{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,16]],"date-time":"2026-09-16T17:03:59Z","timestamp":1789578239816,"version":"build-2803163510"},"reference-count":51,"publisher":"American Chemical Society (ACS)","issue":"35","license":[{"start":{"date-parts":[[2026,8,24]],"date-time":"2026-08-24T00:00:00Z","timestamp":1787529600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,24]],"date-time":"2026-08-24T00:00:00Z","timestamp":1787529600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,24]],"date-time":"2026-08-24T00:00:00Z","timestamp":1787529600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100019082","name":"Shanghai Aerospace Science and Technology Innovation Foundation","doi-asserted-by":"publisher","award":["USCAST2024-076"],"award-info":[{"award-number":["USCAST2024-076"]}],"id":[{"id":"10.13039\/501100019082","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Aerospace Advanced Technology Joint Research Fund","award":["USCAST2022-43"],"award-info":[{"award-number":["USCAST2022-43"]}]},{"name":"Natural Science Foundation of Shanghai","award":["22ZR1432500"],"award-info":[{"award-number":["22ZR1432500"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,9]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Silicon is a premier anode candidate for next-generation lithium-ion batteries, yet its practical application is fundamentally impeded by colossal volumetric expansion and sluggish charge transport. While graphitic carbon nitride (g-C3N4) offers abundant lithiophilic sites as a buffering matrix, its inherent insulating nature and weak van der Waals interactions with Si inevitably lead to rapid structural degradation. Herein, we report a low-temperature molten salt-assisted magnesiothermic reduction strategy that enables the construction of conductive carbon nitride@silicon (CCN@Si) hybrid anodes featuring molecularly tethered interfaces. The AlCl3 molten salt acts as a unique molten-salt thermal-buffering medium that kinetically freezes Si nanoparticle growth. Concurrently, synchronized magnesiothermic denitridation (MD) triggers a critical insulator-to-conductor transition by restoring the delocalized \u03c0-conjugated carbon network. Crucially, this in situ process generates active surface dangling bonds, driving the spontaneous thermodynamic self-assembly of strong Si\u2212C covalent bonds at the heterointerface. Both experimental characterizations and theoretical calculations confirm that this robust interfacial tethering effectively buffers volumetric strain and ensures high-flux, bidirectional electron conduction. Consequently, the CCN@Si anode exhibits exceptional electrochemical stability, delivering a high reversible capacity of 1277.0 mAh g\u20131 after ultralong 2000 cycles at 2 A g\u20131. This defect-driven molecularly tethered paradigm offers a generalizable pathway for developing ultrastable energy storage systems.<\/jats:p>","DOI":"10.1021\/acsami.6c10119","type":"journal-article","created":{"date-parts":[[2026,8,31]],"date-time":"2026-08-31T21:16:05Z","timestamp":1788210965000},"page":"47640-47650","source":"Crossref","is-referenced-by-count":0,"title":["Molecularly Tethered Conductive Network Overcomes Capacity-Stability Trade-Off of Silicon Anodes"],"prefix":"10.1021","volume":"18","author":[{"given":"Yifeng","family":"Xu","sequence":"first","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kai","family":"Ye","sequence":"additional","affiliation":[{"name":"China-UK Low Carbon College, Shanghai Jiao Tong University , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qingdong","family":"Liu","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yiqiu","family":"Zhu","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lian","family":"Gao","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4251-3720","authenticated-orcid":true,"given":"Xuefeng","family":"Song","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,24]]},"reference":[{"issue":"3","key":"2026091612070185000_cit1","doi-asserted-by":"publisher","first-page":"180","DOI":"10.1038\/s41560-019-0338-x","article-title":"Pathways for practical high-energy long-cycling lithium metal batteries","volume":"4","author":"Liu","year":"2019","journal-title":"Nat. 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