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Herein, we develop a dendritic functionalization strategy at the para-position of boron in the classical MR-TADF emitter BCz-BN by tuning the electron-withdrawing characteristics of peripheral dendrons, affording two solution-processable emitters, CN-BN and Ph-BN. The cyano-containing CN-BN exhibits accelerated reverse intersystem crossing but broadened emission due to the presence of strong charge-transfer character. By removing the cyano group, Ph-BN preserves the intrinsic MR character with reduced excited-state relaxation. Combined with the steric protection of the dendritic units, Ph-BN achieves a narrow full width at half maximum (fwhm) of 28 nm and a high EQEmax of 24.9% in solution-processed OLEDs. Notably, the fwhm of Ph-BN increases by only 5 nm from photoluminescence to electroluminescence, whereas BCz-BN exhibits a much larger increase of 16 nm.<\/jats:p>","DOI":"10.1021\/acsami.6c15651","type":"journal-article","created":{"date-parts":[[2026,9,25]],"date-time":"2026-09-25T13:02:36Z","timestamp":1790341356000},"page":"53740-53748","source":"Crossref","is-referenced-by-count":0,"title":["<i>para<\/i>\n                    -Boron Dendritic Modulation of MR-TADF Emitters Enables High-Efficiency Narrowband Solution-Processed OLEDs"],"prefix":"10.1021","volume":"18","author":[{"given":"Tao","family":"Zhou","sequence":"first","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, P. R. China, 211189"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guimin","family":"Zhao","sequence":"additional","affiliation":[{"name":"Southeast University , , ,","place":["Nanjing, P. R. 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