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The method employs diaryl ketone O-aroyl oximes as bifunctional reagents, serving as both radical precursors and nitrogen sources. Under mild visible-light irradiation, primary, secondary, and tertiary alcohol-derived xanthates are efficiently converted to imines with broad functional group tolerance. The protocol is practical, enabling gram-scale synthesis, one-pot imidation, and late-stage functionalization of complex molecules such as quinidine. Mechanistic studies indicate a radical pathway mediated by photocatalyst-induced energy transfer.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c03355","type":"journal-article","created":{"date-parts":[[2026,8,12]],"date-time":"2026-08-12T13:01:54Z","timestamp":1786539714000},"page":"10647-10652","source":"Crossref","is-referenced-by-count":1,"title":["Organophotocatalytic\nAryl Radical-Mediated Deoxygenative\nImination of Alcohols"],"prefix":"10.1021","volume":"28","author":[{"given":"Pan","family":"Huang","sequence":"first","affiliation":[{"name":"Yangzhou University , , Siwangting Road 180 , ,","place":["Yangzhou, China, 225002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Duo","family":"Zhang","sequence":"additional","affiliation":[{"name":"Guangxi University of Science and Technology , , Liushi Road 257 , ,","place":["Liuzhou, China, 545006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lianmin","family":"Yang","sequence":"additional","affiliation":[{"name":"Guangxi University of Science and Technology , , Liushi Road 257 , ,","place":["Liuzhou, China, 545006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shuli","family":"Wang","sequence":"additional","affiliation":[{"name":"Yangzhou University , , Siwangting Road 180 , ,","place":["Yangzhou, China, 225002"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4487-1820","authenticated-orcid":true,"given":"Guodong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Yangzhou University , , Siwangting Road 180 , ,","place":["Yangzhou, China, 225002"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,12]]},"reference":[{"issue":"14","key":"2026082212111746500_cit1a","doi-asserted-by":"publisher","first-page":"11622","DOI":"10.1021\/acs.jmedchem.4c01122","article-title":"An Update on the Nitrogen Heterocycle Compositions\nand Properties of U.S. FDA-Approved Pharmaceuticals (2013\u20132023)","volume":"67","author":"Marshall","year":"2024","journal-title":"J. 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