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A recyclable biomimetic flexible sensor based on Ga-LM was prepared in this study. Nanofiber membranes were fabricated as flexible substrates via electrospinning. Concurrently, conductive inks were obtained by mechanical shearing and ultrasonication. The biomimetic spider-web-structured sensor was ultimately constructed by printing the conductive ink onto the flexible substrate. Experimental results showed that the flexible sensor exhibited a relative resistance change of less than 50% after 700 tensile cycles, demonstrating excellent tensile and electrical stability. The sensor exhibited high recyclability, with an average Ga-LM recovery rate of 95.88%, and demonstrated self-healing capability. In addition, the sensor had favorable biocompatibility, and its air and moisture permeability supported skin-contact wearable applications. In real-time ECG signal monitoring, the sensor achieved a high SNR of 34.88 dB, comparable to that of traditional sensors while offering advantages in flexibility, recyclability, durability, and wearability. This study offers new insights into ECG-monitoring smart clothing, where biomimetic design and material recycling facilitate the sustainable development of flexible sensors.<\/jats:p>","DOI":"10.1021\/acsami.6c08249","type":"journal-article","created":{"date-parts":[[2026,7,23]],"date-time":"2026-07-23T16:11:16Z","timestamp":1784823076000},"page":"40342-40352","source":"Crossref","is-referenced-by-count":1,"title":["A Recyclable Biomimetic Flexible Sensor Based on Gallium-Based Liquid Metal for Real-Time ECG Signal Monitoring"],"prefix":"10.1021","volume":"18","author":[{"given":"Jun","family":"Xu","sequence":"first","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tianjin Key Laboratory Optoelectronic Detection Technology and System , ,","place":["Tianjin, China, 300387"]},{"name":"Tianjin Furuixing Health Technology Co., Ltd. , ,","place":["Tianjin, China, 300350"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-2864-6643","authenticated-orcid":true,"given":"Leran","family":"Kuai","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peihong","family":"Yu","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuxiao","family":"Zhao","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cheng","family":"Zhang","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tianjin Key Laboratory Optoelectronic Detection Technology and System , ,","place":["Tianjin, China, 300387"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7563-9982","authenticated-orcid":true,"given":"Jia","family":"Shi","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]},{"name":"Tianjin University , , ,","place":["Tianjin, China, 300072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rize","family":"Jin","sequence":"additional","affiliation":[{"name":"Tiangong University , , ,","place":["Tianjin, China, 300387"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,23]]},"reference":[{"issue":"8","key":"2026080518112342100_cit1","doi-asserted-by":"publisher","first-page":"581","DOI":"10.1038\/s41569-021-00522-7","article-title":"Smart Wearable Devices in Cardiovascular Care: Where We Are and How to Move Forward","volume":"18","author":"Bayoumy","year":"2021","journal-title":"Nat. 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