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Herein, we report the photothermal oxidation of benzylic C(sp3)\u2013H bonds to carbonyl compounds under air in combination with N-hydroxyphthalimide (NHPI) and Co(OAc)2\u00b74H2O. This method provides an efficient route for converting benzylic groups into the corresponding benzyl ketones.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c03627","type":"journal-article","created":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T13:05:34Z","timestamp":1790255134000},"page":"12447-12452","source":"Crossref","is-referenced-by-count":0,"title":["Photothermal Aerobic Oxidation of Benzylic C\u2013H\nBonds by NHPI\/PINO Catalysis"],"prefix":"10.1021","volume":"28","author":[{"given":"Hongtao","family":"Yang","sequence":"first","affiliation":[{"name":"East China University of Science and Technology , , 130 Meilong Road , ,","place":["Shanghai, P. R. China, 200237"]},{"name":"Anhui Haoyuan Chemical Group Company, Ltd. , Fukang Road No. 1 , , ,","place":["Fuyang, Anhui, P. R. China, 236056"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4025-5361","authenticated-orcid":true,"given":"Limin","family":"Wang","sequence":"additional","affiliation":[{"name":"East China University of Science and Technology , , 130 Meilong Road , ,","place":["Shanghai, P. R. China, 200237"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhenhan","family":"Wu","sequence":"additional","affiliation":[{"name":"Anhui Haoyuan Chemical Group Company, Ltd. , Fukang Road No. 1 , , ,","place":["Fuyang, Anhui, P. R. China, 236056"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8354-5684","authenticated-orcid":true,"given":"Jianwei","family":"Han","sequence":"additional","affiliation":[{"name":"East China University of Science and Technology , , 130 Meilong Road , ,","place":["Shanghai, P. R. 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