{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,20]],"date-time":"2026-08-20T13:31:36Z","timestamp":1787232696017,"version":"build-2736575974"},"reference-count":70,"publisher":"American Chemical Society (ACS)","issue":"33","license":[{"start":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T00:00:00Z","timestamp":1785888000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T00:00:00Z","timestamp":1785888000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T00:00:00Z","timestamp":1785888000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100002865","name":"Chongqing Municipal Science and Technology Bureau","doi-asserted-by":"publisher","award":["CSTB2025TIAD-KPX0020"],"award-info":[{"award-number":["CSTB2025TIAD-KPX0020"]}],"id":[{"id":"10.13039\/501100002865","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100013160","name":"Venture and Innovation Support Program for Chongqing Overseas Returnees","doi-asserted-by":"publisher","award":["CX2021018"],"award-info":[{"award-number":["CX2021018"]}],"id":[{"id":"10.13039\/501100013160","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52173235"],"award-info":[{"award-number":["52173235"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Graduate Research and Innovation Foundation of Chongqing","award":["CYB25025"],"award-info":[{"award-number":["CYB25025"]}]},{"name":"Graduate Research and Innovation Foundation of Chongqing","award":["CYS25027"],"award-info":[{"award-number":["CYS25027"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,20]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>The massive emissions of carbon dioxide (CO2) have triggered serious ecological crises, presenting severe challenges for CO2 sequestration. Mineral carbon sequestration is a promising approach for the integration of carbon capture, utilization, and storage (CCUS). However, its reaction thermodynamic process is universally sluggish, and its in situ crystallization regulation strategies are insufficient. To address the above limitations, inspired by the rapid biomineralization of eggshells catalyzed by carbonic anhydrase (CA), we innovatively introduced amino-functionalized zeolitic imidazolate framework-8 (ZIF-8-NH2) to accelerate the thermodynamics of CO2 hydration and combined it with polyacrylamide (PAM) hydrogel with CaCl2 introduced to achieve in situ CaCO3 crystallization. Experimental results show that the carbon sequestration capacity reaches 7.12 mmol of CO2 ghydrogel\u20131. In terms of mechanistic interpretation, density functional theory (DFT) calculations confirm that ZIF-8-NH2 improves the adsorption performance for CO2, which is attributed to the strong interaction between \u2212NH2 and CO2. Simultaneously, it reduces the transition state (TS) energy barrier in the hydration reaction pathway, accordingly expediting the thermodynamics process. Furthermore, the products can remove heavy metal copper ions with a removal rate of nearly 40%. This work provides a new bioinspired strategy for the design of mineral carbon sequestration materials and broadens the application potential of carbon sequestration products.<\/jats:p>","DOI":"10.1021\/acs.jpclett.6c01941","type":"journal-article","created":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T20:02:09Z","timestamp":1785960129000},"page":"9694-9703","source":"Crossref","is-referenced-by-count":0,"title":["Biomineralization-Inspired\nHydrogels Enable Thermodynamically\nEnhanced CO2 Hydration for Efficient CO2 Sequestration"],"prefix":"10.1021","volume":"17","author":[{"given":"Shuyan","family":"Lu","sequence":"first","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhaoyu","family":"Chen","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tingna","family":"Luo","sequence":"additional","affiliation":[{"name":"The Third Military Medical University (Army Medical University) , , ,","place":["Chongqing, China, 400038"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kailiang","family":"Hu","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guanfeng","family":"Xue","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chong","family":"Cheng","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tingxu","family":"Song","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9334-0247","authenticated-orcid":true,"given":"Rixing","family":"Zhan","sequence":"additional","affiliation":[{"name":"The Third Military Medical University (Army Medical University) , , ,","place":["Chongqing, China, 400038"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6059-8962","authenticated-orcid":true,"given":"John","family":"Wang","sequence":"additional","affiliation":[{"name":"National University of Singapore , ,","place":["Singapore, 117573"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0087-3082","authenticated-orcid":true,"given":"Meng","family":"Li","sequence":"additional","affiliation":[{"name":"Chongqing University , , ,","place":["Chongqing, China, 400044"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,5]]},"reference":[{"issue":"3","key":"2026082008274098000_cit1","doi-asserted-by":"publisher","first-page":"360","DOI":"10.1038\/s41557-022-00904-5","article-title":"CO2 but\nnot as you know it","volume":"14","author":"Rudd","year":"2022","journal-title":"Nat. Chem."},{"issue":"4","key":"2026082008274098000_cit2","doi-asserted-by":"publisher","first-page":"243","DOI":"10.1038\/nclimate3231","article-title":"The role\nof CO2 capture and utilization in mitigating climate change","volume":"7","author":"Mac Dowell","year":"2017","journal-title":"Nat. Clim. Chang."},{"issue":"1","key":"2026082008274098000_cit3","doi-asserted-by":"publisher","first-page":"1694","DOI":"10.1038\/s41598-022-05151-9","article-title":"Innovative\nmethod for CO2 fixation and storage","volume":"12","author":"Sorimachi","year":"2022","journal-title":"Sci. Rep."},{"issue":"6396","key":"2026082008274098000_cit4","doi-asserted-by":"publisher","first-page":"9793","DOI":"10.1126\/science.aas9793","article-title":"Net-zero\nemissions energy systems","volume":"360","author":"Davis","year":"2018","journal-title":"Science"},{"key":"2026082008274098000_cit5","unstructured":"Olhoff, A.\n          \n          Emissions Gap Report\n2022: The Closing Window \u2500 Climate crisis calls for rapid transformation\nof societies; UNEP, 2022, https:\/\/www.unep.org\/emissions-gap-report-2022."},{"issue":"7781","key":"2026082008274098000_cit6","doi-asserted-by":"publisher","first-page":"87","DOI":"10.1038\/s41586-019-1681-6","article-title":"The technological\nand economic prospects for CO2 utilization and removal","volume":"575","author":"Hepburn","year":"2019","journal-title":"Nature"},{"key":"2026082008274098000_cit7","doi-asserted-by":"publisher","first-page":"1289","DOI":"10.1016\/j.apenergy.2018.11.019","article-title":"Carbon Capture, Utilization\nand Storage (CCUS)","volume":"235","author":"Yan","year":"2019","journal-title":"Appl. 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Technol."},{"issue":"7","key":"2026082008274098000_cit32","doi-asserted-by":"publisher","first-page":"1072","DOI":"10.1016\/j.arabjc.2018.07.012","article-title":"Economical,\nenvironmental\nfriendly synthesis, characterization for the production of zeolitic\nimidazolate framework-8 (ZIF-8) nanoparticles with enhanced CO2 adsorption","volume":"11","author":"Khan","year":"2018","journal-title":"Arab. J. Chem."},{"issue":"1","key":"2026082008274098000_cit33","doi-asserted-by":"publisher","first-page":"25","DOI":"10.1007\/s10450-012-9407-1","article-title":"Experimental and molecular\nsimulation studies of CO2 adsorption on zeolitic imidazolate frameworks:\nZIF-8 and amine-modified ZIF-8","volume":"19","author":"Liu","year":"2013","journal-title":"Adsorption"},{"key":"2026082008274098000_cit34","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijbiomac.2024.136928","article-title":"Efficient adsorption of flavonoids\non amino-functionalized ZIF-8\/chitosan aerogels","volume":"282","author":"Zhang","year":"2024","journal-title":"Int. J. Biol. Macromol."},{"key":"2026082008274098000_cit35","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2021.118376","article-title":"In situ growth\nof amino-functionalized ZIF-8 on bacterial cellulose foams for enhanced\nCO2 adsorption","volume":"270","author":"Ma","year":"2021","journal-title":"Carbohydr. 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Phys. Chem. Lett."},{"issue":"1","key":"2026082008274098000_cit49","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-025-66423-2","article-title":"Tough and tear resistant\nhydrogel with a sandwich mineralized structure\ninduced by bidirectional ion migration","volume":"16","author":"Yang","year":"2025","journal-title":"Nat.\nCommun."},{"key":"2026082008274098000_cit50","doi-asserted-by":"publisher","DOI":"10.1016\/j.seppur.2024.131090","article-title":"Enhanced CO2\nadsorption efficiency through aminoethylethanolamine functionalized\nporous ZIF-8 nanoparticles: Experimental investigations, isotherm\nand RSM modeling","volume":"360","author":"Sardar","year":"2025","journal-title":"Sep. Purif. Technol."},{"key":"2026082008274098000_cit51","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2019.123137","article-title":"Enhanced permeability\nin mixed matrix membranes for CO2 capture through\nthe structural regulation of the amino-functionalized Co\/ZIF-8 heterometallic\nnanoparticles","volume":"383","author":"Cong","year":"2020","journal-title":"Chem. Eng. J."},{"key":"2026082008274098000_cit52","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2024.122362","article-title":"Continuously\nenhanced versatile nanocellulose films\nenabled by sustaining CO2 capture and in-situ calcification","volume":"342","author":"Li","year":"2024","journal-title":"Carbohydr. 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