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However, the regulatory role of metal centers with fully or partially filled d orbitals in interfacial behaviors during advanced oxidation processes remains insufficiently understood, posing a critical barrier to the development of efficient decontamination systems. In this study, we rationally designed and fabricated a series of MOF materials featuring ordered \u03c0-conjugated skeletons. These MOFs were constructed using 2-aminoterephthalic acid as the ligand, incorporating diverse metal nodes (Zn, Ti, and Co), and engineering hydrophilic or hydrophobic channels. The tetracycline (TC) degradation efficiencies of these MOFs under visible-light irradiation were systematically compared. By correlating the degradation results with structural characteristics elucidated via X-ray diffraction (XRD), Brunauer-Emmett-Teller (BET) surface area analysis, and X-ray photoelectron spectroscopy (XPS), combined with photoelectrochemical measurements, the influence of different metal centers on charge separation efficiency was comprehensively evaluated. The findings reveal that the Zn-MOF exhibits exceptional photocatalytic performance, which originates from the closed-shell d10 electronic configuration of Zn2+. This unique electronic structure confines electrons within the organic linker, effectively suppressing the recombination of photogenerated electron\u2013hole pairs. Furthermore, the incorporation of Zn2+ centers prolongs the lifetime of photoexcited electrons and optimizes the ligand-to-metal charge transfer (LMCT) process, thereby significantly enhancing photocatalytic activity. Radical trapping experiments identified superoxide radicals (\u2022O2\u2212), photogenerated electrons (e\u2212), and holes (h+) as the dominant reactive species involved in the TC degradation process. This work highlights the potential of water-stable MOFs with suppressed charge recombination for applications in various photochemical processes beyond water treatment.<\/jats:p>","DOI":"10.1021\/acsami.6c06917","type":"journal-article","created":{"date-parts":[[2026,10,21]],"date-time":"2026-10-21T11:01:28Z","timestamp":1792580488000},"source":"Crossref","is-referenced-by-count":0,"title":["Hydrophilic Zinc Metal-Organic Frameworks with Optimized Lewis Acid Centers for Enhanced Photocatalytic Performance"],"prefix":"10.1021","author":[{"given":"Jie","family":"Hu","sequence":"first","affiliation":[{"name":"School of Materials Science & Engineering, Jiangsu University , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hui","family":"Xu","sequence":"additional","affiliation":[{"name":"School of Materials Science & Engineering, Jiangsu University , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenfei","family":"Zhou","sequence":"additional","affiliation":[{"name":"School of Materials Science & Engineering, Jiangsu University , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weixia","family":"Zhou","sequence":"additional","affiliation":[{"name":"School of Materials Science & Engineering, Jiangsu University , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiya","family":"Lv","sequence":"additional","affiliation":[{"name":"Jiangsu University , , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chen","family":"Wu","sequence":"additional","affiliation":[{"name":"The Education University of Hong Kong , , ,","place":["Hong Kong, China, 999077"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Min","family":"Zhou","sequence":"additional","affiliation":[{"name":"Jiangsu University , , ,","place":["Zhenjiang, China, 212013"]},{"name":"The Education University of Hong Kong , , ,","place":["Hong Kong, China, 999077"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lele","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Materials Science & Engineering, Jiangsu University , ,","place":["Zhenjiang, China, 212013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Adnan","family":"Younis","sequence":"additional","affiliation":[{"name":"College of Science, United Arab Emirates University , , P.O. 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