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Herein, we display 5.6 atom % Ag\/Cu2O\u2013Cu catalyst with abundant and steady Ag\/Cu+\/Cu0 interfaces for the efficient conversion of CO2-to-C2+ at ampere level current density. 5.6 atom % Ag\/Cu2O\u2013Cu catalyst attains a desirable FE of 76.5 \u00b1 1.2% toward C2+ products at 1.0 A\/cm2 in 1 M KOH electrolyte and remains stable CO2 electrolysis at 0.50 A\/cm2 for 20 h using a flow cell apparatus. In situ Raman spectrometry and density functional theory calculations indicate that a steady Ag\/Cu+\/Cu0 interface can promote CO2-to-C2+ conversion through adjusting the energy barrier for the formation and dimerization of *CO intermediates. The synergistically heterogeneous interfaces promote the activity, selectivity, and stability of CO2 electroreduction to C2+ products via a tandem route of *COOH, *CO, and *OCCO intermediates over Ag\/Cu+\/Cu0 cooperative sites.<\/jats:p>","DOI":"10.1021\/acsnano.4c18967","type":"journal-article","created":{"date-parts":[[2025,3,13]],"date-time":"2025-03-13T10:19:12Z","timestamp":1741861152000},"page":"11263-11272","source":"Crossref","is-referenced-by-count":109,"title":["Ag Stabilized Cu+\/Cu0 Interface\nCatalysts for Enhanced CO2 Electroreduction to C2+ Products at Ampere Level Current Density"],"prefix":"10.1021","volume":"19","author":[{"given":"Yiyuan","family":"Jiang","sequence":"first","affiliation":[{"name":"Harbin Engineering University , , ,","place":["Harbin, China, 150001"]},{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0001-2691-4826","authenticated-orcid":true,"given":"Chunmei","family":"Lv","sequence":"additional","affiliation":[{"name":"Harbin Engineering University , , ,","place":["Harbin, China, 150001"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Borong","family":"Lu","sequence":"additional","affiliation":[{"name":"Harbin Engineering University , , ,","place":["Harbin, China, 150001"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanpeng","family":"Song","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tianfu","family":"Liu","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaomin","family":"Zhang","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2472-7349","authenticated-orcid":true,"given":"Dunfeng","family":"Gao","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ke","family":"Ye","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Qingdao, China, 266101"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6042-1171","authenticated-orcid":true,"given":"Guoxiong","family":"Wang","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Dalian, China, 116023"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2025,3,13]]},"reference":[{"key":"2026081813195088200_cit1","doi-asserted-by":"publisher","first-page":"262","DOI":"10.1038\/s41586-022-05540-0","article-title":"Operando Studies Reveal Active Cu Nanograins for CO2 Electroreduction","volume":"614","author":"Yang","year":"2023","journal-title":"Nature"},{"key":"2026081813195088200_cit2","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.124525","article-title":"Preparation of Phosphorus-Doped\nCu-Based Catalysts by Electrodeposition Modulates *CHxO\nAdsorption to Facilitate Electrocatalytic Reduction of CO2 to CH4","volume":"360","author":"Li","year":"2025","journal-title":"Appl. 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