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Herein, a multifunctional protective coating, constructed by incorporating vermiculite nanosheets (VN) into a carboxymethyl cellulose (CMC) matrix, was developed to mitigate these challenges. The VN-CMC composite coating exhibits a lamellar structure containing abundant polar groups such as hydroxyl (\u2013OH) and carboxymethyl (\u2013CH2COOH). The desolvation process of Zn2+ is expedited by these polar functional groups, which further direct the homogeneous plating of zinc onto the (002) crystal facet. Moreover, the lamellar architecture contributes to a homogeneous electric field distribution and modulates Zn2+ flux, thereby inhibiting dendrite nucleation and propagation. Consequently, the VN-CMC@Zn anode delivers exceptional long-term stability, sustaining up to 7100 h (at 0.5 mA cm\u20132, 1 mAh cm\u20132) and 3000 h (at 5 mA cm\u20132, 5 mAh cm\u20132). When assembled into a full battery with NaV3O8\u00b71.5H2O (NVO) as the cathode, the composite-protected anode delivers remarkable cycling durability, retaining 90% of its initial capacity after 2000 cycles at 2 A g\u20131. This study offers a promising strategy for the rational engineering of highly reversible Zn metal anodes.<\/jats:p>","DOI":"10.1021\/acsami.6c16237","type":"journal-article","created":{"date-parts":[[2026,10,6]],"date-time":"2026-10-06T03:02:05Z","timestamp":1791255725000},"page":"54979-54990","source":"Crossref","is-referenced-by-count":0,"title":["A Multifunctional Composite Interface Layer toward High-Performance Stable Zn Anode"],"prefix":"10.1021","volume":"18","author":[{"given":"Xuehua","family":"Zhou","sequence":"first","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jia","family":"Wang","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0001-1005-7479","authenticated-orcid":true,"given":"Yan","family":"Zhang","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]},{"name":"Hainan University , , ,","place":["Haikou, China, 570228"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingjing","family":"Wang","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xueer","family":"Wu","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chao","family":"Zhang","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shengjue","family":"Deng","sequence":"additional","affiliation":[{"name":"Anqing Normal University , , ,","place":["Anqing, China, 246011"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bo","family":"Liu","sequence":"additional","affiliation":[{"name":"Stanford University , , ,","place":["Stanford, United States, 94305"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,5]]},"reference":[{"issue":"2","key":"2026101406065640500_cit1","doi-asserted-by":"publisher","DOI":"10.1002\/eem2.70151","article-title":"Hygroscopic Organic Complex Mutated Helmholtz Plane of Zn Anode for Outstanding Zinc Ion Battery","volume":"9","author":"Elshahawy","year":"2026","journal-title":"Energy Environ. 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