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Here, we report a semi-crystalline hydrogel that couples stearyl methacrylate (SMA) side-chain crystallization\/melting with oligo(ethylene glycol) methyl ether methacrylate (OEGMA) lower critical solution temperature phase separation through 1,6-hexanediol diacrylate (HDDA) crosslinking. This dual-phase program generates three adaptive states: low-temperature latent-heat release with a temperature-dependent mid-infrared response, moderate-temperature transparency, and high-temperature broadband solar shielding. The optimized SMA60-OEGMA40-0.5HDDA hydrogel exhibits 92.25% luminous transmittance, 84.14% solar modulation efficiency, 75.11% near-infrared modulation, 1.02 MPa fracture stress, and 207.07% elongation. In model-window tests, it lowers the maximum indoor temperature by 12 \u00b0C relative to a commercial low-emissivity film and yields a 39% lower relative cooling-load index. By synergistically integrating phase-change thermal-energy storage and thermally induced optical regulation within a single material, this work provides a material-design strategy for mitigating conventional trade-offs among transparent daylighting, solar-heat shielding, and thermal management across different temperature ranges and demonstrates potential for passive thermal-management systems in energy-efficient building windows.<\/jats:p>","DOI":"10.1021\/acsami.6c13470","type":"journal-article","created":{"date-parts":[[2026,9,27]],"date-time":"2026-09-27T17:01:32Z","timestamp":1790528492000},"page":"53485-53494","source":"Crossref","is-referenced-by-count":0,"title":["Semi-crystalline Methacrylate Hydrogels for Multistage Solar and Thermal-Radiative Regulation"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-9639-6040","authenticated-orcid":true,"given":"Xiang","family":"Wang","sequence":"first","affiliation":[{"name":"Peking University School and Hospital of Stomatology & National Center for Stomatology & National Clinical Research Center for Oral Diseases & National Engineering Research Center of Oral Biomaterials and Digital Medical Devices & Beijing Key Laboratory of Digital Stomatology & NHC Key Laboratory of Digital Stomatology (Key Laboratory of Digital Stomatology, Chinese Academy of Medical Sciences) & NMPA Key Laboratory for Dental Materials , , ,","place":["Beijing, P. R. China, 100081"]},{"name":"The Chinese University of Hong Kong, Shenzhen , , ,","place":["Shenzhen, P. R. China, 518172"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xianyun","family":"Ma","sequence":"additional","affiliation":[{"name":"Peking University School and Hospital of Stomatology & National Center for Stomatology & National Clinical Research Center for Oral Diseases & National Engineering Research Center of Oral Biomaterials and Digital Medical Devices & Beijing Key Laboratory of Digital Stomatology & NHC Key Laboratory of Digital Stomatology (Key Laboratory of Digital Stomatology, Chinese Academy of Medical Sciences) & NMPA Key Laboratory for Dental Materials , , ,","place":["Beijing, P. R. China, 100081"]},{"name":"China University of Geosciences (Beijing) , , ,","place":["Beijing, P. R. 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