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We designed a novel Cr(0) redox-neutral mode that overcomes traditional Cr(0)\/Cr(II) redox pathways in dearomatization chemistry using (\u03b76-arene)Cr(CO)3, thereby shifting the electrophile scope from obligatory cationic species to neutral nitrenes for the first time. This strategy enables both dearomative 1,2-hydroamination and 1,2-carboamination with exclusive regio- and stereocontrol, broad functional-group tolerance, and preferential site-selectivity for benzene rings over heteroarenes.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c02572","type":"journal-article","created":{"date-parts":[[2026,7,17]],"date-time":"2026-07-17T09:09:39Z","timestamp":1784279379000},"page":"9724-9729","source":"Crossref","is-referenced-by-count":0,"title":["Light-Promoted Dearomative Amination of Nonactivated\nArenes via Redox-Neutral Chromium\u2013Nitrenoid Transfer"],"prefix":"10.1021","volume":"28","author":[{"given":"Hui","family":"Xie","sequence":"first","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wei-Long","family":"Zeng","sequence":"additional","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chu-Qiao","family":"Li","sequence":"additional","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ming-Yang","family":"Wang","sequence":"additional","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hao-Song","family":"Wang","sequence":"additional","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8858-114X","authenticated-orcid":true,"given":"Wei","family":"Li","sequence":"additional","affiliation":[{"name":"Zhejiang University , , ,","place":["Hangzhou, China, 310058"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,17]]},"reference":[{"key":"2026073109274954100_cit1a","doi-asserted-by":"crossref","DOI":"10.1002\/9783527698479","volume-title":"Asymmetric\nDearomatization Reactions","author":"You","year":"2016"},{"key":"2026073109274954100_cit1b","doi-asserted-by":"publisher","first-page":"432","DOI":"10.1021\/acscentsci.0c01651","article-title":"Advances in Catalytic\nAsymmetric Dearomatization","volume":"7","author":"Zheng","year":"2021","journal-title":"ACS Cent. 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