{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T12:54:05Z","timestamp":1791982445774,"version":"4.4.0"},"reference-count":51,"publisher":"American Chemical Society (ACS)","issue":"40","license":[{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T00:00:00Z","timestamp":1790640000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100002858","name":"China Postdoctoral Science Foundation","doi-asserted-by":"publisher","award":["GZC20233564"],"award-info":[{"award-number":["GZC20233564"]}],"id":[{"id":"10.13039\/501100002858","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,14]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Polyethylene oxide (PEO)-based composite solid polymer electrolytes (CPEs) are emerging materials for all-solid-state lithium batteries (ASSLBs). However, the low ionic conductivity and slow multiphase ion transport have stymied their development. To address these limitations, we report a class of multifunctional active fillers based on Keggin-type polyoxometalates (POMs), Li3[PM12O40] (M = Mo, W). Unlike conventional inert fillers, these molecularly precise metal\u2013oxygen clusters provide abundant Lewis basic surface sites, as well as intrinsic Li+ conduction pathways within their crystalline lattice. Comprehensive solid-state nuclear magnetic resonance, density functional theory calculations, and electrochemical analyses revealed that the [PMo12O40]3\u2013 cluster exhibited a weaker Li+ coordination affinity and a lower ion migration barrier than its tungsten analog. This resulted in a higher concentration of free Li+ alongside efficient interfacial and bulk transport channels. Notably, the PEO-based CPE with 10 wt % loading exhibited an ionic conductivity of 7.8 \u00d7 10\u20134 S\/cm at 60 \u00b0C, a high Li+ transference number of 0.80, and superior long-term stability over 1500 h in symmetric Li cells. A high capacity retention of 87% was achieved after 800 cycles at 1 C for ASSLBs assembled with LiFePO4 cathodes, which outperformed conventional PEO-based electrolytes. This study advances the fundamental understanding of multiphase ion migration in solid-state systems and establishes POM clusters as a versatile component of high-performance composite electrolytes.<\/jats:p>","DOI":"10.1021\/acsami.6c14818","type":"journal-article","created":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T21:01:58Z","timestamp":1790715718000},"page":"55479-55489","source":"Crossref","is-referenced-by-count":0,"title":["Regulation of Multiphase Ion Migration in Polyoxometalate-Based Composite Solid-State Electrolytes"],"prefix":"10.1021","volume":"18","author":[{"given":"Sheng","family":"Chen","sequence":"first","affiliation":[{"name":"Zhijian Laboratory, Rocket Force University of Engineering , ,","place":["Xi'an, P. R. China, 710025"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xinyang","family":"Li","sequence":"additional","affiliation":[{"name":"Xi'an Jiaotong University , , ,","place":["Xi'an, P. R. 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