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Nevertheless, although the emulsification capability was intrinsic, the catalytic active sites (Pd metal nanoclusters) remained \u201cextrinsic\u201d. In the present study, we successfully achieved both intrinsic emulsification and intrinsic catalysis using pristine MTT zeolite. The high anisotropy (anisotropy index = 23.2) and excellent dispersibility endowed the zeolite with favorable emulsifying performance, enabling the unmodified zeolite to effectively stabilize Pickering emulsions. Remarkably, Br\u00f8nsted acid sites are naturally present in pristine raw-MTT zeolite. Therefore, we successfully realized the integration of both intrinsic emulsification and intrinsic catalytic functionality within the same zeolitic material, greatly simplifying catalyst design. We constructed a Pickering interfacial catalytic system using fibrous MTT zeolite for epoxide hydration ring opening. The catalyst affords nearly quantitative substrate conversion (99.9%) within 20 min, along with a turnover frequency (TOF) of 70 h\u20131. Furthermore, the MTT zeolite preserves considerable catalytic activity and high recovery efficiency over five successive reaction cycles.<\/jats:p>","DOI":"10.1021\/acsami.6c11264","type":"journal-article","created":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T05:56:44Z","timestamp":1788415004000},"page":"50135-50146","source":"Crossref","is-referenced-by-count":0,"title":["Fibrous Intrinsic Zeolitic Pickering Interfacial Catalysts"],"prefix":"10.1021","volume":"18","author":[{"given":"Shuangjia","family":"Wang","sequence":"first","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qianjun","family":"Wang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenjun","family":"Jiang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Zhang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yiming","family":"Zhang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9664-3235","authenticated-orcid":true,"given":"Jiuxing","family":"Jiang","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , ,","place":["Guangzhou, China, 510006"]},{"name":"XinHuaYue Group , , ,","place":["Maoming, China, 525000"]},{"name":"Gannan Normal University , , ,","place":["Ganzhou, China, 341000"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,31]]},"reference":[{"issue":"3","key":"2026092323295402200_cit1","doi-asserted-by":"publisher","first-page":"167","DOI":"10.1007\/BF02932009","article-title":"Production of chiral epoxides: Epoxide hydrolase-catalyzed enantioselective hydrolysis","volume":"10","author":"Choi","year":"2005","journal-title":"Biotechnol. 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