{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T08:50:10Z","timestamp":1791535810386,"version":"4.3.4"},"reference-count":60,"publisher":"American Chemical Society (ACS)","issue":"37","license":[{"start":{"date-parts":[[2026,9,8]],"date-time":"2026-09-08T00:00:00Z","timestamp":1788825600000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/100018700","name":"HORIZON EUROPE Climate, Energy and Mobility","doi-asserted-by":"publisher","award":["101104032"],"award-info":[{"award-number":["101104032"]}],"id":[{"id":"10.13039\/100018700","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,23]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Anode-free solid-state batteries (AFSSBs) are promising candidates for next-generation high-energy-density batteries, but their widespread use is impeded by nonuniform lithium plating on the anode-side current collector (CC), which compromises stability and cycle life. Although the use of lithiophilic interlayers exhibits uniform Li plating, the underlying mechanisms by which they regulate lithium deposition are not yet fully understood. Here, a correlative focused ion beam\u2013scanning electron microscopy\u2013secondary ion mass spectrometry (FIB-SEM-SIMS) imaging approach combined with lithium isotope tracing is employed to investigate Li plating on different CC substrates. Half-cells with 6Li-enriched counter electrode and gel polymer electrolyte were assembled using bare Cu CC and Cu CC coated with 20 nm Ag and Au interlayers as working electrodes. Chronopotentiometry measurements revealed a nucleation overpotential of 59 mV for bare Cu CC, which decreased to below 1 mV for interlayer-coated substrates. Postmortem FIB-SEM-SIMS analysis was performed to correlate the electrochemical measurements with Li nucleation behavior of these substrates and investigate how differing Li nucleation mechanisms affected the subsequent distribution of Li+ flux. SEM data revealed a pronounced higher areal density of Li electrodeposits on interlayer coated substrates compared to bare Cu CC, while SIMS isotope mapping confirmed more uniform spatial distribution of Li+ flux for the interlayer coated substrates compared with bare Cu CC. Overall, the insights from this study highlight the critical role of CC substrate properties in developing high-performance AFSSBs.<\/jats:p>","DOI":"10.1021\/acsami.6c06240","type":"journal-article","created":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T11:06:56Z","timestamp":1790939216000},"page":"50694-50704","source":"Crossref","is-referenced-by-count":0,"title":["Correlative Electron-Ion Beam Analysis of the Effect of Lithiophilic Interlayers on Regulating the Li+ Flux Distribution in Anode Free Solid-State Batteries"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0009-0009-7940-8853","authenticated-orcid":true,"given":"Sayantan","family":"Sharma","sequence":"first","affiliation":[{"name":"Luxembourg Institute of Science and Technology , , ,","place":["Belvaux, Luxembourg, L-4422"]},{"name":"University of Luxembourg , 2 Avenue de l\u2019Universit\u00e9 , ,","place":["Esch-sur-Alzette, Luxembourg, L-4365"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1267-4224","authenticated-orcid":true,"given":"Alexander","family":"Santiago","sequence":"additional","affiliation":[{"name":"(Cic energigune), Basque Research and Technology Alliance (BRTA) , ,","place":["Vitoria-Gasteiz, Spain, 01510"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7023-0392","authenticated-orcid":true,"given":"Maria","family":"Martinez-Iba\u00f1ez","sequence":"additional","affiliation":[{"name":"(Cic energigune), Basque Research and Technology Alliance (BRTA) , ,","place":["Vitoria-Gasteiz, Spain, 01510"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Athira","family":"Suresh Kumar","sequence":"additional","affiliation":[{"name":"Luxembourg Institute of Science and Technology , , ,","place":["Belvaux, Luxembourg, L-4422"]},{"name":"University of Luxembourg , 2 Avenue de l\u2019Universit\u00e9 , ,","place":["Esch-sur-Alzette, Luxembourg, L-4365"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9968-6695","authenticated-orcid":true,"given":"Olivier","family":"De Castro","sequence":"additional","affiliation":[{"name":"Luxembourg Institute of Science and Technology , , ,","place":["Belvaux, Luxembourg, L-4422"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4966-7653","authenticated-orcid":true,"given":"Jean-Nicolas","family":"Audinot","sequence":"additional","affiliation":[{"name":"Luxembourg Institute of Science and Technology , , ,","place":["Belvaux, Luxembourg, L-4422"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4151-2304","authenticated-orcid":true,"given":"Santhana","family":"Eswara","sequence":"additional","affiliation":[{"name":"Luxembourg Institute of Science and Technology , , ,","place":["Belvaux, Luxembourg, L-4422"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,8]]},"reference":[{"issue":"3","key":"2026100820080810300_cit1","doi-asserted-by":"publisher","first-page":"194","DOI":"10.1038\/nnano.2017.16","article-title":"Reviving the Lithium Metal Anode for High-Energy Batteries","volume":"12","author":"Lin","year":"2017","journal-title":"Nat. Nanotechnol."},{"issue":"15","key":"2026100820080810300_cit2","doi-asserted-by":"publisher","first-page":"10403","DOI":"10.1021\/acs.chemrev.7b00115","article-title":"Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review","volume":"117","author":"Cheng","year":"2017","journal-title":"Chem. Rev."},{"issue":"1","key":"2026100820080810300_cit3","doi-asserted-by":"publisher","first-page":"19","DOI":"10.1038\/nchem.2085","article-title":"Towards Greener and More Sustainable Batteries for Electrical Energy Storage","volume":"7","author":"Larcher","year":"2015","journal-title":"Nat. Chem."},{"issue":"18","key":"2026100820080810300_cit4","doi-asserted-by":"publisher","first-page":"7961","DOI":"10.1021\/acs.chemmater.7b03002","article-title":"Surface Chemistry Mechanism of Ultra-Low Interfacial Resistance in the Solid-State Electrolyte Li7La3Zr2O12","volume":"29","author":"Sharafi","year":"2017","journal-title":"Chem. Mater."},{"issue":"9","key":"2026100820080810300_cit5","doi-asserted-by":"publisher","first-page":"845","DOI":"10.1016\/j.trechm.2019.06.013","article-title":"Chemo-Mechanical Challenges in Solid-State Batteries","volume":"1","author":"Lewis","year":"2019","journal-title":"Trends Chem."},{"issue":"39","key":"2026100820080810300_cit6","doi-asserted-by":"publisher","first-page":"7094","DOI":"10.1002\/adfm.201602353","article-title":"Anode-Free Rechargeable Lithium Metal Batteries","volume":"26","author":"Qian","year":"2016","journal-title":"Adv. Funct. Mater."},{"key":"2026100820080810300_cit7","doi-asserted-by":"publisher","first-page":"179","DOI":"10.1016\/j.ensm.2020.05.009","article-title":"Li2S-Based Anode-Free Full Batteries with Modified Cu Current Collector","volume":"30","author":"Chen","year":"2020","journal-title":"Energy Storage Mater."},{"issue":"8","key":"2026100820080810300_cit8","doi-asserted-by":"publisher","first-page":"A1291","DOI":"10.1149\/2.0091908jes","article-title":"Exploring the Impact of Mechanical Pressure on the Performance of Anode-Free Lithium Metal Cells","volume":"166","author":"Louli","year":"2019","journal-title":"J. Electrochem. Soc."},{"issue":"2","key":"2026100820080810300_cit9","doi-asserted-by":"publisher","first-page":"1132","DOI":"10.1021\/acs.nanolett.6b04755","article-title":"Nanoscale Nucleation and Growth of Electrodeposited Lithium Metal","volume":"17","author":"Pei","year":"2017","journal-title":"Nano Lett."},{"issue":"10","key":"2026100820080810300_cit10","doi-asserted-by":"publisher","first-page":"5289","DOI":"10.1039\/D1EE00767J","article-title":"Strategies towards Enabling Lithium Metal in Batteries: Interphases and Electrodes","volume":"14","author":"Horstmann","year":"2021","journal-title":"Energy Environ. Sci."},{"issue":"7","key":"2026100820080810300_cit11","doi-asserted-by":"publisher","first-page":"665","DOI":"10.1021\/acsmaterialslett.0c00152","article-title":"Controlling the Lithium-Metal Growth To Enable Low-Lithium-Metal-Excess All-Solid-State Lithium-Metal Batteries","volume":"2","author":"Liu","year":"2020","journal-title":"ACS Mater. Lett."},{"issue":"4","key":"2026100820080810300_cit12","doi-asserted-by":"publisher","first-page":"299","DOI":"10.1038\/s41560-020-0575-z","article-title":"High-Energy Long-Cycling All-Solid-State Lithium Metal Batteries Enabled by Silver\u2013Carbon Composite Anodes","volume":"5","author":"Lee","year":"2020","journal-title":"Nat. Energy"},{"issue":"10","key":"2026100820080810300_cit13","doi-asserted-by":"publisher","DOI":"10.1149\/1945-7111\/ac2d11","article-title":"Understanding the Effects of Alloy Films on the Electrochemical Behavior of Lithium Metal Anodes with Operando Optical Microscopy","volume":"168","author":"Sandoval","year":"2021","journal-title":"J. Electrochem. Soc."},{"key":"2026100820080810300_cit14","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2025.237567","article-title":"Unravelling the Effect of Interlayer Metal Materials on Li Deposition in Zero-Excess Lithium Batteries","volume":"653","author":"Xavier","year":"2025","journal-title":"J. Power Sources"},{"issue":"8","key":"2026100820080810300_cit15","doi-asserted-by":"publisher","first-page":"8148","DOI":"10.1021\/acsami.9b01521","article-title":"Lithiophilic Ag Nanoparticle Layer on Cu Current Collector toward Stable Li Metal Anode","volume":"11","author":"Hou","year":"2019","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"17","key":"2026100820080810300_cit16","doi-asserted-by":"publisher","first-page":"20125","DOI":"10.1021\/acsami.1c02621","article-title":"Lithiophilic 3D VN@N-RGO as a Multifunctional Interlayer for Dendrite-Free and Ultrastable Lithium-Metal Batteries","volume":"13","author":"Zhang","year":"2021","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"25","key":"2026100820080810300_cit17","doi-asserted-by":"publisher","first-page":"32259","DOI":"10.1021\/acsami.4c04060","article-title":"Constructing Reversible Li Deposition Interfaces by Tailoring Lithiophilic Functionalities of a Heteroatom-Doped Graphene Interlayer for Highly Stable Li Metal Anodes","volume":"16","author":"Son","year":"2024","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"18","key":"2026100820080810300_cit18","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202105924","article-title":"Plastic Monolithic Mixed-Conducting Interlayer for Dendrite-Free Solid-State Batteries","volume":"9","author":"Xiong","year":"2022","journal-title":"Adv. Sci."},{"issue":"28","key":"2026100820080810300_cit19","doi-asserted-by":"publisher","first-page":"7265","DOI":"10.1021\/acs.jpclett.4c01148","article-title":"Kelvin Probe Force Microscopy and Electrochemical Atomic Force Microscopy Investigations of Lithium Nucleation and Growth: Influence of the Electrode Surface Potential","volume":"15","author":"To-A-Ran","year":"2024","journal-title":"J. Phys. Chem. Lett."},{"issue":"12","key":"2026100820080810300_cit20","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201903993","article-title":"The Role of Interlayer Chemistry in Li-Metal Growth through a Garnet-Type Solid Electrolyte","volume":"10","author":"Kim","year":"2020","journal-title":"Adv. Energy Mater."},{"issue":"15","key":"2026100820080810300_cit21","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202003039","article-title":"Probing Lithium Metals in Batteries by Advanced Characterization and Analysis Tools","volume":"11","author":"Park","year":"2021","journal-title":"Adv. Energy Mater."},{"issue":"9","key":"2026100820080810300_cit22","doi-asserted-by":"publisher","first-page":"2054","DOI":"10.1016\/j.joule.2023.07.022","article-title":"Structural and Electrochemical Evolution of Alloy Interfacial Layers in Anode-Free Solid-State Batteries","volume":"7","author":"Sandoval","year":"2023","journal-title":"Joule"},{"issue":"4","key":"2026100820080810300_cit23","doi-asserted-by":"publisher","DOI":"10.1149\/1945-7111\/accab4","article-title":"Stable Lithium Plating in \u201cLithium Metal-Free\u201d Solid-State Batteries Enabled by Seeded Lithium Nucleation","volume":"170","author":"Haslam","year":"2023","journal-title":"J. Electrochem. Soc."},{"issue":"43","key":"2026100820080810300_cit24","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.add2000","article-title":"Unlocking the in Situ Li Plating Dynamics and Evolution Mediated by Diverse Metallic Substrates in All-Solid-State Batteries","volume":"8","author":"Cui","year":"2022","journal-title":"Sci. Adv."},{"key":"2026100820080810300_cit25","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2025.237328","article-title":"Laser-Induced Breakdown Spectroscopy for Surface Analysis of Solid-State Anode-Less Battery","volume":"647","author":"Capela","year":"2025","journal-title":"J. Power Sources"},{"issue":"29","key":"2026100820080810300_cit26","doi-asserted-by":"publisher","first-page":"16443","DOI":"10.1021\/acs.jpcc.5b03396","article-title":"Investigating Li Microstructure Formation on Li Anodes for Lithium Batteries by in Situ 6Li\/7Li NMR and SEM","volume":"119","author":"Chang","year":"2015","journal-title":"J. Phys. Chem. C"},{"issue":"36","key":"2026100820080810300_cit27","doi-asserted-by":"publisher","first-page":"47406","DOI":"10.1021\/acsami.4c06822","article-title":"Unraveling the Deposition and Dissolution Behavior of the Ag-Modified Li Surface Based on Electrochemical Atomic Force Microscopy","volume":"16","author":"To-A-Ran","year":"2024","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"10","key":"2026100820080810300_cit28","doi-asserted-by":"publisher","first-page":"3221","DOI":"10.1039\/C6EE01674J","article-title":"Transition of Lithium Growth Mechanisms in Liquid Electrolytes","volume":"9","author":"Bai","year":"2016","journal-title":"Energy Environ. Sci."},{"issue":"2","key":"2026100820080810300_cit29","doi-asserted-by":"publisher","DOI":"10.1073\/pnas.2012071118","article-title":"The Early-Stage Growth and Reversibility of Li Electrodeposition in Br-Rich Electrolytes","volume":"118","author":"Biswal","year":"2021","journal-title":"Proc. Natl. Acad. Sci."},{"issue":"45","key":"2026100820080810300_cit30","doi-asserted-by":"publisher","first-page":"20717","DOI":"10.1021\/jacs.2c08182","article-title":"Correlating Kinetics to Cyclability Reveals Thermodynamic Origin of Lithium Anode Morphology in Liquid Electrolytes","volume":"144","author":"Boyle","year":"2022","journal-title":"J. Am. Chem. Soc."},{"issue":"1","key":"2026100820080810300_cit31","doi-asserted-by":"publisher","first-page":"715","DOI":"10.1021\/acsenergylett.2c02387","article-title":"Early Stage Li Plating by Liquid Phase and Cryogenic Transmission Electron Microscopy","volume":"8","author":"Park","year":"2023","journal-title":"ACS Energy Lett."},{"issue":"6","key":"2026100820080810300_cit32","doi-asserted-by":"publisher","first-page":"5101","DOI":"10.1021\/acsaem.0c00543","article-title":"Operando Transmission Electron Microscopy Study of All-Solid-State Battery Interface: Redistribution of Lithium among Interconnected Particles","volume":"3","author":"Basak","year":"2020","journal-title":"ACS Appl. Energy Mater."},{"issue":"3","key":"2026100820080810300_cit33","doi-asserted-by":"publisher","DOI":"10.1038\/nenergy.2016.10","article-title":"Selective Deposition and Stable Encapsulation of Lithium through Heterogeneous Seeded Growth","volume":"1","author":"Yan","year":"2016","journal-title":"Nat. Energy"},{"key":"2026100820080810300_cit34","doi-asserted-by":"publisher","DOI":"10.1007\/978-1-4939-6676-9","volume-title":"Scanning Electron Microscopy and X-Ray Microanalysis","author":"Goldstein","year":"2018"},{"key":"2026100820080810300_cit35","doi-asserted-by":"publisher","DOI":"10.1007\/978-1-4419-9583-4","volume-title":"Electron Energy-Loss Spectroscopy in the Electron Microscope","author":"Egerton","year":"2011"},{"key":"2026100820080810300_cit36","doi-asserted-by":"publisher","first-page":"28705","DOI":"10.1038\/srep28705","article-title":"In-Situ Isotopic Analysis at Nanoscale Using Parallel Ion Electron Spectrometry: A Powerful New Paradigm for Correlative Microscopy","volume":"6","author":"Yedra","year":"2016","journal-title":"Sci. Rep."},{"issue":"6","key":"2026100820080810300_cit37","doi-asserted-by":"publisher","first-page":"1890","DOI":"10.1017\/S1431927622012405","article-title":"A FIB-SEM Based Correlative Methodology for X-Ray Nanotomography and Secondary Ion Mass Spectrometry: An Application Example in Lithium Batteries Research","volume":"28","author":"Cressa","year":"2022","journal-title":"Microsc. Microanal."},{"key":"2026100820080810300_cit38","doi-asserted-by":"publisher","DOI":"10.1016\/j.micron.2024.103746","article-title":"Visualizing the Li Distribution in an All-Solid-State Battery Composite Electrode Using Combined Plasma Focused-Ion Beam Microscopy and Secondary-Ion Mass Spectroscopy","volume":"190","author":"Sun","year":"2025","journal-title":"Micron"},{"key":"2026100820080810300_cit39","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijhydene.2025.150290","article-title":"Hydrogen Distribution in Electrochemically Charged Ti Thin Film: High Resolution SIMS Analysis of Electrolyte-Exposed vs Electrolyte-Free Surfaces","volume":"154","author":"Suresh Kumar","year":"2025","journal-title":"Int. J. Hydrogen Energy"},{"issue":"42","key":"2026100820080810300_cit40","doi-asserted-by":"publisher","first-page":"57141","DOI":"10.1021\/acsami.4c12915","article-title":"Lift-Out Specimen Preparation and Multiscale Correlative Investigation of Li-Ion Battery Electrodes Using Focused Ion Beam-Secondary Ion Mass Spectrometry Platforms","volume":"16","author":"Delfino","year":"2024","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"37","key":"2026100820080810300_cit41","doi-asserted-by":"publisher","first-page":"13943","DOI":"10.1016\/j.ijhydene.2022.12.216","article-title":"Correlative High-Resolution Imaging of Hydrogen in Mg2Ni Hydrogen Storage Thin Films","volume":"48","author":"Andersen","year":"2023","journal-title":"Int. J. Hydrogen Energy"},{"key":"2026100820080810300_cit42","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2020.228177","article-title":"Correlative Electron and Ion Beam Analysis of the Electrochemical Performances of LiV3O8 Cathode Films as a Function of Microstructures","volume":"463","author":"Sarbada","year":"2020","journal-title":"J. Power Sources"},{"key":"2026100820080810300_cit43","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2025.146728","article-title":"Operando Visualization of Li Distribution in Solid-State Batteries Using Focused Ion Beam-Secondary Ion Mass Spectrometry Imaging","volume":"536","author":"Sharma","year":"2025","journal-title":"Electrochim. Acta"},{"key":"2026100820080810300_cit44","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2025.111324","article-title":"Exploring Li Pathways in Si-C\/Gr Electrodes and Their SEI in Li Batteries Using Li Isotope Tracing by MAS NMR and FIB-SIMS","volume":"144","author":"Bofanova","year":"2025","journal-title":"Nano Energy"},{"key":"2026100820080810300_cit45","doi-asserted-by":"publisher","first-page":"9939","DOI":"10.1021\/acsaem.4c02023","article-title":"Isotopic Labeling: A Powerful Tool to Investigate Lithium Transport in a Polymer-Ceramic Composite Electrolyte Designed for Solid-State Batteries","volume":"7","author":"Meyer","year":"2024","journal-title":"ACS Appl. Energy Mater."},{"issue":"2","key":"2026100820080810300_cit46","doi-asserted-by":"publisher","first-page":"731","DOI":"10.1039\/d3ta05012b","article-title":"Visualization and Evaluation of Lithium Diffusion at Grain Boundaries in Li0.29La0.57TiO3 Solid Electrolytes Using Secondary Ion Mass Spectrometry","volume":"12","author":"Hasegawa","year":"2023","journal-title":"J. Mater. Chem. A Mater."},{"issue":"37","key":"2026100820080810300_cit47","doi-asserted-by":"publisher","first-page":"44268","DOI":"10.1021\/acsami.3c08829","article-title":"Lithium Self-Diffusion in a Polymer Electrolyte for Solid-State Batteries: ToF-SIMS\/SsNMR Correlative Characterization and Modeling Based on Lithium Isotopic Labeling","volume":"15","author":"Meyer","year":"2023","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"30","key":"2026100820080810300_cit48","doi-asserted-by":"publisher","first-page":"10754","DOI":"10.1021\/acs.analchem.2c01410","article-title":"Magnetic Sector Secondary Ion Mass Spectrometry on FIB-SEM Instruments for Nanoscale Chemical Imaging","volume":"94","author":"De Castro","year":"2022","journal-title":"Anal. Chem."},{"issue":"22","key":"2026100820080810300_cit49","doi-asserted-by":"publisher","first-page":"8812","DOI":"10.1021\/acs.chemmater.1c02952","article-title":"Safe, Flexible, and High-Performing Gel-Polymer Electrolyte for Rechargeable Lithium Metal Batteries","volume":"33","author":"Castillo","year":"2021","journal-title":"Chem. Mater."},{"issue":"26","key":"2026100820080810300_cit50","doi-asserted-by":"publisher","first-page":"9932","DOI":"10.1021\/acs.analchem.3c01059","article-title":"Toward Operando Structural, Chemical, and Electrochemical Analyses of Solid-State Batteries Using Correlative Secondary Ion Mass Spectrometry Imaging","volume":"95","author":"Cressa","year":"2023","journal-title":"Anal. Chem."},{"key":"2026100820080810300_cit51","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2024.144397","article-title":"Investigation of Li Accumulations in LLZO Based Solid State Batteries via Operando Neutron Imaging and Ex-Situ Correlative Structural and Chemical Analysis","volume":"494","author":"Cressa","year":"2024","journal-title":"Electrochim. Acta"},{"issue":"S2","key":"2026100820080810300_cit52","doi-asserted-by":"publisher","first-page":"1972","DOI":"10.1017\/S1431927620019984","article-title":"Magnetic Sector SIMS System with Continuous Focal Plane Detector for Advanced Analytical Capabilities on FIB Instruments","volume":"26","author":"Wirtz","year":"2020","journal-title":"Microsc. Microanal."},{"key":"2026100820080810300_cit53","doi-asserted-by":"publisher","first-page":"676","DOI":"10.1038\/nmeth.2019","article-title":"Fiji: An Open-Source Platform for Biological-Image Analysis","volume":"9","author":"Schindelin","year":"2012","journal-title":"Nat. Methods"},{"issue":"49","key":"2026100820080810300_cit54","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201905940","article-title":"Controlling Li Ion Flux through Materials Innovation for Dendrite-Free Lithium Metal Anodes","volume":"29","author":"Wang","year":"2019","journal-title":"Adv. Funct. Mater."},{"key":"2026100820080810300_cit55","doi-asserted-by":"publisher","first-page":"24","DOI":"10.1016\/j.ensm.2018.10.015","article-title":"Dendrite-Free Lithium Metal Anode Enabled by Separator Engineering via Uniform Loading of Lithiophilic Nucleation Sites","volume":"19","author":"Liu","year":"2019","journal-title":"Energy Storage Mater."},{"issue":"2","key":"2026100820080810300_cit56","doi-asserted-by":"publisher","first-page":"383","DOI":"10.1103\/PhysRev.184.383","article-title":"Theory of Sputtering. I Sputtering Yield of Amorphous and Polycrystalline Targets","volume":"184","author":"Sigmund","year":"1969","journal-title":"Phys. Rev."},{"key":"2026100820080810300_cit57","doi-asserted-by":"publisher","first-page":"291","DOI":"10.1007\/978-3-642-61871-0_86","volume-title":"The Bombardment Angle Dependence of the Sputtering and Secondary Ion Yield for Oxygen Ion Bombardment of Silicon","author":"Warmoltz","year":"1979"},{"issue":"13","key":"2026100820080810300_cit58","doi-asserted-by":"publisher","first-page":"9384","DOI":"10.1021\/acs.est.1c02971","article-title":"4D Surface Reconstructions to Study Microscale Structures and Functions in Soil Biogeochemistry","volume":"55","author":"Ost","year":"2021","journal-title":"Environ. Sci. Technol."},{"issue":"6","key":"2026100820080810300_cit59","doi-asserted-by":"publisher","DOI":"10.1016\/j.isci.2025.112765","article-title":"Entropy Measures for Quantifying Complexity in Digital Pathology and Spatial Omics","volume":"28","author":"Li","year":"2025","journal-title":"iScience"},{"issue":"7","key":"2026100820080810300_cit60","doi-asserted-by":"publisher","first-page":"44","DOI":"10.1007\/s11242-025-02183-3","article-title":"Entropy-Based Measure of Rock Sample Heterogeneity Derived from Micro-CT Images","volume":"152","author":"da Silva","year":"2025","journal-title":"Transp. Porous Media"}],"container-title":["ACS Applied Materials &amp; Interfaces"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acsami.6c06240","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/aamick\/article-pdf\/18\/37\/50694\/68451939\/am-2026-06240s.pdf","content-type":"application\/pdf","content-version":"vor","intended-application":"syndication"},{"URL":"https:\/\/pubs.acs.org\/aamick\/article-pdf\/18\/37\/50694\/68451939\/am-2026-06240s.pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T08:10:35Z","timestamp":1791533435000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/aamick\/article\/18\/37\/50694\/5426572\/Correlative-Electron-Ion-Beam-Analysis-of-the"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,9,8]]},"references-count":60,"journal-issue":{"issue":"37","published-online":{"date-parts":[[2026,9,8]]},"published-print":{"date-parts":[[2026,9,23]]}},"URL":"https:\/\/doi.org\/10.1021\/acsami.6c06240","relation":{},"ISSN":["1944-8244","1944-8252"],"issn-type":[{"value":"1944-8244","type":"print"},{"value":"1944-8252","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,9,8]]}}}