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Among them, monolayer 1T-TaS2 is a well-known Mott insulating system, whose star-of-David charge density wave reconstruction realizes an emergent triangular lattice of local magnetic moments. Interestingly, in its bulk form, the insulating gap is not correlation-driven but stems from interlayer coupling. Here, we exploit the stacking-dependent nature of the insulating gap to show that, in twisted 1T-TaS2 bilayers, the spatially dependent competition between many-body and single-particle gaps creates Mott\u2013trivial mosaic superlattices, featuring regions with local magnetic moments and nonmagnetic insulating regions. We further demonstrate the tunability of the mosaic correlated state with an interlayer bias, giving rise to controllable charge transfer and quenching of correlations. Our results establish twisted 1T-TaS2 as a flexible platform to engineer mixed spatially modulated correlated insulating phases, arising from the moire\u0301 profile.<\/jats:p>","DOI":"10.1021\/acs.nanolett.6c01799","type":"journal-article","created":{"date-parts":[[2026,8,30]],"date-time":"2026-08-30T22:13:14Z","timestamp":1788127994000},"page":"13177-13184","source":"Crossref","is-referenced-by-count":0,"title":["Moire\u0301\nMott Correlated Mosaics in Twisted Bilayer\n1T-TaS2"],"prefix":"10.1021","volume":"26","author":[{"ORCID":"https:\/\/orcid.org\/0009-0006-6773-3622","authenticated-orcid":true,"given":"Ana","family":"Vera Montoto","sequence":"first","affiliation":[{"name":"Aalto University , , ,","place":["Espoo, Finland, 02150"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9916-1589","authenticated-orcid":true,"given":"Jose L.","family":"Lado","sequence":"additional","affiliation":[{"name":"Aalto University , , ,","place":["Espoo, Finland, 02150"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3385-6409","authenticated-orcid":true,"given":"Adolfo","family":"O. Fumega","sequence":"additional","affiliation":[{"name":"Aalto University , , ,","place":["Espoo, Finland, 02150"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,24]]},"reference":[{"key":"2026100710093338200_cit1","doi-asserted-by":"publisher","first-page":"201","DOI":"10.1038\/s41578-021-00284-1","article-title":"The marvels of moire\u0301 materials","volume":"6","author":"Andrei","year":"2021","journal-title":"Nat. Rev. Mater."},{"key":"2026100710093338200_cit2","doi-asserted-by":"publisher","first-page":"80","DOI":"10.1038\/nature26154","article-title":"Correlated\ninsulator behaviour at half-filling in magic-angle graphene superlattices","volume":"556","author":"Cao","year":"2018","journal-title":"Nature"},{"key":"2026100710093338200_cit3","doi-asserted-by":"publisher","first-page":"653","DOI":"10.1038\/s41586-019-1695-0","article-title":"Superconductors, orbital magnets and correlated states\nin magic-angle bilayer graphene","volume":"574","author":"Lu","year":"2019","journal-title":"Nature"},{"key":"2026100710093338200_cit4","doi-asserted-by":"publisher","first-page":"79","DOI":"10.1126\/science.adv8376","article-title":"Experimental\nevidence for nodal superconducting gap in moire\u0301 graphene","volume":"391","author":"Park","year":"2026","journal-title":"Science"},{"key":"2026100710093338200_cit5","doi-asserted-by":"publisher","first-page":"5528","DOI":"10.1038\/s41467-019-13488-5","article-title":"Parkinson, and Eli Sutter, \u201cSelf-organized twist-heterostructures\nvia aligned van der Waals epitaxy and solid-state transformations,\u201d","volume":"10","author":"Sutter","year":"2019","journal-title":"Nat. Commun."},{"key":"2026100710093338200_cit6","doi-asserted-by":"publisher","first-page":"075416","DOI":"10.1103\/PhysRevB.108.075416","article-title":"Electronic\nproperties of twisted Sb\/WTe2 van der Waals heterostructure\nwith controllable band gap, band alignment, and spin splitting","volume":"108","author":"Wang","year":"2023","journal-title":"Phys. Rev. B"},{"key":"2026100710093338200_cit7","doi-asserted-by":"publisher","first-page":"106","DOI":"10.1016\/j.mattod.2023.06.007","article-title":"Twisted cuprate van\nder Waals heterostructures with controlled Josephson coupling","volume":"67","author":"Martini","year":"2023","journal-title":"Mater. 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A."},{"key":"2026100710093338200_cit29","doi-asserted-by":"publisher","first-page":"2302989","DOI":"10.1002\/adfm.202302989","article-title":"en\u201cLayer Sliding And Twisting\nInduced Electronic Transitions In Correlated Magnetic 1t-Nbse2 Bilayers,\u201d","volume":"33","author":"Dai","year":"2023","journal-title":"Adv. Funct. Mater."},{"key":"2026100710093338200_cit30","doi-asserted-by":"publisher","first-page":"125136","DOI":"10.1103\/PhysRevB.106.125136","article-title":"Engineering\nchiral topological superconductivity in twisted Ising\nsuperconductors","volume":"106","author":"Hu","year":"2022","journal-title":"Phys. Rev. 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