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However, conventional 2D photodetectors typically rely on a single photoresponse mechanism, and studies on synergizing multiple physical mechanisms to enhance detection performance remain insufficient. Herein, we demonstrate a high-performance self-powered Gr\/InSe\/MoS2 van der Waals heterojunction photodetector with a unilateral depletion n-n junction. By rationally integrating graphene, InSe, and MoS2, the device realizes remarkable synergistic enhancement by dual-mechanism of photovoltaic and photothermoelectric effects. Benefiting from the thermoelectric field induced by the temperature gradient in MoS2 aligns with the built-in field of the n-n junction, effectively promote efficient photocarrier separation and significantly improving the photoresponse. Under zero-bias operation, it exhibits a broadband photoresponse from 355 to 1064 nm, a peak responsivity of 650 mA W\u22121 at 532 nm, an ultralow dark current of 5.3 \u00d7 10\u221213 A, and a fast rise time of 15.6 \u03bcs. Meanwhile, the device displays distinct polarization sensitivity originating from the in-plane anisotropy of InSe. It is successfully applied to image encryption, polarization imaging, and near-infrared optical communication, providing a promising strategy for designing advanced multifunctional self-powered photodetectors.<\/jats:p>","DOI":"10.1021\/acsami.6c11587","type":"journal-article","created":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T05:13:23Z","timestamp":1788412403000},"page":"49464-49475","source":"Crossref","is-referenced-by-count":0,"title":["Synergistic Dual-Mechanism Self-Powered Photodetector with Broadband Polarization Sensitivity for Multifunctional Applications"],"prefix":"10.1021","volume":"18","author":[{"given":"Jiaxuan","family":"Wang","sequence":"first","affiliation":[{"name":"Changchun University of Science and Technology , , ,","place":["Changchun, People\u2019s Republic of China, 130022"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9346-6146","authenticated-orcid":true,"given":"Yingtian","family":"Xu","sequence":"additional","affiliation":[{"name":"Changchun University of Science and Technology , , ,","place":["Changchun, People\u2019s Republic of China, 130022"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5948-2767","authenticated-orcid":true,"given":"Heng","family":"Liu","sequence":"additional","affiliation":[{"name":"Changchun University of Science and Technology , , ,","place":["Changchun, People\u2019s Republic of China, 130022"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1669-1358","authenticated-orcid":true,"given":"He","family":"Zhang","sequence":"additional","affiliation":[{"name":"Changchun University of Science and Technology , , ,","place":["Changchun, People\u2019s Republic of China, 130022"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yunping","family":"Lan","sequence":"additional","affiliation":[{"name":"Changchun University of Science and Technology , , ,","place":["Changchun, People\u2019s Republic of China, 130022"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,31]]},"reference":[{"issue":"30","key":"2026091614073561000_cit1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.201901347","article-title":"2D Metal Chalcogenides for IR Photodetection","volume":"15","author":"Wang","year":"2019","journal-title":"Small"},{"issue":"50","key":"2026091614073561000_cit2","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201804712","article-title":"The Interaction between Quantum Dots and Graphene: The Applications in Graphene-Based Solar Cells and Photodetectors","volume":"28","author":"Wu","year":"2018","journal-title":"Adv. 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