{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T14:16:31Z","timestamp":1790000191678,"version":"4.0.1"},"reference-count":51,"publisher":"American Chemical Society (ACS)","issue":"37","license":[{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52403403"],"award-info":[{"award-number":["52403403"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52463033"],"award-info":[{"award-number":["52463033"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Guizhou Province","award":["Qian ke he ji chu - MS [2026] 167"],"award-info":[{"award-number":["Qian ke he ji chu - MS [2026] 167"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,21]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Solid-state lighting technologies for protected horticulture and data security demand luminescent materials whose emission characteristics can be precisely engineered. Here, a novel lead-free double perovskite Cs2NaLuCl6:Sb3+,Pr3+ was synthesized via a hydrothermal route to supply the blue and red photons essential for plant photosynthesis. Incorporating Sb3+ (ns2 configuration) into the host lattice generates broadband blue self-trapped exciton (STE) emission, while codoping with Pr3+ establishes an efficient energy-transfer pathway from STEs to the Pr3+\u00a03P0 state, promoting the 3P0 \u2192 3F2 transition at 653 nm to produce intense red light, thereby achieving blue-red dual-band emission within a single-component matrix. The as-fabricated LED exhibits an internal quantum efficiency of 59.09% and a spectral coincidence of 87.91% with the chlorophyll b absorption profile. Furthermore, leveraging its excitation-wavelength-dependent photoluminescence, a multilevel dynamic anticounterfeiting system employing excitation selectivity and long-pass optical filtering was demonstrated. A high-quality white LED was also constructed, achieving a color rendering index of 91.2, a correlated color temperature of 3602 K, and CIE coordinates of (0.3948, 0.3736). This work provides a high-performance phosphor for horticultural lighting, anticounterfeiting, and display applications.<\/jats:p>","DOI":"10.1021\/acs.inorgchem.6c03339","type":"journal-article","created":{"date-parts":[[2026,9,10]],"date-time":"2026-09-10T04:01:11Z","timestamp":1789012871000},"page":"21905-21919","source":"Crossref","is-referenced-by-count":0,"title":["Dual Self-Trapped\nExciton and Rare-Earth Emissions\nfrom Sb3\n                    <b>+<\/b>\n                    \/Pr3\n                    <b>+<\/b>\n                    -Activated\nMetal Halide toward Plant Cultivation Lighting, Dynamic Multilevel\nAnti-Counterfeiting, and High-CRI WLEDs"],"prefix":"10.1021","volume":"65","author":[{"given":"Yuanhui","family":"Dai","sequence":"first","affiliation":[{"name":"Guizhou University , , ,","place":["Guiyang, China, 550025"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huangyao","family":"Chen","sequence":"additional","affiliation":[{"name":"Guizhou University , , ,","place":["Guiyang, China, 550025"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ti","family":"Feng","sequence":"additional","affiliation":[{"name":"Guizhou University , , ,","place":["Guiyang, China, 550025"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiang","family":"Guo","sequence":"additional","affiliation":[{"name":"Guizhou University , , ,","place":["Guiyang, China, 550025"]},{"name":"Power Semiconductor Device Reliability Research Center of the Ministry of Education , ,","place":["Guiyang, China, 550025"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0001-0243-2793","authenticated-orcid":true,"given":"Ruirui","family":"Cui","sequence":"additional","affiliation":[{"name":"Guizhou University , , ,","place":["Guiyang, China, 550025"]},{"name":"Power Semiconductor Device Reliability Research Center of the Ministry of Education , ,","place":["Guiyang, China, 550025"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,9]]},"reference":[{"key":"2026092108520652500_cit1","doi-asserted-by":"publisher","first-page":"319","DOI":"10.1038\/s41377-024-01679-9","article-title":"Compositional engineering\nof phase-stable and highly efficient deep-red\nemitting phosphor for advanced plant lighting systems","volume":"13","author":"Qiao","year":"2024","journal-title":"Sci. Appl.: Light"},{"issue":"4","key":"2026092108520652500_cit2","doi-asserted-by":"publisher","first-page":"2414578","DOI":"10.1002\/adma.202414578","article-title":"Enhanced stability\nand brightness through co-substitution: promoting plant growth with\ngreen-excited deep red phosphor Ca1-zSrzLi1-xMg2xAl3-xN4: yEu2+","volume":"37","author":"Wang","year":"2025","journal-title":"Adv. Mater."},{"issue":"7","key":"2026092108520652500_cit3","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202419333","article-title":"Pseudohalide anions\ndriven structural modulation in\ndistorted tetrahedral manganese (II) hybrids toward tunable green-red\nemissions","volume":"64","author":"Zhang","year":"2025","journal-title":"Angew. Chem. Int. Ed."},{"issue":"1","key":"2026092108520652500_cit4","doi-asserted-by":"publisher","first-page":"5641","DOI":"10.1038\/s41467-025-60852-9","article-title":"Suppressing electron\u2013phonon\ncoupling for narrow-band emitting Eu (II)-based perovskitoids","volume":"16","author":"Han","year":"2025","journal-title":"Nat. Commun."},{"issue":"15","key":"2026092108520652500_cit5","doi-asserted-by":"publisher","first-page":"2418751","DOI":"10.1002\/adfm.202418751","article-title":"KBaScSi3O9:\nEu2+ glass-ceramics as single-phase high-power\nwhite emitters","volume":"35","author":"Kuang","year":"2025","journal-title":"Adv. Funct. Mater."},{"key":"2026092108520652500_cit6","doi-asserted-by":"publisher","first-page":"170825","DOI":"10.1016\/j.cej.2025.170825","article-title":"Photochromic properties and mechanism of Mn2+-doped Cs2AgInCl6 double perovskite\nhalides:\nimpact of synthesis route","volume":"525","author":"Yang","year":"2025","journal-title":"Chem. Eng. J."},{"issue":"1","key":"2026092108520652500_cit7","doi-asserted-by":"publisher","first-page":"2420","DOI":"10.1038\/s41467-023-38007-5","article-title":"A high-temperature\ndouble perovskite molecule-based antiferroelectric with excellent\nanti-breakdown capacity for energy storage","volume":"14","author":"Liu","year":"2023","journal-title":"Nat. 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Sci."},{"issue":"1","key":"2026092108520652500_cit11","doi-asserted-by":"publisher","first-page":"16","DOI":"10.1007\/s40820-019-0244-6","article-title":"Lead-free halide double perovskite\nmaterials: a new superstar toward green and stable optoelectronic\napplications","volume":"11","author":"Chu","year":"2019","journal-title":"Nano Micro Lett."},{"issue":"20","key":"2026092108520652500_cit12","doi-asserted-by":"publisher","first-page":"2207571","DOI":"10.1002\/advs.202207571","article-title":"Halide double perovskite nanocrystals doped with rare-earth\nions for multifunctional applications","volume":"10","author":"Li","year":"2023","journal-title":"Adv.\nSci."},{"issue":"28","key":"2026092108520652500_cit13","doi-asserted-by":"publisher","first-page":"11634","DOI":"10.1002\/anie.202004562","article-title":"Incorporating rare-earth\nterbium (III) ions into Cs2AgInCl6: Bi nanocrystals\ntoward tunable photoluminescence","volume":"59","author":"Liu","year":"2020","journal-title":"Angew. 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Technol."},{"key":"2026092108520652500_cit23","doi-asserted-by":"publisher","first-page":"103309","DOI":"10.1016\/j.mattod.2026.103309","article-title":"Concurrent\nphonon\nand bandgap engineering in a single host: toward color-tunable and\nperformance-programmable persistent luminescence phosphors","volume":"96","author":"Ding","year":"2026","journal-title":"Mater. Today"},{"issue":"9","key":"2026092108520652500_cit24","doi-asserted-by":"publisher","first-page":"3333","DOI":"10.1021\/acs.chemmater.9b00410","article-title":"Design\noptimization of lead-free perovskite Cs2AgInCl6: Bi nanocrystals with 11.4% photoluminescence quantum yield","volume":"31","author":"Liu","year":"2019","journal-title":"Chem. Mater."},{"issue":"21","key":"2026092108520652500_cit25","doi-asserted-by":"publisher","first-page":"5341","DOI":"10.1039\/D4MH00723A","article-title":"Lattice doping of lanthanide ions\nin Cs2ZrCl6 nanocrystals enabling phase transition\nand tunable photoluminescence","volume":"11","author":"Liu","year":"2024","journal-title":"Mater. Horiz."},{"issue":"12","key":"2026092108520652500_cit26","doi-asserted-by":"publisher","first-page":"1581","DOI":"10.1007\/s11426-018-9308-2","article-title":"X-ray scintillation\nin lead-free double perovskite crystals","volume":"61","author":"Hu","year":"2018","journal-title":"Sci.\nChina: Chem."},{"key":"2026092108520652500_cit27","doi-asserted-by":"publisher","first-page":"133","DOI":"10.1016\/j.jcis.2019.06.083","article-title":"Improved\nthermal\nstability of photoluminescence in Cs4PbBr6 microcrystals\/CsPbBr3 nanocrystals","volume":"554","author":"Wang","year":"2019","journal-title":"J. Colloid Interface\nSci."},{"issue":"13","key":"2026092108520652500_cit28","doi-asserted-by":"publisher","first-page":"2403289","DOI":"10.1002\/adom.202403289","article-title":"Double perovskite\nscintillators enabled by co-doped trap regulation for thermally enhanced\nx-ray imaging","volume":"13","author":"Huang","year":"2025","journal-title":"Adv. Opt. Mater."},{"issue":"23","key":"2026092108520652500_cit29","doi-asserted-by":"publisher","first-page":"18456","DOI":"10.1039\/D5RA01415H","article-title":"Rational design of a lead-free Cs2Na0.4Ag0.6In0.9Bi0.1Cl6: 0.15 Mn2+ double perovskite for enhancing\nthe colour rendition index\nof UV-pumped W-LEDs","volume":"15","author":"Balaji","year":"2025","journal-title":"RSC Adv."},{"issue":"13","key":"2026092108520652500_cit30","doi-asserted-by":"publisher","first-page":"4627","DOI":"10.1039\/D3TC04453J","article-title":"Near-infrared\nCr3+-doped lead-free halide perovskite microcrystals for\ninformation encryption and temperature thermometry","volume":"12","author":"Zhao","year":"2024","journal-title":"J. Mater. Chem. C"},{"issue":"6","key":"2026092108520652500_cit31","doi-asserted-by":"publisher","first-page":"3038","DOI":"10.1021\/acs.inorgchem.4c05370","article-title":"Designing polychromatic\nluminescence in Mn2+-doped Cs2NaLuCl6 double perovskite crystals via energy transfer\nengineering for optical thermometry and x-ray imaging","volume":"64","author":"Ge","year":"2025","journal-title":"Inorg. Chem."},{"issue":"22, Part A","key":"2026092108520652500_cit32","doi-asserted-by":"publisher","first-page":"36170","DOI":"10.1016\/j.ceramint.2025.05.338","article-title":"Bi3+-enhanced\nupconversion luminescence and high-sensitivity\noptical thermometry in Er3+\/Yb3+ co-doped Cs2NaYCl6 double perovskite crystals","volume":"51","author":"Wu","year":"2025","journal-title":"Ceram. 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Lett."},{"issue":"3","key":"2026092108520652500_cit36","doi-asserted-by":"publisher","first-page":"2202369","DOI":"10.1002\/adom.202202369","article-title":"Boosting energy transfer from self-trapped\nexciton to Er3+ through Sb3+ doping in Cs2Na (Lu\/Er) Cl6 double perovskites","volume":"11","author":"Zhang","year":"2023","journal-title":"Adv. Opt. Mater."},{"issue":"49","key":"2026092108520652500_cit37","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202514331","article-title":"Suppressed concentration quenching via divalent eu\/sr\nalloying in hybrid iodides scintillators toward bright luminescence\nfor x-ray imaging","volume":"64","author":"Chen","year":"2025","journal-title":"Angew. Chem. Int. 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Mater."},{"issue":"4","key":"2026092108520652500_cit40","doi-asserted-by":"publisher","first-page":"2308487","DOI":"10.1002\/adma.202308487","article-title":"Highly bright and stable lead-free double perovskite white light-emitting\ndiodes","volume":"36","author":"Jin","year":"2024","journal-title":"Adv. Mater."},{"issue":"23","key":"2026092108520652500_cit41","doi-asserted-by":"publisher","first-page":"10756","DOI":"10.1021\/acs.inorgchem.4c01339","article-title":"Sb3+\/Sm3+ codoped Cs2NaScCl6\nall-inorganic double perovskite: blue emission of self-trapped excitons\nand red-emission via energy transfer","volume":"63","author":"Jiang","year":"2024","journal-title":"Inorg.\nChem."},{"issue":"22","key":"2026092108520652500_cit42","doi-asserted-by":"publisher","first-page":"2002210","DOI":"10.1002\/advs.202002210","article-title":"Unveiling the excited-state dynamics of Mn2+ in 0D Cs4PbCl6 perovskite nanocrystals","volume":"7","author":"Zhang","year":"2020","journal-title":"Adv. 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Rare Earths"},{"issue":"34","key":"2026092108520652500_cit45","doi-asserted-by":"publisher","first-page":"23150","DOI":"10.1039\/D3CP03440B","article-title":"Glass-based\nLED system for indoor\nhorticulture: enhanced plant growth through Sm3+ and Tm3+ co-doped luminescent glasses","volume":"25","author":"Ekim","year":"2023","journal-title":"Phys.\nChem. Chem. Phys."},{"issue":"22","key":"2026092108520652500_cit46","doi-asserted-by":"publisher","first-page":"34805","DOI":"10.1016\/j.ceramint.2023.08.154","article-title":"Two-site\noccupancy induced a broadband blue-emitting in Eu2+ doped\nNa3Ba2Ca (PO4) 3 phosphor","volume":"49","author":"Wu","year":"2023","journal-title":"Ceram. Int."},{"issue":"19","key":"2026092108520652500_cit47","doi-asserted-by":"publisher","first-page":"23527","DOI":"10.1021\/acsami.3c03881","article-title":"Chromaticity-tunable\nall-inorganic color converters fabricated by 3D printing for modular\nplant growth lighting devices","volume":"15","author":"Yang","year":"2023","journal-title":"ACS Appl. Mater.\nInterfaces"},{"issue":"34","key":"2026092108520652500_cit48","doi-asserted-by":"publisher","first-page":"11793","DOI":"10.1039\/D1DT02088A","article-title":"Design of highly\nefficient deep-red emission in the Mn4+ doped new-type\nstructure CaMgAl10O17 for plant growth LED light","volume":"50","author":"Zhou","year":"2021","journal-title":"Dalton Trans."},{"issue":"15","key":"2026092108520652500_cit49","doi-asserted-by":"publisher","first-page":"25232","DOI":"10.1016\/j.ceramint.2023.05.056","article-title":"Blue-red dual color\nemitting phosphor Cs2NaLuCl6: Sb3+, Ho3+ for plant growth\nLEDs","volume":"49","author":"Chen","year":"2023","journal-title":"Ceram. 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