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Herein, we address this challenge by designing fully bio-based diblock copolymers (i.e., Glc6\/7-b-Sol) comprising hydrophilic maltooligosaccharide blocks predominantly composed of maltohexaose\/maltoheptaose (Glc6\/7) units and hydrophobic, plant-derived solanesol blocks. These copolymers form amphiphilic assemblies that integrate concentration-dependent viscoelasticity, mechanical responsiveness, and oil\u2013water interfacial stabilization. The copolymer self-assembles into ultra-high-aspect-ratio (\u22481200) wormlike micelles in water, each with a solanesyl core and sugar corona. Small-angle X-ray scattering experiments revealed significant inter-worm correlations at high concentrations, whereas the micellar cross-sectional diameter remained unchanged. Rheological measurements revealed strong concentration-dependent viscoelasticity at 40 g L\u20131, with a solution-to-gel-like transition affording elastic-dominated behavior, pronounced shear thinning, and full thixotropic recovery following repeated deformation at 1000% strain. The wormlike micelle rapidly fragmented into shorter segments when probe-sonicated, followed by partial reassembly of its length. The mechanically fragmented assemblies formed via sonication in the presence of oil were found to stabilize n-dodecane-in-water Pickering-like emulsions. The optimal 10 vol % n-dodecane-containing formulation afforded oil droplets with a mean diameter of 213 \u00b1 10 nm that showed long-term stability for over 17 d. These findings establish mechanically reversible, fully bio-based wormlike micelles with tunable viscoelasticities as sustainable, surfactant-free platform materials for food, pharmaceutical, and material formulations.<\/jats:p>","DOI":"10.1021\/acsami.6c10603","type":"journal-article","created":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T19:01:56Z","timestamp":1788548516000},"page":"50104-50119","source":"Crossref","is-referenced-by-count":0,"title":["Tunable Sugar\u2013Solanesol Block Copolymer Wormlike Micelles for Pickering-like Emulsions"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-5515-665X","authenticated-orcid":true,"given":"Weeranuch","family":"Lang","sequence":"first","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0003-2176-4587","authenticated-orcid":true,"given":"Sho","family":"Fukushima","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0704-2054","authenticated-orcid":true,"given":"Minami","family":"Ebe","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yurika","family":"Fujiwara","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-4001-1528","authenticated-orcid":true,"given":"Binti Hashim","family":"Hamidah","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8554-0636","authenticated-orcid":true,"given":"Takayuki","family":"Nonoyama","sequence":"additional","affiliation":[{"name":"Faculty of Advanced Life Science, Hokkaido University , ,","place":["Sapporo, Japan, 001-0021"]},{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 001-0021"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7245-586X","authenticated-orcid":true,"given":"Redouane","family":"Borsali","sequence":"additional","affiliation":[{"name":"Univ. Grenoble Alpes, CNRS, CERMAV , ,","place":["Grenoble, France, 38000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6775-9850","authenticated-orcid":true,"given":"Kenji","family":"Takahashi","sequence":"additional","affiliation":[{"name":"Kanazawa University , , ,","place":["Kanazawa, Japan, 920-1192"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6522-2523","authenticated-orcid":true,"given":"Feng","family":"Li","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9716-8237","authenticated-orcid":true,"given":"Takuya","family":"Yamamoto","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3238-813X","authenticated-orcid":true,"given":"Kenji","family":"Tajima","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5449-9642","authenticated-orcid":true,"given":"Toshifumi","family":"Satoh","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]},{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 001-0021"]},{"name":"National Central University , , ,","place":["Taoyuan, Taiwan, 320317"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3746-2084","authenticated-orcid":true,"given":"Takuya","family":"Isono","sequence":"additional","affiliation":[{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 060-8628"]},{"name":"Hokkaido University , , ,","place":["Sapporo, Japan, 001-0021"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,4]]},"reference":[{"key":"2026092323293232100_cit1","doi-asserted-by":"publisher","first-page":"77","DOI":"10.1016\/j.cis.2006.11.017","article-title":"Properties, Main Applications and Perspectives of Worm Micelles","volume":"128","author":"Ezrahi","year":"2007","journal-title":"Adv. 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