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Constructing novel fluorocarbon surfactant structures is one of the effective means of developing their alternatives. To this end, we herein prepared a novel fluorocarbon surfactant (BHFB) and compared its performance with that of a structurally analogous fluorocarbon surfactant (WTFB). The results indicate that BHFB with a rigid benzene ring structure exhibits superior surface activity. This is attributed to the \u03c0-\u03c0 stacking interaction of the benzene rings, which enables BHFB to arrange more tightly at the air-liquid interface. Consequently, BHFB exhibits lower surface tension and critical micelle concentration (CMC) (\u03b3CMC = 17.07 mN\/m, CMC = 1.098 \u00d7 10\u20135 mol\/L). Moreover, the introduction of the rigid benzene ring structure also improves the physicochemical properties of BHFB, such as thermal stability, aggregation behavior, wettability, and foam stability. In contrast, WTFB without a benzene ring structure is weaker than BHFB in all performance aspects. This work provides further insight into the structural design of novel eco-friendly fluorocarbon surfactants.<\/jats:p>","DOI":"10.1021\/acs.jpcb.6c03599","type":"journal-article","created":{"date-parts":[[2026,9,15]],"date-time":"2026-09-15T13:01:59Z","timestamp":1789477319000},"page":"10061-10075","source":"Crossref","is-referenced-by-count":0,"title":["Effects of the\nRigid Benzene Ring Spacer Group on\nthe Thermal Stability, Surface Activity and Aggregation Behavior of\nQuaternary Ammonium Salt Cationic Fluorocarbon Surfactants"],"prefix":"10.1021","volume":"130","author":[{"given":"Hao","family":"Hu","sequence":"first","affiliation":[{"name":"Nanjing University of Science and Technology , , ,","place":["Nanjing, P.R. China, 210094"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhencheng","family":"Yang","sequence":"additional","affiliation":[{"name":"Nanjing University of Science and Technology , , ,","place":["Nanjing, P.R. China, 210094"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hecheng","family":"Zhu","sequence":"additional","affiliation":[{"name":"Nanjing University of Science and Technology , , ,","place":["Nanjing, P.R. China, 210094"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Miao","family":"Xu","sequence":"additional","affiliation":[{"name":"Nanjing University of Science and Technology , , ,","place":["Nanjing, P.R. China, 210094"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Biao","family":"Jiang","sequence":"additional","affiliation":[{"name":"Nanjing University of Science and Technology , , ,","place":["Nanjing, P.R. China, 210094"]},{"name":"Chinese Academy of Sciences , , ,","place":["Shanghai, P. R. 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