{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T19:45:36Z","timestamp":1792784736640,"version":"4.5.0"},"reference-count":52,"publisher":"American Chemical Society (ACS)","issue":"40","license":[{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"National Natural Science Foundation of China (NSFC)","award":["22275035"],"award-info":[{"award-number":["22275035"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"crossref"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,8]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Long-wavelength room-temperature phosphorescent carbon dots (CDs), especially the red phosphorescent ones, have garnered significant attention due to their low-energy emission and potential applications. However, the achievement of red phosphorescence in CDs presents a substantial challenge, and the underlying emission mechanism remains largely elusive. This work proposes a construction strategy for long-wavelength phosphorescence of CDs driven by matrix-induced low-energy charge transfer (CT) excited states. By guiding the directional migration and aggregation of intrinsic triplet excitons of CDs toward CT-related low-energy triplets, long-wavelength phosphorescence emission can be achieved without relying solely on traditional regulation of the intrinsic energy levels of phosphorescent centers. Based on this design philosophy, using (R)-methylbenzylamine and pyromellitic acid as precursors, long-wavelength room-temperature phosphorescent CDs were successfully constructed via a one-step hydrothermal method. Combining femtosecond transient absorption spectroscopy, single-crystal structure analysis, transmission electron microscopy, X-ray photoelectron spectroscopy, and theoretical calculations, it was confirmed that the formation of low-energy CT states induced by matrix effects drives the migration and aggregation of intrinsic triplet excitons toward CT-related low-energy triplets, constituting the key mechanism for long-wavelength phosphorescence generation. The broad applicability of this strategy was further validated using two different representative matrix systems. Therefore, the design strategy for long-wavelength CDs phosphorescence proposed in this study provides a new theoretical framework and design approach for the rational development of long-wavelength and even near-infrared CD-based phosphorescent materials.<\/jats:p>","DOI":"10.1021\/acs.jpclett.6c02632","type":"journal-article","created":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T07:02:09Z","timestamp":1790665329000},"page":"11583-11595","source":"Crossref","is-referenced-by-count":0,"title":["Triplet Exciton\nConvergence toward Charge-Transfer\nStates Enables Long-Wavelength Room-Temperature Phosphorescence from\nCarbon Dots"],"prefix":"10.1021","volume":"17","author":[{"given":"Guohui","family":"Yang","sequence":"first","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fu","family":"Qin","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xu","family":"Yu","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoyue","family":"Wang","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xinyu","family":"Wang","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianliang","family":"Bai","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shengyu","family":"Qian","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qian","family":"Wang","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pengsong","family":"Cui","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenyang","family":"Liu","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5140-1053","authenticated-orcid":true,"given":"Lili","family":"Ren","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,29]]},"reference":[{"key":"2026100811163675700_cit1","doi-asserted-by":"publisher","first-page":"6339","DOI":"10.1038\/s41467-025-61714-0","article-title":"Building\nBridges through Dynamic Coupling for Organic Phosphorescence","volume":"16","author":"Li","year":"2025","journal-title":"Nat. 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