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Herein, multicomponent dynamic covalent photoresponsive elastomers are fabricated through Diels\u2013Alder (D-A) chemistry, utilizing furan-functionalized SBS (SBS-Fu) cross-linked with maleimide-modified tetraphenylethylene (TPEDMI) and\/or cellulose-based maleimide (ECMI). Synergistic optimization of composition and structure endows SBS-10Fu\/TPEDMI10% with optimal mechanical properties, featuring an elongation of 820%, a tensile strength of 27.6 MPa, and a toughness of 83.1 MJ\/m3. By integrating the aggregation-induced emission (AIE) of TPE, the photoinduced electron transfer (PET) effect of TPEDMI, and the thermoreversibility of D-A adducts, the resulting materials exhibit temperature\/photoresponsive fluorescence modulation. The obtained over 99% UV-shielding efficiency can suppress the undesirable TPE photocyclization, thereby enabling information writing and erasing. When combined with favorable shape memory (Rf = 99.4%, Rr = 99.7%), a dual-mode encryption platform is further achieved. This study presents a comprehensive design framework for multifunctional elastomers targeting information encryption and smart systems.<\/jats:p>","DOI":"10.1021\/acsami.6c15911","type":"journal-article","created":{"date-parts":[[2026,9,30]],"date-time":"2026-09-30T10:02:17Z","timestamp":1790762537000},"page":"55510-55524","source":"Crossref","is-referenced-by-count":0,"title":["Mechanically Tunable, Ultraviolet-Shielding, and Recyclable Smart Elastomers for Information Encryption via Fluorescence Switching and Shape Memory"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0009-0009-3460-6231","authenticated-orcid":true,"given":"Xuwen","family":"Li","sequence":"first","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-8187-3678","authenticated-orcid":true,"given":"Ting","family":"Liu","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yinglin","family":"Chen","sequence":"additional","affiliation":[{"name":"Guangdong Sunion Advanced Novel Technology Co., Ltd. , , ,","place":["Maoming, Guangdong Province, China, 525000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiaxin","family":"Yang","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3897-9907","authenticated-orcid":true,"given":"Hongwei","family":"Ma","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanshai","family":"Wang","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hai-tao","family":"Zhang","sequence":"additional","affiliation":[{"name":"Guangdong Sunion Advanced Novel Technology Co., Ltd. , , ,","place":["Maoming, Guangdong Province, China, 525000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Li","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9304-551X","authenticated-orcid":true,"given":"Li","family":"Han","sequence":"additional","affiliation":[{"name":"Dalian University of Technology , , ,","place":["Dalian, China, 116024"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,30]]},"reference":[{"issue":"6","key":"2026101408080135200_cit1","doi-asserted-by":"publisher","first-page":"834","DOI":"10.1038\/s41563-024-01845-9","article-title":"Phase patterning of liquid crystal elastomers by laser-induced dynamic crosslinking","volume":"23","author":"Choi","year":"2024","journal-title":"Nat. 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