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Herein, wheat straw was converted into a biodegradable straw for potential food-contact applications through hierarchical interface engineering comprising stearic acid hydrophobization, a poly(lactic acid)\/cellulose nanocrystal-thioctic acid (PLA\/CNC-TA) reinforcing interlayer, and a polydopamine (PDA) outer layer. Stearic acid reduced water uptake, whereas CNC-TA enhanced interfacial compatibility and stress transfer through hydrogen bonding and thioctic-acid-associated interactions. The optimized PP4\/WS-SA straw achieved a tensile strength of 64.8 MPa and retained approximately 46 MPa after water exposure. PDA introduced catechol and amine groups, enabling partial capture of negatively charged micro-\/nano plastics (MNP), with a maximum turbidity-based removal efficiency of approximately 36%. The straw also exhibited improved thermal stability, food-simulant migration values below the tested limits, and progressive soil degradation, demonstrating a promising value-added application for agricultural-residue tableware.<\/jats:p>","DOI":"10.1021\/acs.jafc.6c07731","type":"journal-article","created":{"date-parts":[[2026,9,12]],"date-time":"2026-09-12T15:02:47Z","timestamp":1789225367000},"page":"31757-31770","source":"Crossref","is-referenced-by-count":0,"title":["Hierarchical Interlayer\nDesign for Wheat Straw-Based\nStraws: Exceptional Mechanical Robustness and In-Situ Capture of Micro\/Nano\nPlastics"],"prefix":"10.1021","volume":"74","author":[{"given":"Zihan","family":"Xu","sequence":"first","affiliation":[{"name":"Zhejiang Sci-Tech University , , Xiasha Higher Education Park Avenue 2 No.928 , ,","place":["Hangzhou, China, 310018"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Aiping","family":"Zhan","sequence":"additional","affiliation":[{"name":"Zhejiang Sci-Tech University , , Xiasha Higher Education Park Avenue 2 No.928 , ,","place":["Hangzhou, China, 310018"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaohong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Zhejiang Jingxing Paper Joint Stock Co., Ltd , ,","place":["Pinghu, China, 314214"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hou-Yong","family":"Yu","sequence":"additional","affiliation":[{"name":"Zhejiang Sci-Tech University , , Xiasha Higher Education Park Avenue 2 No.928 , ,","place":["Hangzhou, China, 310018"]},{"name":"Donghua University , , 2999 Renmin: North\u00b7 Road , Songjiang District, ,","place":["Shanghai, China, 201620"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,12]]},"reference":[{"key":"2026101408095919200_cit1","doi-asserted-by":"publisher","first-page":"6649","DOI":"10.1038\/s41467-025-61693-2","article-title":"Biomimetic\nlayered, ecological, advanced, multi-functional film for sustainable\npackaging","volume":"16","author":"Dhatt","year":"2025","journal-title":"Nat. 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