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In this work, robust thermodynamic stabilization was achieved by introducing methylammonium chloride (MACl) in PbS QD surface passivation, as validated by theoretical modeling and experimental characterization. MACl passivation reconstructed the surface energy landscape, establishing a physical barrier that suppressed PbS QD fusion and ligand re-adsorption, while extensive halide coordination minimized structural disorder and reduced sub-bandgap trap states. As a result, the optimized PbS QD photodiodes exhibited a peak external quantum efficiency of 56% and a specific detectivity of 1.12 \u00d7 1012 Jones at 1450 nm, an order-of-magnitude enhancement over control devices. This strategy enabled high-sensitivity SWIR imaging and established thermodynamic surface stabilization as a scalable avenue for advanced infrared optoelectronics.<\/jats:p>","DOI":"10.1021\/acsami.6c14167","type":"journal-article","created":{"date-parts":[[2026,9,22]],"date-time":"2026-09-22T16:01:45Z","timestamp":1790092905000},"page":"54241-54251","source":"Crossref","is-referenced-by-count":1,"title":["Thermodynamic Stabilization of PbS Quantum Dots for High-Performance Short-Wave Infrared Photodetection"],"prefix":"10.1021","volume":"18","author":[{"given":"Yiqun","family":"Li","sequence":"first","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, P. R. China, 230026"]},{"name":"Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences , , ,","place":["Guangzhou, P. R. 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