{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,30]],"date-time":"2026-09-30T08:59:49Z","timestamp":1790758789852,"version":"4.1.0"},"reference-count":53,"publisher":"American Chemical Society (ACS)","issue":"38","license":[{"start":{"date-parts":[[2026,9,19]],"date-time":"2026-09-19T00:00:00Z","timestamp":1789776000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,19]],"date-time":"2026-09-19T00:00:00Z","timestamp":1789776000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,19]],"date-time":"2026-09-19T00:00:00Z","timestamp":1789776000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001665","name":"Agence Nationale de la Recherche","doi-asserted-by":"publisher","award":["ANR-10-EQPX-37"],"award-info":[{"award-number":["ANR-10-EQPX-37"]}],"id":[{"id":"10.13039\/501100001665","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001665","name":"Agence Nationale de la Recherche","doi-asserted-by":"publisher","award":["ANR-18-CE24-0016"],"award-info":[{"award-number":["ANR-18-CE24-0016"]}],"id":[{"id":"10.13039\/501100001665","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001665","name":"Agence Nationale de la Recherche","doi-asserted-by":"publisher","award":["ANR-21-CE30-0059"],"award-info":[{"award-number":["ANR-21-CE30-0059"]}],"id":[{"id":"10.13039\/501100001665","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001665","name":"Agence Nationale de la Recherche","doi-asserted-by":"publisher","award":["ANR-24-CE09-3415-02"],"award-info":[{"award-number":["ANR-24-CE09-3415-02"]}],"id":[{"id":"10.13039\/501100001665","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,30]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Processing-induced interfacial losses limit perovskite nanocrystal light-emitting diodes (PeLEDs) at display-relevant device areas, yet the steps responsible are rarely identified with statistical confidence beyond champion-device reporting. Here, we combine an all-inorganic CsPbBr3 emitter with a replicated factorial study at 28 mm2 active area. Nanocrystals capped with phenylpropylamine (PPA) by a room-temperature modified ligand-assisted reprecipitation (MLARP) route are deposited as two sequential films separated by a \u223c2.8 nm polyvinylpyrrolidone (PVP) interlayer, with mild vacuum conditioning before the top layer. Seven of thirteen architectures were replicated over two fabrication sessions, giving 71 functional devices from 84 (84.5% yield). A matched 2 \u00d7 2 factorial ANOVA identifies vacuum conditioning as the dominant factor for EQE (partial \u03b72 = 0.90), with a smaller but significant PVP contribution (p = 0.006) and a significant PVP \u00d7 vacuum interaction for maximum luminance (p &amp;lt; 0.001). The combined route gives a median EQEmax of 12.2% (IQR 0.5%) at 12\/12 yield and a champion device with EQEmax = 13.23% at 520 nm, 21,537 cd.m\u20132, 30.8 lm.W\u20131 at 100 cd.m\u20132, 1.7% roll-off at 10 mA.cm\u20132, and encapsulated \u03c450 = 3 h at 200 cd.m\u20132, measured in an integrating sphere. Photoluminescence lifetimes recover from 5.0 to 14.9 ns in the bilayer and the corresponding photoluminescence quantum yield from 8.9% to 28.7%. Across solution, film and both half-device stacks the quantum yield scales linearly with the amplitude-weighted lifetime at a common radiative rate, placing these losses in nonradiative channels and consistent with reduced interfacial quenching. At the same time, transfer-matrix modeling shows outcoupling to be emitter-position dependent (10.4% vs 13.3%), so radiative, transport, and optical contributions remain unseparated. The PVP\/vacuum route defines a statistically robust processing window for nanocrystal PeLEDs at a 28 mm2 active area.<\/jats:p>","DOI":"10.1021\/acsami.6c13884","type":"journal-article","created":{"date-parts":[[2026,9,19]],"date-time":"2026-09-19T23:01:33Z","timestamp":1789858893000},"page":"52932-52950","source":"Crossref","is-referenced-by-count":0,"title":["Interfacial Conditioning for High-Brightness 28 mm2 Active-Area Phenylpropylamine-Capped CsPbBr3 Perovskite Nanocrystal Light-Emitting Diodes Synthesized by a Modified Ligand-Assisted Reprecipitation Method"],"prefix":"10.1021","volume":"18","author":[{"given":"Ernest","family":"Ruby","sequence":"first","affiliation":[{"name":"LUMIN, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR 9024) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rafa","family":"Alamri","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rakan","family":"Alaneazi","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ga\u00eblle","family":"Tripp\u00e9-Allard","sequence":"additional","affiliation":[{"name":"LUMIN, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR 9024) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nicolas","family":"Guiblin","sequence":"additional","affiliation":[{"name":"(i) Laboratoire SPMS, Universit\u00e9 Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR8580); (ii) LMPS - Laboratoire de M\u00e9canique Paris-Saclay, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS, (UMR 9026) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jacqueline","family":"Tran","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Maxime","family":"Vallet","sequence":"additional","affiliation":[{"name":"(i) Laboratoire SPMS, Universit\u00e9 Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR8580); (ii) LMPS - Laboratoire de M\u00e9canique Paris-Saclay, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS, (UMR 9026) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kassiog\u00e9","family":"Demb\u00e9l\u00e9","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8413-0504","authenticated-orcid":true,"given":"Martin","family":"Foldyna","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Emmanuelle","family":"Deleporte","sequence":"additional","affiliation":[{"name":"LUMIN, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR 9024) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yvan","family":"Bonnassieux","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Denis","family":"Tondelier","sequence":"additional","affiliation":[{"name":"LPICM, CNRS, \u00c9cole Polytechnique, Institut Polytechnique de Paris , route de Saclay , ,","place":["Palaiseau, France, 91128"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2902-9240","authenticated-orcid":true,"given":"C\u00e9dric R","family":"Mayer","sequence":"additional","affiliation":[{"name":"LUMIN, Universit\u00e9 Paris-Saclay, ENS Paris-Saclay, CentraleSup\u00e9lec, CNRS (UMR 9024) , ,","place":["Gif-sur-Yvette, France, 91190"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,19]]},"reference":[{"key":"2026093002084083400_cit1","doi-asserted-by":"publisher","first-page":"7444","DOI":"10.1021\/acs.chemrev.9b00107","article-title":"Perovskites for Next-Generation Optical Sources","volume":"119","author":"Quan","year":"2019","journal-title":"Chem. 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