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Herein, a polyamide-based NF membrane was engineered via a complementary interface strategy involving (2-hydroxypropyl)-\u03b2-cyclodextrin (CD) doping and secondary sulfonamidation with sulfuryl chloride (SC). The resulting CD-PA-SC membrane exhibited excellent water permeance (26.9 L m\u22122 h\u22121 bar\u22121, 3.5- and 2.4-fold higher than NF 90 and NF 270), while maintaining high rejection for five typical EPs with diverse properties and selectively allowing the passage of dietary mineral ions. Time-of-flight secondary ion mass spectrometry analysis, transition state theory, MD simulation, and DFT calculations revealed that CD-PA-SC\u2019s thinner and more hydrophilic active layer promotes water permeance; its more negative surface charge facilitates mineral ion passage; and the tailored pore size, together with the CD-enhanced intrapore diffusion resistance, ensures enhanced broad-spectrum EP rejection. Thus, CD-PA-SC combines high efficiency, a low carbon footprint, and healthy water production, with promising applications in secondary water supply and point-of-use purifiers. This complementary dual-step modification strategy offers new insights into designing NF membranes for multiobjective separations in advanced drinking water treatment.<\/jats:p>","DOI":"10.1021\/acs.est.6c10025","type":"journal-article","created":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T16:20:20Z","timestamp":1788452420000},"page":"25894-25908","source":"Crossref","is-referenced-by-count":0,"title":["A\nHigh-Permeance\nNanofiltration Membrane via Complementary\nInterface Engineering for Enhanced Selectivity between Mineral Salts\nand Emerging Pollutants"],"prefix":"10.1021","volume":"60","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0113-9672","authenticated-orcid":true,"given":"Chenghai","family":"Lu","sequence":"first","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]},{"name":"University of Chinese Academy of Sciences , ,","place":["Beijing, China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu","family":"Sun","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]},{"name":"Shandong Jianzhu University , , ,","place":["Jinan, PR China, 250101"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhuofeng","family":"Zhou","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mingqi","family":"Zhang","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]},{"name":"University of Chinese Academy of Sciences , ,","place":["Beijing, China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1770-3522","authenticated-orcid":true,"given":"Guangzhi","family":"He","sequence":"additional","affiliation":[{"name":"University of Chinese Academy of Sciences , ,","place":["Beijing, China, 100049"]},{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9898-835X","authenticated-orcid":true,"given":"Chengzhi","family":"Hu","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Beijing, China, 100085"]},{"name":"University of Chinese Academy of Sciences , ,","place":["Beijing, China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,2]]},"reference":[{"issue":"6710","key":"2026091511105722400_cit1","doi-asserted-by":"publisher","first-page":"784","DOI":"10.1126\/science.adh9578","article-title":"Mapping safe drinking\nwater use in low- and middle-income countries","volume":"385","author":"Greenwood","year":"2024","journal-title":"Science"},{"issue":"1","key":"2026091511105722400_cit2","doi-asserted-by":"publisher","first-page":"7320","DOI":"10.1038\/s41467-024-51528-x","article-title":"Self-reported anticipated harm from\ndrinking water across 141 countries","volume":"15","author":"Miller","year":"2024","journal-title":"Nat. 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