{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,7,28]],"date-time":"2026-07-28T14:06:56Z","timestamp":1785247616333,"version":"3.55.0"},"reference-count":61,"publisher":"American Chemical Society (ACS)","issue":"29","license":[{"start":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T00:00:00Z","timestamp":1784160000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T00:00:00Z","timestamp":1784160000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T00:00:00Z","timestamp":1784160000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52125001"],"award-info":[{"award-number":["52125001"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52370033"],"award-info":[{"award-number":["52370033"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003392","name":"Natural Science Foundation of Fujian Province","doi-asserted-by":"publisher","award":["2024J010021"],"award-info":[{"award-number":["2024J010021"]}],"id":[{"id":"10.13039\/501100003392","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,7,28]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Electrochemical CO2 reduction (CO2RR) under near-neutral conditions offers enhanced operational stability and compatibility with reactive carbon capture, yet downstream separation of dissolved products from supporting alkali cations remains a major barrier to practical deployment. Here we report a dual-cation-exchange-membrane solid electrolyte reactor (SER) that enables simultaneous organic acid separation, alkali cation recovery, and CO2 regeneration from neutral CO2RR effluents through highly efficient ion transport. Compared with state-of-the-art flow-electrode capacitive deionization systems, the SER exhibits substantially enhanced ion-transport performance without requiring flow electrodes or supporting electrolytes. Organic acids are selectively retained in the separation chamber with efficiencies of up to 94.7%, whereas more than 95% of alkali cations are recovered in the cathode chamber. Mechanistic analyses reveal that proton-assisted conductivity enhancement governs cation transport, whereas organic acid crossover remains limited and is primarily associated with electro-osmotic drag accompanying cation migration through the membrane. Integration of the SER with a practical reactive-capture electrolyzer demonstrates stable continuous coupling of carbon capture, electrochemical conversion, product separation and electrolyte recovery. These findings establish solid electrolyte reactors as an energy-efficient platform for electrochemical separations and highlight their potential for scalable downstream processing in CO2 electrovalorization systems.<\/jats:p>","DOI":"10.1021\/acs.est.6c05107","type":"journal-article","created":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T15:24:33Z","timestamp":1784215473000},"page":"20293-20303","source":"Crossref","is-referenced-by-count":0,"title":["Dual Cation-Exchange\nMembrane Solid Electrolyte Reactors\nfor Organic Acid Separation and Alkali Cation Recovery from Neutral\nCO2 Electroreduction"],"prefix":"10.1021","volume":"60","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-4968-3880","authenticated-orcid":true,"given":"Yong","family":"Jiang","sequence":"first","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenghao","family":"Xu","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hang","family":"Lin","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanwei","family":"Luo","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weihong","family":"Zheng","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bingjie","family":"Sun","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huilin","family":"Chen","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yan","family":"Wang","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xintong","family":"Xu","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiping","family":"Tang","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Na","family":"Chu","sequence":"additional","affiliation":[{"name":"Fujian Normal University , , ,","place":["Fuzhou, China, 350117"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3060-588X","authenticated-orcid":true,"given":"Raymond Jianxiong","family":"Zeng","sequence":"additional","affiliation":[{"name":"Fujian Agriculture and Forestry University , , ,","place":["Fuzhou, China, 350002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiangdong","family":"Zhu","sequence":"additional","affiliation":[{"name":"Institute of Soil Science, Chinese Academy of Sciences , , ,","place":["Nanjing, China, 210018"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7345-0844","authenticated-orcid":true,"given":"Peng","family":"Liang","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,16]]},"reference":[{"issue":"7","key":"2026072809095060300_cit1","doi-asserted-by":"publisher","first-page":"3648","DOI":"10.1021\/acs.chemrev.3c00206","article-title":"CO2 Electrolyzers","volume":"124","author":"O\u2019Brien","year":"2024","journal-title":"Chem. 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Chem., Int.\nEd."},{"issue":"51","key":"2026072809095060300_cit21","doi-asserted-by":"publisher","DOI":"10.1073\/pnas.2312876120","article-title":"Efficient and stable acidic CO2 electrolysis to formic\nacid by a reservoir structure design","volume":"120","author":"Chi","year":"2023","journal-title":"Proc.\nNatl. Acad. Sci. U. S. A."},{"issue":"32","key":"2026072809095060300_cit22","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202408412","article-title":"pH-Universal Electrocatalytic\nCO2 Reduction with Ampere-Level Current\nDensity on Doping-Engineered Bismuth Sulfide","volume":"63","author":"Jiang","year":"2024","journal-title":"Angew. Chem., Int. 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Technol."},{"key":"2026072809095060300_cit35","doi-asserted-by":"publisher","DOI":"10.1016\/j.ccr.2024.215835","article-title":"Design of\nthree-dimensional faradic electrode materials for high-performance\ncapacitive deionization","volume":"510","author":"Wang","year":"2024","journal-title":"Coord. Chem. 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Technol."},{"issue":"5","key":"2026072809095060300_cit38","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202505142","article-title":"Power-to-Protein:\nAnion-Exchange-Membrane-Free Solid-State Electrolysis for Efficient\nFormic Acid Production and Microbial Protein Synthesis","volume":"16","author":"Chu","year":"2026","journal-title":"Adv. Energy Mater."},{"issue":"4","key":"2026072809095060300_cit39","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202415806","article-title":"Fast Seawater Desalination Integrated\nwith Electrochemical CO2 Reduction","volume":"64","author":"Hu","year":"2025","journal-title":"Angew. Chem.,\nInt. 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