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In this transformation, arenes are first thianthrenated, followed by a cascade reaction of cycloisomerization, migratory insertion, and \u03b2-hydride elimination with enynones to afford furyl-substituted alkenylarenes. This highly site-selective olefination features excellent safety, a broad substrate scope, and good tolerance of halogen substituents. Notably, the successful derivatization of drug(like) molecules demonstrates the substantial potential of this method for the late-stage functionalization of arene-based drugs.<\/jats:p>","DOI":"10.1021\/acs.orglett.6c03954","type":"journal-article","created":{"date-parts":[[2026,9,28]],"date-time":"2026-09-28T12:01:50Z","timestamp":1790596910000},"page":"12837-12842","source":"Crossref","is-referenced-by-count":0,"title":["Thianthrenium\nSalt-Mediated Site-Selective Coupling\nof Arenes with Enynones"],"prefix":"10.1021","volume":"28","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5177-5282","authenticated-orcid":true,"given":"Shihaozhi","family":"Wang","sequence":"first","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jia-hui","family":"Shi","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shan","family":"Xu","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1429-9472","authenticated-orcid":true,"given":"Xue-jing","family":"Zhang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9888-0744","authenticated-orcid":true,"given":"Ming","family":"Yan","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,28]]},"reference":[{"key":"2026100910140475100_cit1a","doi-asserted-by":"publisher","first-page":"908","DOI":"10.1039\/C9CS00542K","article-title":"Recent progress\non donor and donor\u2013donor carbenes","volume":"49","author":"Zhu","year":"2020","journal-title":"Chem.\nSoc. 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