{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T15:23:05Z","timestamp":1788535385429,"version":"build-2803163510"},"reference-count":51,"publisher":"American Chemical Society (ACS)","issue":"35","license":[{"start":{"date-parts":[[2026,8,26]],"date-time":"2026-08-26T00:00:00Z","timestamp":1787702400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,26]],"date-time":"2026-08-26T00:00:00Z","timestamp":1787702400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,26]],"date-time":"2026-08-26T00:00:00Z","timestamp":1787702400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"The Shanghai Municipal Science and Technology Major Project"}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,4]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Chiral aryl-substituted succinic acid diesters are valuable intermediates for the synthesis of wide range of chiral bioactive molecules, yet their enantioselective synthesis remains a significant challenge. Herein, we report the first example of a nickel-catalyzed asymmetric hydrogenation of aryl-substituted maleic acid diesters. This catalytic system exhibits a broad substrate scope and good functional-group tolerance, delivering the target products in up to 99% isolated yield and 97% ee (enantiomeric excess). The resulting succinic acid diesters can be readily converted into a variety of structurally diverse chiral derivatives. Mechanistic studies, including deuterium-labeling experiments and kinetic analysis, were conducted to elucidate the catalytic cycle, and a plausible reaction pathway is proposed.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c03282","type":"journal-article","created":{"date-parts":[[2026,9,1]],"date-time":"2026-09-01T11:15:18Z","timestamp":1788261318000},"page":"11111-11116","source":"Crossref","is-referenced-by-count":0,"title":["Nickel-Catalyzed\nAsymmetric Hydrogenation of Aryl-Substituted\nMaleic Acid Diesters"],"prefix":"10.1021","volume":"28","author":[{"given":"Jiawei","family":"Han","sequence":"first","affiliation":[{"name":"Henan Normal University , , ,","place":["Xinxiang, China, 453007"]},{"name":"Shanghai Jiao Tong University, Shanghai Academy of Natural Sciences (SANS) , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhiling","family":"Wang","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University, Shanghai Academy of Natural Sciences (SANS) , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yunshun","family":"Deng","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University, Shanghai Academy of Natural Sciences (SANS) , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianzhong","family":"Chen","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University, Shanghai Academy of Natural Sciences (SANS) , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ilya D.","family":"Gridnev","sequence":"additional","affiliation":[{"name":"Russian Academy of Sciences , , Leninsky Prospekt 47 , ,","place":["Moscow, Russian Federation, 119991"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0629-4524","authenticated-orcid":true,"given":"Hai-Ming","family":"Guo","sequence":"additional","affiliation":[{"name":"Henan Normal University , , ,","place":["Xinxiang, China, 453007"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4788-4195","authenticated-orcid":true,"given":"Wanbin","family":"Zhang","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University, Shanghai Academy of Natural Sciences (SANS) , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,26]]},"reference":[{"key":"2026090409091864100_cit1a","doi-asserted-by":"publisher","first-page":"2735","DOI":"10.1021\/cr9804543","article-title":"Design\nand Therapeutic Application of Matrix Metalloproteinase Inhibitors","volume":"99","author":"Whittaker","year":"1999","journal-title":"Chem. 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Chem."},{"key":"2026090409091864100_cit15e","doi-asserted-by":"publisher","first-page":"2876","DOI":"10.1021\/acs.chemrev.8b00404","article-title":"Hydride Transfer\nReactions Catalyzed by Cobalt Complexes","volume":"119","author":"Ai","year":"2019","journal-title":"Chem.\nRev."},{"key":"2026090409091864100_cit15f","doi-asserted-by":"publisher","first-page":"1101","DOI":"10.1021\/acs.accounts.9b00029","article-title":"P-Chiral Phosphorus\nLigands Based on a 2,3-Dihydrobenzo[d][1,3]Oxaphosphole\nMotif for Asymmetric Catalysis","volume":"52","author":"Xu","year":"2019","journal-title":"Acc. Chem. Res."},{"key":"2026090409091864100_cit15g","doi-asserted-by":"publisher","first-page":"1096","DOI":"10.6023\/cjoc201912025","article-title":"Recent Advances of\nNickel-Catalyzed Homogeneous Asymmetric Hydrogenation","volume":"40","author":"Liu","year":"2020","journal-title":"Chin. J. Org. Chem."},{"key":"2026090409091864100_cit15h","doi-asserted-by":"publisher","first-page":"3211","DOI":"10.1039\/D0CS00082E","article-title":"Asymmetric\nHydrogenation Catalyzed by First-Row Transition Metal Complexes","volume":"50","author":"Wen","year":"2021","journal-title":"Chem. Soc. Rev."},{"key":"2026090409091864100_cit15i","doi-asserted-by":"publisher","first-page":"3213","DOI":"10.6023\/cjoc202208003","article-title":"Earth-Abundant Metal-Catalyzed\nAsymmetric Hydrogenation of Carbon\u2013Nitrogen Unsaturated Bonds","volume":"42","author":"Liu","year":"2022","journal-title":"Chin. J. Org. Chem."},{"key":"2026090409091864100_cit15j","doi-asserted-by":"publisher","first-page":"646","DOI":"10.6023\/A23040140","article-title":"Development\nof Construction of Chiral C\u2013X Bonds through Nickel-Catalyzed\nAsymmetric Hydrogenation","volume":"81","author":"Cai","year":"2023","journal-title":"Acta Chim. Sinica"},{"key":"2026090409091864100_cit15k","doi-asserted-by":"publisher","first-page":"3135","DOI":"10.1002\/cjoc.202400352","article-title":"Earth-Abundant Nickel-Catalyzed Asymmetric Hydrogenation","volume":"42","author":"Wang","year":"2024","journal-title":"Chin. J. Chem."},{"key":"2026090409091864100_cit15l","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202315773","article-title":"Cobalt-Catalyzed Asymmetric Hydrogenation:\nSubstrate Specificity and Mechanistic Variability","volume":"63","author":"Chakrabortty","year":"2024","journal-title":"Angew. Chem. Int. Ed."},{"key":"2026090409091864100_cit15n","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202425589","article-title":"Weak Attractive\nNoncovalent Interactions in Metal-Catalyzed Asymmetric Hydrogenation","volume":"64","author":"Chen","year":"2025","journal-title":"Angew. Chem. Int. Ed."},{"key":"2026090409091864100_cit15o","doi-asserted-by":"publisher","DOI":"10.1016\/j.cclet.2025.111929","article-title":"Recent Advances on\nAsymmetric Reduction via Dynamic Kinetic Resolution","volume":"37","author":"Zhou","year":"2026","journal-title":"Chin. Chem. Lett."},{"key":"2026090409091864100_cit15p","doi-asserted-by":"publisher","DOI":"10.6023\/cjoc202606009","article-title":"Research Progress\non the Synthesis of Chiral Lactams via Transition Metal-Catalyzed\nAsymmetric Hydrogenation","author":"Liu","year":"2026","journal-title":"Chin. J. Org. Chem."},{"key":"2026090409091864100_cit15q","doi-asserted-by":"publisher","first-page":"2722","DOI":"10.1021\/acs.orglett.2c00826","article-title":"Nickel-Catalyzed Asymmetric Hydrogenation of \u03b3-Keto Acids, Esters, and Amides to Chiral \u03b3-Lactones and \u03b3-Hydroxy Acid\nDerivatives","volume":"24","author":"Xiao","year":"2022","journal-title":"Org. Lett."},{"key":"2026090409091864100_cit15r","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202306380","article-title":"Copper-Catalyzed Chemoselective Asymmetric Hydrogenation of C = O\nBonds of Exocyclic \u03b1, \u03b2-Unsaturated Pentanones","volume":"62","author":"Guan","year":"2023","journal-title":"Angew. Chem. Int.\nEd."},{"key":"2026090409091864100_cit15s","doi-asserted-by":"publisher","first-page":"556","DOI":"10.1038\/s41586-024-07581-z","article-title":"Asymmetric Hydrogenation of Ketimines with Minimally\nDifferent Alkyl Groups","volume":"631","author":"Wang","year":"2024","journal-title":"Nature"},{"key":"2026090409091864100_cit15t","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202416313","article-title":"Copper-Catalyzed Asymmetric Hydrogenation of Unsymmetrical Ortho-Br Substituted Benzophenones","volume":"64","author":"Guan","year":"2025","journal-title":"Angew. Chem. Int. 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Synth."},{"key":"2026090409091864100_cit16i","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202510401","article-title":"Enantioselective Nickel-Catalyzed\nHydrogenation of \u03b1-Alkylidene Succinimides\nEnabled by Weak Noncovalent Interactions","volume":"64","author":"Cai","year":"2025","journal-title":"Angew.\nChem. Int. Ed."},{"key":"2026090409091864100_cit16j","doi-asserted-by":"publisher","DOI":"10.1039\/D6SC05630J","article-title":"Nickel-Catalyzed Asymmetric\nHydrogenation of \u03b1,\u03b2-Unsaturated Ester Phosphonates","author":"Wei","year":"2026","journal-title":"Chem. Sci."},{"key":"2026090409091864100_cit17a","doi-asserted-by":"publisher","first-page":"153","DOI":"10.1002\/cjoc.201700645","article-title":"Efficient\nP-Chiral Biaryl Bisphosphorus Ligands for Palladium-Catalyzed Asymmetric\nHydrogenation","volume":"36","author":"Jiang","year":"2018","journal-title":"Chin. J. Chem."},{"key":"2026090409091864100_cit17b","doi-asserted-by":"publisher","first-page":"1987","DOI":"10.31635\/ccschem.023.202303564","article-title":"Asymmetric Autotandem Palladium Catalysis\nfor \u03b1,\u03b2-Unsaturated\nLactones: Merging Olefin and Ester Hydrogenation","volume":"6","author":"Sun","year":"2024","journal-title":"CCS Chem."},{"key":"2026090409091864100_cit18","doi-asserted-by":"publisher","first-page":"355","DOI":"10.1038\/s41586-018-0413-7","article-title":"Cooperative Asymmetric\nReactions Combining Photocatalysis and Enzymatic Catalysis","volume":"560","author":"Litman","year":"2018","journal-title":"Nature"},{"key":"2026090409091864100_cit19","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202204156","article-title":"Asymmetric Double Hydroxycarbonylation\nof Alkynes to Chiral Succinic\nAcids Enabled by Palladium Relay Catalysis","volume":"61","author":"Ji","year":"2022","journal-title":"Angew. Chem. Int. Ed."}],"container-title":["Organic Letters"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.orglett.6c03282","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/orlef7\/article-pdf\/28\/35\/11111\/67423893\/acs.orglett.6c03282.pdf","content-type":"application\/pdf","content-version":"vor","intended-application":"syndication"},{"URL":"https:\/\/pubs.acs.org\/orlef7\/article-pdf\/28\/35\/11111\/67423893\/acs.orglett.6c03282.pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T14:54:00Z","timestamp":1788533640000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/orlef7\/article\/28\/35\/11111\/5330134\/Nickel-Catalyzed-Asymmetric-Hydrogenation-of-Aryl"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,8,26]]},"references-count":51,"journal-issue":{"issue":"35","published-online":{"date-parts":[[2026,8,26]]},"published-print":{"date-parts":[[2026,9,4]]}},"URL":"https:\/\/doi.org\/10.1021\/acs.orglett.6c03282","relation":{},"ISSN":["1523-7060","1523-7052"],"issn-type":[{"value":"1523-7060","type":"print"},{"value":"1523-7052","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,8,26]]}}}