{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T20:48:51Z","timestamp":1791578931933,"version":"4.3.4"},"reference-count":45,"publisher":"American Chemical Society (ACS)","issue":"39","license":[{"start":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T00:00:00Z","timestamp":1790208000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T00:00:00Z","timestamp":1790208000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T00:00:00Z","timestamp":1790208000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100018542","name":"Natural Science Foundation of Sichuan Province","doi-asserted-by":"publisher","award":["2026YFHZ0055"],"award-info":[{"award-number":["2026YFHZ0055"]}],"id":[{"id":"10.13039\/501100018542","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Quality Engineering Program of South China Normal University","award":["2024-78"],"award-info":[{"award-number":["2024-78"]}],"id":[{"id":"https:\/\/ror.org\/01kq0pv72","id-type":"ROR","asserted-by":"crossref"}]},{"name":"Industry-University Collaboration Project of South China Normal University","award":["33326038"],"award-info":[{"award-number":["33326038"]}],"id":[{"id":"https:\/\/ror.org\/01kq0pv72","id-type":"ROR","asserted-by":"crossref"}]},{"name":"National Natural Science Foundation of China (NSFC)","award":["U2541258"],"award-info":[{"award-number":["U2541258"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"crossref"}]},{"name":"National Natural Science Foundation of China (NSFC)","award":["W2533150"],"award-info":[{"award-number":["W2533150"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"crossref"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,7]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Solid-state polymer electrolytes (SPEs) suffer from a persistent trade-off between sluggish ion transport and unstable electrode\u2013electrolyte interface. Herein, a synergistic \u201cpolymer grafting\u2013inorganic defect\u201d strategy is proposed to simultaneously address both bottlenecks. A low-crystallinity poly(vinylidene fluoride) (PVDF) matrix is first obtained via lithium sulfonate grafting (denoted as PVDF-STFE), which disrupts polymer chain packing and provides additional Li+ hopping sites. Into this matrix, we incorporated gadolinium-doped ceria (GDC) fillers rich in intrinsic oxygen vacancies. These vacancies act as strong Lewis acid sites that perform three coordinated functions: (i) anchoring TFSI\u2013 anions to promote salt dissociation, raising the Li+ transference number to 0.84; (ii) further disrupting polymer chain ordering to reduce crystallinity, lowering the activation energy for ion transport; and (iii) homogenizing interfacial Li+ flux to suppress dendritic growth. Control experiments using pristine CeO2, structurally identical but vacancy-deficient, confirm that oxygen vacancies, not mere physical filling, dominate these synergistic effects. The composite electrolyte comprising PVDF-STFE and GDC (denoted as PS-GDC) delivers a high room-temperature ionic conductivity (8.91 \u00d7 10\u20134 S cm\u20131), a wide electrochemical window over 5.0 V, and enables dendrite-free Li deposition as evidenced by post-cycling scanning electron microscopy (SEM). Quantitative X-ray photoelectron spectroscopy (XPS) reveals the formation of a LiF-enriched (65.11%) and parasitic-poor (24.02% Li\u2013O species) solid electrolyte interphase. Consequently, the assembled LiFePO4||Li cell retains 71.4% of its initial capacity after 400 cycles at 0.5 C and demonstrates stable operation up to 5 C. This work establishes a defect-mediated interfacial paradigm for designing a robust composite SPE.<\/jats:p>","DOI":"10.1021\/acsami.6c13878","type":"journal-article","created":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T10:01:55Z","timestamp":1790244115000},"page":"54006-54020","source":"Crossref","is-referenced-by-count":0,"title":["Oxygen-Vacancy-Mediated Triple Synergy in Gd-Doped Ceria Fillers Enables Dendrite-Free Solid-State Lithium Metal Batteries"],"prefix":"10.1021","volume":"18","author":[{"given":"Tian","family":"Ouyang","sequence":"first","affiliation":[{"name":"South China Normal University , , ,","place":["Shanwei, P. R. 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