , , , ,","place":["Amherst, Massachusetts, United States, 01003"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,4]]},"reference":[{"issue":"2","key":"2026081810421030500_cit1","doi-asserted-by":"publisher","first-page":"119","DOI":"10.1038\/s41578-023-00623-4","article-title":"Fluorination in advanced\nbattery design","volume":"9","author":"Wang","year":"2024","journal-title":"Nat. Rev. Mater."},{"issue":"9","key":"2026081810421030500_cit2","doi-asserted-by":"publisher","first-page":"6225","DOI":"10.1021\/jacs.3c14213","article-title":"Fluorinated Nonporous\nAdaptive Cages for the Efficient Removal of\nPerfluorooctanoic Acid from Aqueous Source Phases","volume":"146","author":"He","year":"2024","journal-title":"J. Am. Chem. Soc."},{"issue":"10","key":"2026081810421030500_cit3","doi-asserted-by":"publisher","first-page":"1198","DOI":"10.1038\/s44221-025-00489-6","article-title":"Electro-activated dual-affinity membrane for efficiently removing\nper- and polyfluoroalkyl substances from drinking water","volume":"3","author":"Liu","year":"2025","journal-title":"Nat. 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Technol."},{"issue":"1","key":"2026081810421030500_cit7","doi-asserted-by":"publisher","first-page":"1972","DOI":"10.1038\/s41467-025-57272-0","article-title":"Broad-spectrum\ncapture of hundreds of per- and polyfluoroalkyl substances from fluorochemical\nwastewater","volume":"16","author":"Liang","year":"2025","journal-title":"Nat. Commun."},{"issue":"4","key":"2026081810421030500_cit8","doi-asserted-by":"publisher","first-page":"340","DOI":"10.1038\/s41561-024-01402-8","article-title":"Underestimated\nburden of per- and\npolyfluoroalkyl substances in global surface waters and groundwaters","volume":"17","author":"Grunfeld","year":"2024","journal-title":"Nat. Geosci."},{"issue":"5","key":"2026081810421030500_cit9","doi-asserted-by":"publisher","first-page":"451","DOI":"10.1038\/s44221-023-00077-6","article-title":"Substantial defluorination of polychlorofluorocarboxylic\nacids triggered\nby anaerobic microbial hydrolytic dechlorination","volume":"1","author":"Jin","year":"2023","journal-title":"Nat. Water"},{"key":"2026081810421030500_cit10","first-page":"59623","volume-title":"National primary\ndrinking water regulations; Announcement of the results of EPA\u2019s\nfourth review of existing drinking water standards The Federal Register","author":"U.S. Environmental Protection Agency.","year":"2024"},{"issue":"1","key":"2026081810421030500_cit11","doi-asserted-by":"publisher","first-page":"2132","DOI":"10.1038\/s41467-022-29816-1","article-title":"Installation of synergistic\nbinding sites onto porous organic polymers\nfor efficient removal of perfluorooctanoic acid","volume":"13","author":"Liu","year":"2022","journal-title":"Nat. Commun."},{"issue":"1","key":"2026081810421030500_cit12","doi-asserted-by":"publisher","first-page":"90","DOI":"10.1080\/10643389.2020.1816125","article-title":"Recent progress in\nadsorptive removal of per- and poly-fluoroalkyl\nsubstances (PFAS) from water\/wastewater","volume":"52","author":"Vu","year":"2022","journal-title":"Crit.\nRev. Environ. Sci. Technol."},{"key":"2026081810421030500_cit13","doi-asserted-by":"publisher","first-page":"695","DOI":"10.1016\/j.jhazmat.2018.11.067","article-title":"Novel synergy of\nSi-rich minerals and reactive MgO for stabilisation\/solidification\nof contaminated sediment","volume":"365","author":"Wang","year":"2019","journal-title":"J. Hazard. 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A.; Nakatsuji, H.; et al., Gaussian 16, Revision C. 01; Gaussian, Inc.: Wallingford CT, 2023."},{"issue":"11","key":"2026081810421030500_cit39","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.ade8839","article-title":"Physics-based\ngenerative model of curvature sensing peptides; distinguishing sensors\nfrom binders","volume":"9","author":"van Hilten","year":"2023","journal-title":"Sci. Adv."},{"key":"2026081810421030500_cit40","doi-asserted-by":"publisher","first-page":"1522","DOI":"10.1016\/j.cej.2015.08.010","article-title":"A comparative\nstudy on the adsorption of 8-amino-1-naphthol-3,6-disulfonic acid\nby a macroporous amination resin","volume":"283","author":"Zhang","year":"2016","journal-title":"Chem. Eng.\nJ."},{"issue":"8","key":"2026081810421030500_cit41","doi-asserted-by":"publisher","first-page":"551","DOI":"10.1007\/s00339-019-2847-7","article-title":"A novel SiO2\u2013GO\/acrylic resin nanocomposite: fabrication, characterization\nand properties","volume":"125","author":"Dong","year":"2019","journal-title":"Appl. Phys. A"},{"key":"2026081810421030500_cit42","doi-asserted-by":"publisher","first-page":"126658","DOI":"10.1016\/j.seppur.2024.126658","article-title":"Electroplating\nwastewater\ntreatment and resource recovery via a hybrid process of stepwise alkalization,\nFenton, and chlorination","volume":"339","author":"Liu","year":"2024","journal-title":"Sep. Purif. Technol."},{"key":"2026081810421030500_cit43","doi-asserted-by":"publisher","first-page":"123504","DOI":"10.1016\/j.watres.2025.123504","article-title":"Intensifying\ntransition metal ion\nremoval and recovery from acidic wastewater via electrodialysis (ED)\n-based process","volume":"280","author":"Ruya","year":"2025","journal-title":"Water Res."},{"issue":"8","key":"2026081810421030500_cit44","doi-asserted-by":"publisher","first-page":"082503","DOI":"10.1063\/5.0216272","article-title":"A comprehensive\nelectron wavefunction analysis toolbox for chemists, Multiwfn","volume":"161","author":"Lu","year":"2024","journal-title":"J. Chem. 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Soc."},{"issue":"1","key":"2026081810421030500_cit47","doi-asserted-by":"publisher","first-page":"3050","DOI":"10.1038\/s41467-025-58338-9","article-title":"Advanced enzyme-assembled\nhydrogels for the remediation of contaminated water","volume":"16","author":"Zhang","year":"2025","journal-title":"Nat. Commun."},{"issue":"1","key":"2026081810421030500_cit48","doi-asserted-by":"publisher","first-page":"4368","DOI":"10.1038\/s41467-022-31881-5","article-title":"Sustainable\nenvironmental remediation via biomimetic multifunctional lignocellulosic\nnano-framework","volume":"13","author":"Li","year":"2022","journal-title":"Nat. Commun."},{"issue":"9","key":"2026081810421030500_cit49","doi-asserted-by":"publisher","first-page":"5608","DOI":"10.1021\/acs.est.0c08224","article-title":"Thermal regeneration of spent granular\nactivated carbon\npresents an opportunity to break the forever PFAS cycle","volume":"55","author":"Baghirzade","year":"2021","journal-title":"Environ. Sci. Technol."},{"issue":"5","key":"2026081810421030500_cit50","doi-asserted-by":"publisher","first-page":"537","DOI":"10.1038\/s44160-025-00799-3","article-title":"Allosteric regulation in metal\u2013organic\ncages","volume":"4","author":"Yang","year":"2025","journal-title":"Nat. Synth."},{"issue":"47","key":"2026081810421030500_cit51","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202416799","article-title":"Cover Picture:\nAllostery at a Protein-Protein Interface Harboring an Intermolecular\nMotional Network (Angew. Chem. Int. Ed. 47\/2024)","volume":"63","author":"Medina Gomez","year":"2024","journal-title":"Angew. Chem., Int. 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