{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T19:45:46Z","timestamp":1792784746849,"version":"4.5.0"},"reference-count":54,"publisher":"American Chemical Society (ACS)","issue":"41","license":[{"start":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T00:00:00Z","timestamp":1791331200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T00:00:00Z","timestamp":1791331200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T00:00:00Z","timestamp":1791331200000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"Key Laboratory of Carbon Fibers and Functional Polymers, Beijing University of Chemical Technology","award":["202210250777003000"],"award-info":[{"award-number":["202210250777003000"]}],"id":[{"id":"https:\/\/ror.org\/00df5yc52","id-type":"ROR","asserted-by":"crossref"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,21]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Although transparent insulating aerogels are promising for energy-efficient glazing, their practical application remains limited by optical scattering, structural inhomogeneity, poor mechanical properties, and complex preparation processes. Herein, we report an octa(tetramethylammonium) polyhedral oligomeric silsesquioxane (OctaTMA-POSS)-regulated nucleation-growth strategy to fabricate mechanically robust transparent aerogels via ambient-pressure drying. Methyltriethoxysilane (MTES) was used as the precursor, and OctaTMA-POSS served as a multifunctional nanobuilding block whose intrinsic alkaline catalytic activity eliminated the need for additional acid or base catalysts. The rigid POSS cage acted as a seed-like nucleation center and was incorporated into the aerogel skeleton to regulate primary-particle growth and reinforce the framework. In situ monitoring of the gelation process revealed that this strategy effectively regulated primary-particle growth, yielding a fine, uniform nanoporous skeleton. The resulting aerogel exhibited a visible-light transmittance of up to 88.86%, a low thermal conductivity of 23.1 mW\u00b7m\u20131\u00b7K\u20131, a maximum deformation of 63.7% with a compressive strength of 12.12 MPa, and an initial decomposition temperature (Td5) of 520 \u00b0C. This work provides a simple and cost-effective route to high-performance transparent insulating aerogels for energy-efficient glazing and building-envelope applications.<\/jats:p>","DOI":"10.1021\/acsami.6c14717","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T23:01:39Z","timestamp":1791414099000},"page":"56634-56646","source":"Crossref","is-referenced-by-count":0,"title":["A Self-Catalyzed, Seed-Regulated Nucleation-Growth Strategy for Ambient-Pressure-Dried Transparent Aerogels Combining Mechanical Robustness and Thermal Insulation"],"prefix":"10.1021","volume":"18","author":[{"given":"Mengguo","family":"Li","sequence":"first","affiliation":[{"name":"Beijing University of Chemical Technology , , ,","place":["Beijing, China, 100029"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Meixue","family":"Liu","sequence":"additional","affiliation":[{"name":"Beijing University of Chemical Technology , , ,","place":["Beijing, China, 100029"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziping","family":"Zhou","sequence":"additional","affiliation":[{"name":"Aerospace Research Institute of Materials and Processing Technology, Science and Technology on Advanced Functional Composites Technology , ,","place":["Beijing, China, 100076"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianjun","family":"Shi","sequence":"additional","affiliation":[{"name":"Aerospace Research Institute of Materials and Processing Technology, Science and Technology on Advanced Functional Composites Technology , ,","place":["Beijing, China, 100076"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qifang","family":"Li","sequence":"additional","affiliation":[{"name":"Beijing University of Chemical Technology , , ,","place":["Beijing, China, 100029"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guangxin","family":"Chen","sequence":"additional","affiliation":[{"name":"Beijing University of Chemical Technology , , ,","place":["Beijing, China, 100029"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7485-1030","authenticated-orcid":true,"given":"Zheng","family":"Zhou","sequence":"additional","affiliation":[{"name":"Beijing University of Chemical Technology , , ,","place":["Beijing, China, 100029"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,7]]},"reference":[{"issue":"19","key":"2026102108072732100_cit1","doi-asserted-by":"publisher","DOI":"10.3390\/buildings15193478","article-title":"A Case Study on the Energy Efficiency of Windows in Institutional and Residential Buildings","volume":"15","author":"Qiu","year":"2025","journal-title":"Buildings"},{"issue":"1","key":"2026102108072732100_cit2","doi-asserted-by":"publisher","first-page":"71","DOI":"10.1016\/S0378-7788(01)00079-2","article-title":"Energy Performance of Windows in High-Rise Residential Buildings in Hong Kong","volume":"34","author":"Bojic","year":"2002","journal-title":"Energy Build."},{"key":"2026102108072732100_cit3","doi-asserted-by":"publisher","DOI":"10.1016\/j.enbuild.2025.115405","article-title":"Advancements in Energy-Active Window Systems: A Comprehensive Review","volume":"332","author":"Mahdi","year":"2025","journal-title":"Energy Build."},{"key":"2026102108072732100_cit4","doi-asserted-by":"publisher","DOI":"10.3389\/fenrg.2024.1463678","article-title":"The Effect of Window Proportions in Low-Rise Residential Buildings on Annual Energy Consumption in Humid Temperate Climate (Case Study: Rasht City in Iran)","volume":"12","author":"Bagheri","year":"2024","journal-title":"Front. 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