{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,11,5]],"date-time":"2026-11-05T09:28:54Z","timestamp":1793870934725,"version":"4.6.1"},"reference-count":71,"publisher":"American Chemical Society (ACS)","issue":"43","license":[{"start":{"date-parts":[[2026,10,22]],"date-time":"2026-10-22T00:00:00Z","timestamp":1792627200000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"name":"German Research Council (DFG)","award":["450218497"],"award-info":[{"award-number":["450218497"]}]},{"name":"German Research Council (DFG)","award":["459278559"],"award-info":[{"award-number":["459278559"]}]},{"name":"German Research Council (DFG)","award":["544048794"],"award-info":[{"award-number":["544048794"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,11,4]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Multizone synthesis and localized deposition of bimetallic nanoarchitectures remain major challenges in additive manufacturing at the nanoscale, particularly when control over nanoarchitecture and localized functionality is required. Here, a multizone gas-phase electrodeposition strategy for the simultaneous synthesis and localized deposition of Pt\/In core\u2212shell nanoparticles through coupled vapor-phase encapsulation and electrostatic confinement is reported. In contrast to previous gas-phase electrodeposition studies that primarily focused on metallic and metal-oxide nano- and microarchitectures, the present work extends the process to bimetallic core\u2212shell nanoarchitectures as functional nanoscale building blocks. Spark-generated Pt nanoparticles interact in flight with transported In vapor, enabling ligand-free Pt\/In encapsulation before deposition. By controlling the In vapor supply through the evaporation temperature, two distinct nanoarchitectures are obtained: centric Pt-core\/In-shell nanoparticles (evaporation temperature 750 \u00b0C) and eccentric core\u2212shell nanoparticles (evaporation temperature 900 \u00b0C) with asymmetric shell distribution. In-flight particle collection reveals that the asymmetry initiates during high-temperature formation and becomes more pronounced during cooling after deposition. The charged Pt\/In core\u2212shell nanoparticles are selectively deposited into predefined Si micro-openings and linear patterns. The eccentric Pt\/In structures exhibit broadened visible-light absorption and generate a measurable photo-thermoelectric response under illumination at 532 nm. The polarity reversal strongly supports the thermoelectric origin of the response. This approach establishes gas-phase electrodeposition as a route toward localized bimetallic core\u2212shell nanoarchitectures for optothermal and thermoelectric applications.<\/jats:p>","DOI":"10.1021\/acsami.6c17121","type":"journal-article","created":{"date-parts":[[2026,10,22]],"date-time":"2026-10-22T18:01:42Z","timestamp":1792692102000},"page":"59780-59793","source":"Crossref","is-referenced-by-count":0,"title":["Gas Phase Multizone Synthesis and Localized Deposition of Pt\/In Core\u2212Shell Nanoparticles and Their Photothermoelectric Application"],"prefix":"10.1021","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3587-8596","authenticated-orcid":true,"given":"Soumya","family":"Biswas","sequence":"first","affiliation":[{"name":"Institut f\u00fcr Mikro- und Nanoelektronik, Technische Universit\u00e4t Ilmenau , , Gustav-Kirchhoff-Str. 1 , , ,","place":["Ilmenau, Thuringia, Germany, 98693"]},{"name":"Technische Universit\u00e4t Ilmenau , , Gustav-Kirchhoff-Str. 7 , 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