{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,12]],"date-time":"2026-08-12T08:35:41Z","timestamp":1786523741583,"version":"build-2736575974"},"reference-count":54,"publisher":"American Chemical Society (ACS)","issue":"31","license":[{"start":{"date-parts":[[2026,7,29]],"date-time":"2026-07-29T00:00:00Z","timestamp":1785283200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,7,29]],"date-time":"2026-07-29T00:00:00Z","timestamp":1785283200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,7,29]],"date-time":"2026-07-29T00:00:00Z","timestamp":1785283200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,12]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Two-dimensional (2D) magnetic materials provide a fertile platform for exploring low-dimensional magnetism and anisotropy-driven magnetic ordering, yet achieving continuous and controllable tuning of magnetic anisotropy remains a significant challenge. Here, we report a systematic chemical strategy to modulate magnetic anisotropy in a family of quasi-2D-layered hybrid organic\u2013inorganic perovskites, (PEA)2Mn1\u2013xCuxCl4 (0 \u2264 x \u2264 1). Single crystals spanning the full compositional range were grown via a slow evaporation method, yielding phase-pure materials that exhibit continuous solid-solution behavior without phase segregation. Structural characterization confirms a common layered framework across all compositions, with gradual lattice evolution upon Mn2+\/Cu2+ substitution. Comprehensive DC and AC magnetization measurements performed along orthogonal crystallographic directions reveal a progressive transformation of the magnetic ground state from Ising-type antiferromagnetism in (PEA)2MnCl4 to XY-type ferromagnetism in (PEA)2CuCl4. Intermediate compositions display coexistence of antiferromagnetic and ferromagnetic interactions, accompanied by a continuous crossover from easy-axis to easy-plane magnetic anisotropy. Field-dependent measurements further demonstrate a coherent evolution of spin-flop behavior, hysteresis, and saturation magnetization across the series. These results establish chemical substitution as an effective and versatile route for engineering magnetic anisotropy in hybrid perovskites, positioning transition-metal-based 2D HOIPs as a chemically programmable platform for tunable low-dimensional magnetism and future spintronic applications.<\/jats:p>","DOI":"10.1021\/acsami.6c09056","type":"journal-article","created":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T13:15:37Z","timestamp":1785849337000},"page":"42848-42859","source":"Crossref","is-referenced-by-count":0,"title":["Composition-Driven Control of Magnetic Anisotropy in Hybrid Organic\u2013Inorganic Metal Halides"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-4255-8219","authenticated-orcid":true,"given":"Nilave","family":"Chakraborty","sequence":"first","affiliation":[{"name":"University of Utah , , 315 South 1400 East , , ,","place":["Salt Lake City, Utah, United States, 84112"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-4092-9735","authenticated-orcid":true,"given":"Puja","family":"Thapa","sequence":"additional","affiliation":[{"name":"North Carolina State University , , , ,","place":["Raleigh, North Carolina, United States, 27695"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-2366-8798","authenticated-orcid":true,"given":"Jacob Kjeldahl","family":"Jensen","sequence":"additional","affiliation":[{"name":"University of Utah , , 315 South 1400 East , , ,","place":["Salt Lake City, Utah, United States, 84112"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4662-3265","authenticated-orcid":true,"given":"Dali","family":"Sun","sequence":"additional","affiliation":[{"name":"North Carolina State University , , , ,","place":["Raleigh, North Carolina, United States, 27695"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1130-1306","authenticated-orcid":true,"given":"Luisa","family":"Whittaker-Brooks","sequence":"additional","affiliation":[{"name":"University of Utah , , 315 South 1400 East , , ,","place":["Salt Lake City, Utah, United States, 84112"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,29]]},"reference":[{"key":"2026081200063687800_cit1","doi-asserted-by":"publisher","first-page":"1237","DOI":"10.1039\/C1DT11544H","article-title":"Canted Antiferromagnetism and Spin Reorientation Transition in Layered Inorganic\u2013Organic Perovskite (C6H5CH2CH2NH3)2MnCl4","volume":"41","author":"Park","year":"2012","journal-title":"Dalton Trans."},{"key":"2026081200063687800_cit2","doi-asserted-by":"publisher","first-page":"95","DOI":"10.1103\/PhysRevB.62.95","article-title":"Magnetic Ordering in Two-Dimensional Heisenberg Antiferromagnets with Variable Interlayer Distances","volume":"62","author":"Lee","year":"2000","journal-title":"Phys. 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