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Beyond the well-known polariton ballistic-to-diffusive turnover in the linear response regime, these atomistic simulations reveal a nonlinear freezing mechanism of vibrational polariton transport; that is, under strong pumping of the upper polariton, the initially ballistically propagating upper polariton completely freezes and localizes energy to molecules at specific locations. This mechanism originates from pump-induced breaking of the in-plane translation symmetry: significant molecular excitations at the pulse hot spot broaden the polariton density of states, thus funneling population to the k\u2225 \u2192 0 band edge with vanishing group velocities. Overall, our work provides numerical insights for exploring novel mechanisms of vibrational polaritons.<\/jats:p>","DOI":"10.1021\/acs.nanolett.6c03367","type":"journal-article","created":{"date-parts":[[2026,9,14]],"date-time":"2026-09-14T17:01:53Z","timestamp":1789405313000},"page":"13012-13018","source":"Crossref","is-referenced-by-count":0,"title":["Nonlinear Freezing of Vibrational Polariton Transport\nvia Mesoscale Simulations"],"prefix":"10.1021","volume":"26","author":[{"ORCID":"https:\/\/orcid.org\/0009-0001-3704-1565","authenticated-orcid":true,"given":"Xinwei","family":"Ji","sequence":"first","affiliation":[{"name":"University of Delaware , , , ,","place":["Newark, Delaware, United States, 19716"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0361-5687","authenticated-orcid":true,"given":"Tao E.","family":"Li","sequence":"additional","affiliation":[{"name":"University of Delaware , , , ,","place":["Newark, Delaware, United States, 19716"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,14]]},"reference":[{"key":"2026093009092479700_cit1","doi-asserted-by":"publisher","first-page":"5981","DOI":"10.1038\/ncomms6981","article-title":"Coherent Coupling\nof Molecular Resonators with a Microcavity\nMode","volume":"6","author":"Shalabney","year":"2015","journal-title":"Nat. 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