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To develop a fiber-based gas filter that is effective against SO2 gas, zeolite imidazole framework-8 (ZIF-8) was applied to polypropylene nonwoven by various methods. Among the tested methods, the sol\u2013gel impregnation method showed the highest ZIF-8 loading efficiency. There existed an optimal loading of ZIF-8 for the maximum adsorption efficiency, and it was associated with the accessibility of gas molecules to the ZIF-8 pores and active sites. Dominant adsorption processes and mechanisms were investigated by fitting the theoretical sorption models to experimental data. The results demonstrate that the increased ZIF-8 loading to fibers, beyond a certain level, may hinder the diffusivity and increase the barrier effect, eventually decreasing the adsorption efficiency. This study is novel and significant in that a multifaceted approach, including experimental analysis, theoretical investigation, and computational modeling, was made for scrutinizing the intricate phenomena occurring in the gas sorption process. The results of this study provide the fundamental yet practical information on the manufacturing considerations for the optimal design of MOF-loaded fibrous adsorbents.<\/jats:p>","DOI":"10.1021\/acsami.0c19957","type":"journal-article","created":{"date-parts":[[2021,1,4]],"date-time":"2021-01-04T13:29:34Z","timestamp":1609766974000},"page":"1620-1631","source":"Crossref","is-referenced-by-count":45,"title":["Fiber-Based\nGas Filter Assembled via In Situ Synthesis\nof ZIF-8 Metal Organic Frameworks for an Optimal Adsorption\nof SO2: Experimental and Theoretical Approaches"],"prefix":"10.1021","volume":"13","author":[{"given":"Jinwook","family":"Lee","sequence":"first","affiliation":[{"name":"Seoul National University , , ,","place":["Seoul, Republic of Korea, 08826"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3910-7281","authenticated-orcid":true,"given":"Kyeongeun","family":"Lee","sequence":"additional","affiliation":[{"name":"Seoul National University , , ,","place":["Seoul, Republic of Korea, 08826"]},{"name":"FITI Testing & Research Institute , , ,","place":["Seoul, Republic of Korea, 07791"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5043-9378","authenticated-orcid":true,"given":"Jooyoun","family":"Kim","sequence":"additional","affiliation":[{"name":"Seoul National University , , ,","place":["Seoul, Republic of Korea, 08826"]},{"name":"Seoul National University , , ,","place":["Seoul, Republic of Korea, 08826"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2021,1,4]]},"reference":[{"key":"2026090310511348200_cit1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201704679","article-title":"Adsorption and Detection\nof Hazardous Trace Gases by\nMetal\u2013Organic Frameworks","volume":"30","author":"Woellner","year":"2018","journal-title":"Adv. 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