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Effectively exciting and controlling defects in such devices, thereby enabling tunable optoelectronic responses, is critical for both functional realization and performance enhancement. Here, we report a MIS heterostructure photodetector consisting of monolayer graphene (Gr), hexagonal boron nitride (h-BN), and monolayer molybdenum disulfide (MoS2). Defect states within h-BN layers are successfully activated, allowing controlled interlayer charge transfer among the two-dimensional materials. Under visible-light illumination, the device reveals a wavelength-selective photoresponse at 405 and 638 nm. The mechanism underlying the selective photocurrent generation is elucidated through defect-state modeling of h-BN combined with energy-band alignment analysis. Notably, the device demonstrates a high switching ratio of up to 105 and an ultrafast response time of approximately 7\u20138 \u03bcs. These characteristics enable the demonstration of its potential for applications such as raster-scanned photocurrent imaging and optoelectronic logic operations.<\/jats:p>","DOI":"10.1021\/acsami.6c10578","type":"journal-article","created":{"date-parts":[[2026,8,9]],"date-time":"2026-08-09T19:01:57Z","timestamp":1786302117000},"page":"44633-44643","source":"Crossref","is-referenced-by-count":0,"title":["Manipulation of Photoresponse via Defect-Level Excitations in Metal\u2013Insulator\u2013Semiconductor-Type Two-Dimensional Heterostructure for Optoelectronic Logic Gates"],"prefix":"10.1021","volume":"18","author":[{"given":"Jiayuan","family":"Zhou","sequence":"first","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ran","family":"Tian","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yingjie","family":"Tao","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kaipeng","family":"Ni","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huanghuang","family":"Cheng","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chuangwei","family":"Wu","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shanyu","family":"Gao","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Danfeng","family":"Sun","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3084-8681","authenticated-orcid":true,"given":"Xuegang","family":"Chen","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6174-974X","authenticated-orcid":true,"given":"Wenshuai","family":"Gao","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7971-8354","authenticated-orcid":true,"given":"Yuxuan","family":"Jiang","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]},{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0870-995X","authenticated-orcid":true,"given":"Mingliang","family":"Tian","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]},{"name":"Chinese Academy of Sciences , , ,","place":["Hefei, China, 230031"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6562-7838","authenticated-orcid":true,"given":"Liang","family":"Li","sequence":"additional","affiliation":[{"name":"Hefei Institutes of Physical Science, Chinese Academy of Sciences , , ,","place":["Hefei, China, 230031"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9588-5491","authenticated-orcid":true,"given":"Xue","family":"Liu","sequence":"additional","affiliation":[{"name":"Anhui University , , ,","place":["Hefei, China, 230601"]},{"name":"Leibniz International Joint Research Center of Materials Sciences of Anhui Province , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,9]]},"reference":[{"key":"2026081907184950300_cit1","doi-asserted-by":"publisher","first-page":"839","DOI":"10.1038\/nnano.2009.292","article-title":"Ultrafast graphene photodetector","volume":"4","author":"Xia","year":"2009","journal-title":"Nat. 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