{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T08:46:00Z","timestamp":1792053960423,"version":"4.4.0"},"reference-count":53,"publisher":"American Chemical Society (ACS)","license":[{"start":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T00:00:00Z","timestamp":1792022400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T00:00:00Z","timestamp":1792022400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T00:00:00Z","timestamp":1792022400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100010256","name":"Guangzhou Municipal Science and Technology Project","doi-asserted-by":"publisher","award":["201804020005"],"award-info":[{"award-number":["201804020005"]}],"id":[{"id":"10.13039\/501100010256","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>All-inorganic CsPbI3\u2013xBrx perovskites have emerged as promising photovoltaic materials owing to their excellent thermal stability and tunable bandgap. However, solution-processed CsPbI3\u2013xBrx films continue to suffer from sluggish crystallization kinetics and poor phase stability, which severely limit device performance. Herein, we introduce 6-(trifluoromethyl)\u20132(3H)-benzothiazolethione (TFMBT) as a multifunctional additive to regulate nucleation and phase transformation. The N\u2013H and C=S groups of TFMBT synergistically weaken the DMSO-[PbI6]4\u2013 coordination via hydrogen bonding and Lewis acid\u2013base interactions, facilitating solvent removal and lowering the nucleation barrier. Meanwhile, the CF3 group engages the N\u2013H group of DMA+ in N\u2013H\u00b7\u00b7\u00b7F contacts, accelerating DMA+ deintercalation and Cs+ incorporation to expedite phase transformation. This synergistic effect cooperatively accelerates the crystallization kinetics, yielding high-quality films with enlarged, uniform grains and suppressed defects. Benefiting from the optimized crystallization regulation and improved film quality, the TFMBT-modified carbon-based CsPbI3\u2013xBrx perovskite solar cells achieve a champion power conversion efficiency of 15.34%, significantly outperforming the control devices (12.75%), along with excellent stability.<\/jats:p>","DOI":"10.1021\/acsami.6c17062","type":"journal-article","created":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T01:01:38Z","timestamp":1792026098000},"source":"Crossref","is-referenced-by-count":0,"title":["Bifunctional Modulation of Nucleation and Phase Transformation by TFMBT for Efficient Carbon-Based CsPbI3\u2013\n                    <i>x<\/i>\n                    Br\n                    <i>x<\/i>\n                    Perovskite Solar Cells"],"prefix":"10.1021","author":[{"given":"Guangli","family":"Liu","sequence":"first","affiliation":[{"name":"Guangdong University of Technology , , No. 100 Waihuan Xi Road, Higher Education Mega Center , ,","place":["Guangzhou, P. 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