{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T18:17:56Z","timestamp":1790014676384,"version":"4.0.1"},"reference-count":54,"publisher":"American Chemical Society (ACS)","issue":"29","license":[{"start":{"date-parts":[[2026,7,12]],"date-time":"2026-07-12T00:00:00Z","timestamp":1783814400000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100024870","name":"Exacte en Natuurwetenschappen","doi-asserted-by":"publisher","award":["VI.Vidi.203.027"],"award-info":[{"award-number":["VI.Vidi.203.027"]}],"id":[{"id":"10.13039\/501100024870","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100000781","name":"European Research Council","doi-asserted-by":"publisher","award":["101116984"],"award-info":[{"award-number":["101116984"]}],"id":[{"id":"10.13039\/501100000781","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003246","name":"Nederlandse Organisatie voor Wetenschappelijk Onderzoek","doi-asserted-by":"publisher","award":["19486"],"award-info":[{"award-number":["19486"]}],"id":[{"id":"10.13039\/501100003246","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,7,28]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>2D materials and their monolayers have attracted widespread interest by virtue of their unique electronic and optical properties. In addition to their remarkable physical characteristics, their atomically thin nature enables integration in ultracompact photonic and electronic devices, with potential for dynamic tunability via strain, charge carrier modulation or heterostructure engineering. While early research relied on micrometer-scale mechanically exfoliated flakes, recent advances\u2500particularly gold-assisted exfoliation of transition metal dichalcogenides (TMDCs)\u2500have enabled the preparation of high-quality, large-area monolayers, facilitating scalable device integration. For the field of nanophotonics in particular, the ability to transfer large-area 2D materials onto both flat and patterned substrates is essential for the development of functional devices. However, existing transfer techniques are often limited in scalability, compatibility with structured surfaces, or preservation of material quality. Here, we present a versatile and reliable transfer method of large-area monolayers and hBN\/monolayer heterostructures onto both flat and nanostructured substrates. Our approach, based on the physical properties of low-density polyethylene, enhances excitonic emission of TMDCs and is compatible with a variety of device architectures. We demonstrate its applicability by fabricating devices that modulate the photoluminescence of TMDC monolayers through the manipulation of the photonic environment, strain or electrical gating. We further demonstrate the fabrication of van der Waals heterostructures using the same method. By enabling clean transfer of a wide range of monolayers and heterostructures, this technique offers a practical pathway for the development of next-generation optoelectronic platforms with improved functionality, scalability, and tunability.<\/jats:p>","DOI":"10.1021\/acsnano.6c04231","type":"journal-article","created":{"date-parts":[[2026,7,12]],"date-time":"2026-07-12T13:05:17Z","timestamp":1783861517000},"page":"20611-20622","source":"Crossref","is-referenced-by-count":1,"title":["Large-Area Deterministic\nStamping of 2D Materials\non Patterned Surfaces"],"prefix":"10.1021","volume":"20","author":[{"given":"Bernardo S.","family":"Dias","sequence":"first","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8378-1230","authenticated-orcid":true,"given":"Reynolds","family":"Dziobek-Garrett","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]},{"name":"Advanced Research Center for Nanolithography , Science Park 106 , ,","place":["Amsterdam, The Netherlands, 1098 XG"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gabriella","family":"Mentasti","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Abhishek","family":"Gupta","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Alexander","family":"Lambertz","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]},{"name":"AMOLF , , ,","place":["Amsterdam, The Netherlands, 1098 XG"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7317-9863","authenticated-orcid":true,"given":"Esther","family":"Alarco\u0301n-Llado\u0301","sequence":"additional","affiliation":[{"name":"AMOLF , , ,","place":["Amsterdam, The Netherlands, 1098 XG"]},{"name":"Universiteit van Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2612-2762","authenticated-orcid":true,"given":"Peter","family":"Schall","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Roland","family":"Bliem","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]},{"name":"Advanced Research Center for Nanolithography , Science Park 106 , ,","place":["Amsterdam, The Netherlands, 1098 XG"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3033-8005","authenticated-orcid":true,"given":"Jorik","family":"van de Groep","sequence":"additional","affiliation":[{"name":"University of Amsterdam , , ,","place":["Amsterdam, The Netherlands, 1098 XH"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,12]]},"reference":[{"key":"2026072810084986500_cit1","doi-asserted-by":"publisher","first-page":"895","DOI":"10.1038\/s41565-024-01695-1","article-title":"The Future of Two-Dimensional Semiconductors\nBeyond Moore\u2019s Law","volume":"19","author":"Kim","year":"2024","journal-title":"Nat. Nanotechnol."},{"key":"2026072810084986500_cit2","doi-asserted-by":"publisher","first-page":"3961","DOI":"10.1021\/acsphotonics.5c00353","article-title":"Roadmap for Photonics with 2D Materials","volume":"12","author":"de Abajo","year":"2025","journal-title":"ACS Photonics"},{"key":"2026072810084986500_cit3","doi-asserted-by":"publisher","first-page":"9452","DOI":"10.1021\/acsnano.4c14168","article-title":"Spintronic Devices\nUpon 2D Magnetic Materials and Heterojunctions","volume":"19","author":"Jia","year":"2025","journal-title":"ACS Nano"},{"key":"2026072810084986500_cit4","doi-asserted-by":"publisher","first-page":"042002","DOI":"10.1088\/2053-1583\/aacfc1","article-title":"The Computational\n2D Materials Database: High-Throughput Modeling and Discovery of Atomically\nThin Crystals","volume":"5","author":"Haastrup","year":"2018","journal-title":"2D Mater."},{"key":"2026072810084986500_cit5","doi-asserted-by":"publisher","first-page":"14203","DOI":"10.1021\/acsomega.0c01676","article-title":"Recent Advances in the Carrier Mobility\nof Two-Dimensional Materials: A Theoretical Perspective","volume":"5","author":"Mir","year":"2020","journal-title":"ACS Omega"},{"key":"2026072810084986500_cit6","doi-asserted-by":"publisher","first-page":"29","DOI":"10.1038\/s41699-020-00162-4","article-title":"Bandgap\nEngineering of Two-Dimensional Semiconductor Materials","volume":"4","author":"Chaves","year":"2020","journal-title":"npj 2D Mater. 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Interfaces"},{"key":"2026072810084986500_cit8","doi-asserted-by":"publisher","first-page":"10134","DOI":"10.1007\/s12274-024-6936-3","article-title":"Progress and Prospects\nof Moire\u0301 Superlattices in Twisted TMD Heterostructures","volume":"17","author":"Shah","year":"2024","journal-title":"Nano Res."},{"key":"2026072810084986500_cit9","doi-asserted-by":"publisher","first-page":"022501","DOI":"10.1088\/2515-7639\/ad2083","article-title":"Roadmap\non 2D Topological Insulators","volume":"7","author":"Weber","year":"2024","journal-title":"JPhys Mater."},{"key":"2026072810084986500_cit10","doi-asserted-by":"publisher","first-page":"2529","DOI":"10.1021\/acsphotonics.3c01839","article-title":"Modulation and Optoelectronic\nApplications\nof van der Waals Interlayer Excitons","volume":"11","author":"Zhao","year":"2024","journal-title":"ACS Photonics"},{"key":"2026072810084986500_cit11","doi-asserted-by":"publisher","first-page":"5575","DOI":"10.1038\/srep05575","article-title":"Photoluminescence\nQuenching in Gold\u2013MoS2 Hybrid Nanoflakes","volume":"4","author":"Bhanu","year":"2014","journal-title":"Sci. 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Mater."},{"key":"2026072810084986500_cit30","doi-asserted-by":"publisher","first-page":"022004","DOI":"10.1088\/2053-1583\/ad2f43","article-title":"A Review on Transfer Methods of Two-Dimensional Materials","volume":"11","author":"Cheliotis","year":"2024","journal-title":"2D Mater."},{"key":"2026072810084986500_cit31","doi-asserted-by":"publisher","first-page":"701","DOI":"10.1007\/s00397-022-01360-1","article-title":"Characterization of Industrial Low-Density\nPolyethylene: a Thermal, Dynamic Mechanical, and Rheological Investigation","volume":"61","author":"Poh","year":"2022","journal-title":"Rheol. Acta"},{"key":"2026072810084986500_cit32","doi-asserted-by":"publisher","first-page":"97","DOI":"10.1080\/01694243.2013.847045","article-title":"Optimization\nof Atmospheric Plasma\nTreatment of LDPE Films: Influence on Adhesive Properties and Ageing\nBehavior","volume":"28","author":"Fombuena","year":"2014","journal-title":"J. Adhes. Sci. Technol."},{"key":"2026072810084986500_cit33","doi-asserted-by":"publisher","first-page":"44","DOI":"10.1038\/s41699-022-00323-7","article-title":"Evaluation of Polyvinyl\nChloride Adhesion to 2D Crystal Flakes","volume":"6","author":"Wakafuji","year":"2022","journal-title":"npj\n2D Mater. Appl."},{"key":"2026072810084986500_cit34","doi-asserted-by":"publisher","first-page":"152","DOI":"10.1038\/s42005-023-01268-z","article-title":"Probing Surface\nWetting Across Multiple Force, Length and Time Scales","volume":"6","author":"Daniel","year":"2023","journal-title":"Commun. Phys."},{"key":"2026072810084986500_cit35","doi-asserted-by":"publisher","first-page":"2419184","DOI":"10.1002\/adma.202419184","article-title":"Strain-Induced Decoupling Drives\nGold-Assisted Exfoliation of Large-Area\nMonolayer 2D Crystals","volume":"37","author":"Ziewer","year":"2025","journal-title":"Adv. Mater."},{"key":"2026072810084986500_cit36","doi-asserted-by":"publisher","first-page":"6299","DOI":"10.1021\/acs.nanolett.9b02431","article-title":"Enhancing Photoluminescence\nand Mobilities in WS2 Monolayers with Oleic Acid Ligands","volume":"19","author":"Tanoh","year":"2019","journal-title":"Nano Lett."},{"key":"2026072810084986500_cit37","doi-asserted-by":"publisher","first-page":"576","DOI":"10.1021\/acsnanoscienceau.5c00091","article-title":"Mechanism\nof Oleic Acid-Mediated\nSulfur Vacancy Healing in Monolayer WS2","volume":"5","author":"Daniel","year":"2025","journal-title":"ACS Nanosci. 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A."},{"key":"2026072810084986500_cit41","doi-asserted-by":"publisher","first-page":"110801","DOI":"10.1063\/1.5124302","article-title":"Engineered\nHyperuniformity for Directional\nLight Extraction","volume":"4","author":"Gorsky","year":"2019","journal-title":"APL Photonics"},{"key":"2026072810084986500_cit42","doi-asserted-by":"publisher","first-page":"9694","DOI":"10.1021\/acsnano.2c12759","article-title":"Recent Advances in 2D Material Theory, Synthesis, Properties, and\nApplications","volume":"17","author":"Lin","year":"2023","journal-title":"ACS Nano"},{"key":"2026072810084986500_cit43","doi-asserted-by":"publisher","first-page":"1837","DOI":"10.1038\/s41467-023-37500-1","article-title":"Macroscopic Transition Metal Dichalcogenides Monolayers With Uniformly\nHigh Optical Quality","volume":"14","author":"Li","year":"2023","journal-title":"Nat. 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Mater."},{"key":"2026072810084986500_cit47","doi-asserted-by":"publisher","first-page":"2","DOI":"10.1007\/s44214-025-00075-7","article-title":"Distinct Moire\u0301\nExciton Dynamics in WS2\/WSe2 Heterostructure","volume":"4","author":"Kai","year":"2025","journal-title":"Quantum Front."},{"key":"2026072810084986500_cit48","doi-asserted-by":"publisher","first-page":"4731","DOI":"10.1021\/acsnano.4c15459","article-title":"Electrical\nControl of Photoluminescence in 2D Semiconductors Coupled to Plasmonic\nLattices","volume":"19","author":"Moilanen","year":"2025","journal-title":"ACS Nano"},{"key":"2026072810084986500_cit49","doi-asserted-by":"publisher","first-page":"15030","DOI":"10.1038\/s41598-019-51490-5","article-title":"The Effect\nof Surface Roughness on the Contact Line and Splashing Dynamics of\nImpacting Droplets","volume":"9","author":"Quetzeri-Santiago","year":"2019","journal-title":"Sci. Rep."},{"key":"2026072810084986500_cit50","doi-asserted-by":"publisher","first-page":"14841","DOI":"10.1021\/acsnano.4c00590","article-title":"Transfer of 2D Films:\nFrom Imperfection\nto Perfection","volume":"18","author":"Pham","year":"2024","journal-title":"ACS Nano"},{"key":"2026072810084986500_cit51","doi-asserted-by":"publisher","first-page":"143536","DOI":"10.1016\/j.scitotenv.2020.143536","article-title":"Plastic Biodegradation:\nFrontline Microbes and Their Enzymes","volume":"759","author":"Amobonye","year":"2021","journal-title":"Sci. Total\nEnviron."},{"key":"2026072810084986500_cit52","doi-asserted-by":"publisher","first-page":"2574","DOI":"10.1039\/D5CS00531K","article-title":"Transfer\nand Beyond: Emerging Strategies and Trends in Two-Dimensional Material\nDevice Fabrication","volume":"55","author":"Huang","year":"2026","journal-title":"Chem. Soc. Rev."},{"key":"2026072810084986500_cit53","doi-asserted-by":"publisher","first-page":"11731","DOI":"10.1021\/acsomega.1c06855","article-title":"Large-Area Transfer\nof 2D TMDCs Assisted by a Water-Soluble Layer for Potential Device\nApplications","volume":"7","author":"Sharma","year":"2022","journal-title":"ACS Omega"},{"key":"2026072810084986500_cit54","doi-asserted-by":"publisher","DOI":"10.1002\/smtd.202501693","article-title":"Large-Area\nPhotonic Membranes Achieving Uniform and Strong Enhancement of Photoluminescence\nand Second-Harmonic Generation in Monolayer WSe2","volume":"10","author":"Hsieh","year":"2026","journal-title":"Small Methods"}],"container-title":["ACS Nano"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acsnano.6c04231","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/ancac3\/article-pdf\/20\/29\/20611\/65884482\/acsnano.6c04231.pdf","content-type":"application\/pdf","content-version":"vor","intended-application":"syndication"},{"URL":"https:\/\/pubs.acs.org\/ancac3\/article-pdf\/20\/29\/20611\/65884482\/acsnano.6c04231.pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,7,28]],"date-time":"2026-07-28T14:40:04Z","timestamp":1785249604000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/ancac3\/article\/20\/29\/20611\/5207017\/Large-Area-Deterministic-Stamping-of-2D-Materials"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,7,12]]},"references-count":54,"journal-issue":{"issue":"29","published-online":{"date-parts":[[2026,7,12]]},"published-print":{"date-parts":[[2026,7,28]]}},"URL":"https:\/\/doi.org\/10.1021\/acsnano.6c04231","relation":{},"ISSN":["1936-0851","1936-086X"],"issn-type":[{"value":"1936-0851","type":"print"},{"value":"1936-086X","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,7,12]]}}}