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Here, we report TBT\u2013ThT\u2013O, a donor\u2013acceptor small molecule in which a strong D\u2013\u03c0\u2013A\u2013\u03c0\u2013D framework, \u03c0-bridge extension, and radical character act cooperatively to enhance intramolecular charge transfer and suppress radiative decay, thereby favoring nonradiative heat dissipation under sunlight. TBT\u2013ThT\u2013O exhibits broadened solar absorption extended to 2000 nm and excellent photothermal stability. When immobilized in porous polyurethane foam to construct an interfacial evaporator, TBT\u2013ThT\u2013O@PU achieves a high evaporation rate of 1.356 kg m\u20132 h\u20131 and a solar-to-vapor efficiency of 93.05% under 1 sun. As a photothermal coating coupled with a thermoelectric module, the system delivers a voltage of 245 mV and an output power density of 3.936 W m\u20132 under 1 sun. Furthermore, a lens-assisted hybrid platform is demonstrated to intensify outdoor solar flux for simultaneous freshwater production and electricity generation. This work demonstrates that D\u2013A radicaloid molecular engineering provides a viable route to stable, high-performance organic photothermal materials for integrated solar desalination and power generation.<\/jats:p>","DOI":"10.1021\/acsami.6c16869","type":"journal-article","created":{"date-parts":[[2026,10,13]],"date-time":"2026-10-13T19:01:59Z","timestamp":1791918119000},"source":"Crossref","is-referenced-by-count":0,"title":["Donor-Acceptor Radicaloid Materials with Enhanced Nonradiative Decay Enable Efficient Solar-Thermal Conversion"],"prefix":"10.1021","author":[{"given":"Shibo","family":"Cheng","sequence":"first","affiliation":[{"name":"The Chinese University of Hong Kong (Shenzhen), Longgang , , , ,","place":["Shenzhen, Guangdong, China, 518172"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yucheng","family":"Wang","sequence":"additional","affiliation":[{"name":"The Chinese University of Hong Kong (Shenzhen), Longgang , , , ,","place":["Shenzhen, Guangdong, China, 518172"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huilin","family":"Xie","sequence":"additional","affiliation":[{"name":"Nankai International Advanced Research Institute (Shenzhen Futian), Nankai University , ,","place":["Shenzhen, P.R. China, 518045"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4528-9824","authenticated-orcid":true,"given":"Jianquan","family":"Zhang","sequence":"additional","affiliation":[{"name":"The Chinese University of Hong Kong (Shenzhen), Longgang , , , ,","place":["Shenzhen, Guangdong, China, 518172"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0293-964X","authenticated-orcid":true,"given":"Ben Zhong","family":"Tang","sequence":"additional","affiliation":[{"name":"The Chinese University of Hong Kong (Shenzhen), Longgang , , , ,","place":["Shenzhen, Guangdong, China, 518172"]},{"name":"The Hong Kong University of Science and Technology , , , ,","place":["Kowloon, Hong Kong, China, 999077"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,13]]},"reference":[{"issue":"1","key":"2026101315015191800_cit1","doi-asserted-by":"publisher","first-page":"16","DOI":"10.1038\/nmat4834","article-title":"The path towards sustainable energy","volume":"16","author":"Chu","year":"2017","journal-title":"Nat. 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