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The environmental and operational stability of the devices remains a significant issue, particularly in n-type OMIECs, prompting the molecular design of materials with lower LUMO levels and tighter intermolecular forces. In this work, we apply a common strategy that achieves these goals, fluorination, to our previously developed silicon phthalocyanine OMIEC and use silane-based surface treatments as a case study for the effect of surface treatment on the performance of small-molecule OECTs. When compared to the non-fluorinated material, bis(2-[2-(2-methoxyethoxy)ethoxy]acetate) silicon tetrafluoro phthalocyanine (MEEA-F4SiPc) OECTs fabricated on SiO2 demonstrate a lower threshold voltage (VT) at 0.406 \u00b1 0.056 V and better cycling stability. Using surface treatments resulted in faster uptake of ions when swelling as evidenced by EIS and Raman spectroscopy. Though this also resulted in slight improvements in the transient characteristics of the OECTs through faster \u03c4on values, the steady-state characteristics of the OECTs were unchanged. This study suggests surface treatment as a strategy for improved small-molecule OECT performance.<\/jats:p>","DOI":"10.1021\/acsami.6c11871","type":"journal-article","created":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T21:02:27Z","timestamp":1788469347000},"page":"49558-49568","source":"Crossref","is-referenced-by-count":0,"title":["Evaluating the Impact of Surface Treatments on a Fluorinated Silicon Phthalocyanine Organic Mixed Ionic-Electronic Conductor"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3216-3261","authenticated-orcid":true,"given":"May","family":"Ourabi","sequence":"first","affiliation":[{"name":"University of Ottawa , , 161 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8603-0507","authenticated-orcid":true,"given":"Nicolas","family":"Ledos","sequence":"additional","affiliation":[{"name":"University of Ottawa , , 161 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]},{"name":"University of Ottawa, , 150 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9959-2015","authenticated-orcid":true,"given":"Jaclyn","family":"Brusso","sequence":"additional","affiliation":[{"name":"University of Ottawa, , 150 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9863-7039","authenticated-orcid":true,"given":"Beno\u00eet H.","family":"Lessard","sequence":"additional","affiliation":[{"name":"University of Ottawa , , 161 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]},{"name":"University of Ottawa, , 150 Louis Pasteur , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]},{"name":"University of Ottawa , , 800 King Edward Ave. , , ,","place":["Ottawa, Ontario, Canada, K1N 6N5"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,3]]},"reference":[{"issue":"1","key":"2026091614065430300_cit1","doi-asserted-by":"publisher","first-page":"13","DOI":"10.1038\/s41563-019-0435-z","article-title":"Organic Mixed Ionic\u2212Electronic Conductors","volume":"19","author":"Paulsen","year":"2020","journal-title":"Nat. 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