{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T12:25:13Z","timestamp":1786969513108,"version":"build-2736575974"},"reference-count":53,"publisher":"American Chemical Society (ACS)","issue":"30","license":[{"start":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T00:00:00Z","timestamp":1784505600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T00:00:00Z","timestamp":1784505600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T00:00:00Z","timestamp":1784505600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"State Key Laboratory of Advanced Polymer Materials","award":["sklapm2025-4-24"],"award-info":[{"award-number":["sklapm2025-4-24"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,5]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>A physically crosslinked multifunctional hydrogel based on poly(acrylic acid)\/hydroxypropyl cellulose\/aluminum chloride (PAA\/HPC\/AlCl3) was developed for flexible sensing applications. The network, constructed solely through hydrogen bonds and Al3+ coordination bonds, exhibits stretchability, adhesiveness, and reversible thermochromism. Freeze-thaw cycling serves as a green physical strategy to regulate performance: after treatment, tensile strength increased from 0.11 to 3.60 MPa, hysteresis strain decreased from 35 to 9.5%, and dissipated energy rose from 7.839 to 53.699 MJ\u00b7m\u20133. Low-field NMR reveals that freeze-thaw promotes water redistribution and chain aggregation, strengthening non-covalent interactions without introducing chemical crosslinkers. By adjusting Al3+ content and freeze-thaw cycles, the upper critical solution temperature (UCST) can be synergistically tuned between 15 and 54 \u00b0C, enabling reversible thermochromism. Before freeze-thaw, the hydrogel exhibits excellent adhesion, high strain sensitivity (GF = 5.4, 3\u2013500%), high temperature sensitivity (TCR = \u20130.019\/\u00b0C, detection limit 0.1 \u00b0C), and electromechanical self-healing, allowing accurate detection from human motion to Morse code. Post freeze-thaw, hydrogels combine high strength with stable thermoresponsive properties. In vitro hemolysis and CCK-8 assays confirmed the hydrogel's hemocompatibility and cytocompatibility. A preliminary in vivo wound contact test on rats revealed only mild, fully reversible irritation with no persistent damage. This work achieves differentiated performance regulation in a single system through a simple and environmentally friendly processing method, offering a sustainable design approach for flexible sensors.<\/jats:p>","DOI":"10.1021\/acsami.6c06534","type":"journal-article","created":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T17:08:13Z","timestamp":1784567293000},"page":"41336-41354","source":"Crossref","is-referenced-by-count":0,"title":["High-Strength, Tunable Thermoresponsive, Biocompatible, and Highly Sensitive Sensing Properties of Freeze-Thaw-Regulated Poly(acrylic acid)\/Hydroxypropyl Cellulose Hydrogels"],"prefix":"10.1021","volume":"18","author":[{"given":"Yifan","family":"Xie","sequence":"first","affiliation":[{"name":"Sichuan University , , ,","place":["Chengdu, China, 610065"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jincheng","family":"Zou","sequence":"additional","affiliation":[{"name":"Sichuan University , , ,","place":["Chengdu, China, 610065"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Senmiao","family":"Wang","sequence":"additional","affiliation":[{"name":"Sichuan University , , ,","place":["Chengdu, China, 610065"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9555-2013","authenticated-orcid":true,"given":"Minmin","family":"Fan","sequence":"additional","affiliation":[{"name":"Sichuan University , , ,","place":["Chengdu, China, 610065"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xi","family":"Zhang","sequence":"additional","affiliation":[{"name":"Sichuan University , , ,","place":["Chengdu, China, 610065"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,20]]},"reference":[{"key":"2026081707105151200_cit1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2023.121677","article-title":"Sodium carboxymethyl cellulose and MXene reinforced multifunctional conductive hydrogels for multimodal sensors and flexible supercapacitors","volume":"327","author":"Yin","year":"2024","journal-title":"Carbohydr. 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