{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T10:50:44Z","timestamp":1791975044036,"version":"4.4.0"},"reference-count":54,"publisher":"American Chemical Society (ACS)","issue":"40","license":[{"start":{"date-parts":[[2026,9,28]],"date-time":"2026-09-28T00:00:00Z","timestamp":1790553600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,28]],"date-time":"2026-09-28T00:00:00Z","timestamp":1790553600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,28]],"date-time":"2026-09-28T00:00:00Z","timestamp":1790553600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"FAW R&D Projects","award":["20240301002ZD"],"award-info":[{"award-number":["20240301002ZD"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,14]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Silicon (Si) is a highly promising anode for next-generation all-solid-state batteries (ASSBs) owing to its exceptional theoretical capacity and low propensity for dendrite formation. However, severe volume fluctuations during (de)lithiation induce chemomechanical degradation and progressive loss of solid\u2013solid contact, drastically limiting long-term cycling stability. Here, we report a structurally engineered anode comprising a porous silicon core conformally encapsulated by a graphene-like hard-carbon (HC) layer (pSi@C) to resolve these interfacial bottlenecks. The predefined internal voids of the porous framework intrinsically buffer Si swelling, while the robust carbon shell mitigates macroscopic mechanical stress and establishes a highly efficient mixed ionic\u2013electronic transport network. Utilizing in situ three-electrode electrochemical impedance spectroscopy, we successfully decouple the interfacial kinetics, revealing significantly suppressed interfacial resistance during operation. Consequently, paired with an NCM811 cathode in a full-cell configuration, the pSi@C anode demonstrates robust cycling, delivering a capacity retention of 73.2% after 200 cycles at 0.5 C. This combined architectural design fundamentally addresses the chemomechanical failure of Si, offering a compelling pathway for the practical deployment of high-energy-density ASSBs.<\/jats:p>","DOI":"10.1021\/acsami.6c14371","type":"journal-article","created":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T03:02:07Z","timestamp":1790650927000},"page":"54872-54881","source":"Crossref","is-referenced-by-count":0,"title":["Mitigating Chemomechanical Degradation in All-Solid-State Batteries\n                    <i>via<\/i>\n                    Combined Porous Silicon and Hard-Carbon Architectures"],"prefix":"10.1021","volume":"18","author":[{"given":"Yangchen","family":"Wu","sequence":"first","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]},{"name":"Nanjing University of Aeronautics and Astronautics , , ,","place":["Shenzhen, China, 518000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinmin","family":"Luo","sequence":"additional","affiliation":[{"name":"China FAW Corporation Limited , ,","place":["Changchun, China, 130013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhijie","family":"Yang","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yiting","family":"Fang","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ximin","family":"Zhai","sequence":"additional","affiliation":[{"name":"China FAW Corporation Limited , ,","place":["Changchun, China, 130013"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Han","family":"Cui","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hao","family":"Dang","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0410-7000","authenticated-orcid":true,"given":"Bing","family":"Ding","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]},{"name":"Nanjing University of Aeronautics and Astronautics , , ,","place":["Shenzhen, China, 518000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4464-672X","authenticated-orcid":true,"given":"Xiaogang","family":"Zhang","sequence":"additional","affiliation":[{"name":"Nanjing University of Aeronautics and Astronautics , , No. 29 Yudao Street , ,","place":["Nanjing, China, 210016"]},{"name":"Nanjing University of Aeronautics and Astronautics , , ,","place":["Shenzhen, China, 518000"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,28]]},"reference":[{"issue":"3","key":"2026101406075145600_cit1","doi-asserted-by":"publisher","first-page":"230","DOI":"10.1038\/s41560-023-01208-9","article-title":"Challenges in Speeding Up Solid-State Battery Development","volume":"8","author":"Janek","year":"2023","journal-title":"Nat. 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