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Innovation Fund Project","award":["2025B-015"],"award-info":[{"award-number":["2025B-015"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Quinone-based organic electrodes are attractive for aqueous proton batteries owing to their fast and reversible proton-coupled redox chemistry. However, their practical application is largely restricted by severe dissolution in acidic electrolytes, poor structural stability, and low electronic conductivity. Herein, we report a molecularly anchored n-type quinone\/graphene heterostructure constructed by integrating tetraaminobenzoquinone (TABq) with reduced graphene oxide (rGO) through a facile solvothermal strategy. Strong \u03c0\u2013\u03c0 stacking, hydrogen-bonding interactions, and covalent linkages effectively immobilize TABq molecules on the conductive rGO framework, thereby suppressing active-material dissolution, enhancing electrode integrity, and constructing efficient electron\/proton transport pathways. The open heterointerface and abundant redox-active sites further promote rapid proton uptake\/release and accelerate charge-transfer kinetics. Benefiting from this rational heterostructure design, the optimized TABq\/rGO electrode delivers a high specific capacity of 349.78 mAh g\u20131 at 1 A g\u20131, remarkable rate capability of 131.12 mAh g\u20131 even at 100 A g\u20131, and excellent cycling durability. When coupled with a 3,4,9,10-perylenetetracarboxylic dianhydride anode, the full cell achieves a reversible capacity of 129.03 mAh g\u20131 at 0.75 A g\u20131 and maintains 75.43% of its capacity after 1000 cycles. Moreover, TABq\/rGO-based symmetric proton battery exhibits outstanding long-term stability, retaining 74.17% of its capacity after 10,000 cycles. Experimental characterizations combined with density functional theory calculations reveal that the TABq\/rGO heterointerface regulates charge distribution, stabilizes the quinone redox centers, and lowers the kinetic barrier for proton storage. This work highlights an effective molecular anchoring strategy for developing high-capacity, high-rate, and durable organic electrodes for advanced aqueous proton batteries.<\/jats:p>","DOI":"10.1021\/acsami.6c11056","type":"journal-article","created":{"date-parts":[[2026,10,13]],"date-time":"2026-10-13T20:01:57Z","timestamp":1791921717000},"source":"Crossref","is-referenced-by-count":0,"title":["Molecularly Anchored n-Type Quinone\/Graphene Heterostructures Enabling High-Capacity and Ultra-stable Proton Storage"],"prefix":"10.1021","author":[{"given":"Shimeng","family":"Guo","sequence":"first","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaopei","family":"Yang","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Baiting","family":"Li","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ran","family":"Wang","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yongqi","family":"Mi","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanxuan","family":"Yin","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sehrish","family":"Gull","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering, Nankai University , , ,","place":["Tianjin, China, 300350"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1826-3736","authenticated-orcid":true,"given":"Guankui","family":"Long","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering, Nankai University , , ,","place":["Tianjin, China, 300350"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5810-6009","authenticated-orcid":true,"given":"Pengcheng","family":"Du","sequence":"additional","affiliation":[{"name":"Lanzhou University , , ,","place":["Lanzhou, China, 730000"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,13]]},"reference":[{"key":"2026101316015248900_cit1","doi-asserted-by":"publisher","first-page":"928","DOI":"10.1126\/science.1212741","article-title":"Electrical Energy Storage for the Grid: a Battery of Choices","volume":"334","author":"Dunn","year":"2011","journal-title":"Science"},{"key":"2026101316015248900_cit2","doi-asserted-by":"publisher","first-page":"176","DOI":"10.1038\/s41893-022-00864-1","article-title":"Charging Sustainable Batteries","volume":"5","author":"Bauer","year":"2022","journal-title":"Nat. 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