{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,19]],"date-time":"2026-10-19T08:47:50Z","timestamp":1792399670248,"version":"4.4.0"},"reference-count":47,"publisher":"American Chemical Society (ACS)","issue":"20","license":[{"start":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T00:00:00Z","timestamp":1790899200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T00:00:00Z","timestamp":1790899200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T00:00:00Z","timestamp":1790899200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["GNYZ2026004"],"award-info":[{"award-number":["GNYZ2026004"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["23CAA01015"],"award-info":[{"award-number":["23CAA01015"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52673172"],"award-info":[{"award-number":["52673172"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,19]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Infected wound repair requires hydrogel dressings that maintain antibacterial contact at wet, exudative, and mechanically dynamic tissue interfaces. Quaternary ammonium hydrogels provide intrinsic contact-active antibacterial activity, yet their performance is often limited by insufficient wet adhesion, weak network stability, and poor self-healing. Here, we report a dual-supramolecularly reinforced antibacterial hydrogel, PDQE\/PAGD-gel, constructed by integrating a quaternary ammonium bactericidal network with \u03b2-cyclodextrin-grafted poly(vinyl alcohol) reinforcement. In this design, quaternary ammonium groups provide membrane-disruptive contact bactericidal activity, while \u03b2-cyclodextrin-grafted poly(vinyl alcohol) reinforces the hydrated network through dual supramolecular interactions, including \u03b2-cyclodextrin\u2013alkyl host\u2013guest association and hydrogen bonding. Freeze\u2013thaw-induced PVA crystalline domains further serve as physical cross-linking points to improve network stability. This integrated network preserves antibacterial cationic accessibility while improving wet-tissue attachment, mechanical recovery, and interfacial stability. PDQE\/PAGD-gel exhibited a high equilibrium swelling ratio of 1052.2%, recovered mechanical integrity after damage, and achieved more than 99.5% contact bactericidal efficiency against Staphylococcus aureus and Escherichia coli within 140 min. It also showed low cytotoxicity, increased the L929 scratch closure rate to 65.4%, and maintained hemocompatibility with hemolysis below 4.0%. In a Staphylococcus aureus-infected full-thickness mouse wound model, PDQE\/PAGD-gel reduced bacterial burden and accelerated wound closure to 94.4% by day 12, accompanied by enhanced re-epithelialization and collagen deposition. This work establishes a dual-supramolecular physical-reinforcement strategy for contact-active antibacterial hydrogels in infected wound repair.<\/jats:p>","DOI":"10.1021\/acsabm.6c01592","type":"journal-article","created":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T11:01:33Z","timestamp":1790938893000},"page":"9901-9915","source":"Crossref","is-referenced-by-count":0,"title":["Dual-Supramolecularly Reinforced Quaternary Ammonium Hydrogel for Contact-Active Infected Wound Repair"],"prefix":"10.1021","volume":"9","author":[{"given":"Yixin","family":"Zhou","sequence":"first","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zilong","family":"Gao","sequence":"additional","affiliation":[{"name":"Beijing Institute of Technology , , ,","place":["Beijing, China, 100081"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu","family":"Zhang","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-4036-8465","authenticated-orcid":true,"given":"Xingjun","family":"Zhao","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ying","family":"Dai","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yiqing","family":"Zeng","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kai","family":"Yang","sequence":"additional","affiliation":[{"name":"Beijing Institute of Technology , , ,","place":["Beijing, China, 100081"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3305-8498","authenticated-orcid":true,"given":"Xiaofei","family":"Chen","sequence":"additional","affiliation":[{"name":"Beijing Institute of Technology , , ,","place":["Beijing, China, 100081"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7922-0599","authenticated-orcid":true,"given":"Li","family":"Chen","sequence":"additional","affiliation":[{"name":"Northeast Normal University , , ,","place":["Changchun, People's Republic of China, 130024"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,2]]},"reference":[{"issue":"7","key":"2026101904071206300_cit1","doi-asserted-by":"publisher","first-page":"389","DOI":"10.1089\/wound.2012.0381","article-title":"Biofilms and Inflammation in Chronic Wounds","volume":"2","author":"Zhao","year":"2013","journal-title":"Adv. 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