{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,16]],"date-time":"2026-10-16T13:55:55Z","timestamp":1792158955658,"version":"4.4.0"},"reference-count":37,"publisher":"American Chemical Society (ACS)","issue":"41","license":[{"start":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T00:00:00Z","timestamp":1791158400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T00:00:00Z","timestamp":1791158400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T00:00:00Z","timestamp":1791158400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22571249"],"award-info":[{"award-number":["22571249"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100007128","name":"Natural Science Foundation of Shaanxi Province","doi-asserted-by":"publisher","award":["2025JC-YBQN-120"],"award-info":[{"award-number":["2025JC-YBQN-120"]}],"id":[{"id":"10.13039\/501100007128","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,16]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Interception of aryldifluoromethyl radicals by unactivated alkenes is typically limited to 1,2-difunctionalization. We report a photoexcited palladium-catalyzed defluoroalkylative rearrangement that combines selective monodefluorination of trifluoromethylarenes, radical addition, local 1,2-migration, and carbonyl formation. The redox-neutral cascade achieves formal 1,2,3-trifunctionalization of allylic alcohols, providing \u03b1-alkynyl, \u03b1-aryl, and \u03b1-heteroaryl \u03b2-(aryldifluoromethyl) ketones with broad functional-group compatibility and without stoichiometric oxidants, thereby redirecting postaddition alkyl radicals from conventional termination toward migration-enabled skeletal reorganization under visible-light irradiation in a single operation.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c03929","type":"journal-article","created":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T07:02:27Z","timestamp":1791183747000},"page":"13064-13069","source":"Crossref","is-referenced-by-count":0,"title":["Photoexcited\nPalladium-Catalyzed Defluorinative 1,2-Functional-Group\nMigration of Allylic Alcohols"],"prefix":"10.1021","volume":"28","author":[{"given":"Xinyue","family":"Ma","sequence":"first","affiliation":[{"name":"Northwest University , , ,","place":["Xi\u2019an, China, 710127"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qianqian","family":"Li","sequence":"additional","affiliation":[{"name":"Northwest University , , ,","place":["Xi\u2019an, China, 710127"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wei","family":"Sun","sequence":"additional","affiliation":[{"name":"Northwest University , , ,","place":["Xi\u2019an, China, 710127"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7838-4003","authenticated-orcid":true,"given":"Zhijun","family":"Zuo","sequence":"additional","affiliation":[{"name":"Northwest University , , ,","place":["Xi\u2019an, China, 710127"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,5]]},"reference":[{"key":"2026101608472813300_cit1a","doi-asserted-by":"publisher","first-page":"320","DOI":"10.1039\/B610213C","article-title":"Fluorine in\nmedicinal chemistry","volume":"37","author":"Purser","year":"2008","journal-title":"Chem. 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