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Here, we report magnetic field-induced rotational symmetry distortion of the in-plane anisotropic magnetoresistance (AMR) in kagome semimetal Ni3In2Se2 nanoflakes synthesized via an iterative chemical vapor transport approach. High-quality Ni3In2Se2 nanoflakes possess a canted ferromagnetic order, along with a large magnetoresistance of 590%, an out-of-plane AMR of 200%, and a carrier mobility up to 8761 cm2 V\u20131 s\u20131. Furthermore, a large in-plane AMR of 41% and the planar Hall effect (PHE) are detected in Ni3In2Se2, with PHE stemming from the complex interaction of field-induced ferromagnetism and orbital magnetoresistance. Notably, the in-plane AMR exhibits a field-induced rotational symmetry distortion, characterized by the coexistence of the two-, four-, and six-fold AMR components. Band structure calculations suggest that the low-temperature distortions in the AMR of Ni3In2Se2 may arise from field-induced orbital polarization and field-enhanced Fermi surface anisotropy. Our findings contribute to understanding exotic transport behaviors in kagome semimetals and advancing low-power electronic devices and future spintronic applications.<\/jats:p>","DOI":"10.1021\/acsnano.6c06737","type":"journal-article","created":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T10:59:46Z","timestamp":1784545186000},"page":"21316-21326","source":"Crossref","is-referenced-by-count":0,"title":["Field-Induced Rotational\nSymmetry Distortion of In-Plane\nAnisotropic Magnetoresistance in Kagome Semimetal Ni3In2Se2 Nanoflakes"],"prefix":"10.1021","volume":"20","author":[{"given":"Senhao","family":"Lv","sequence":"first","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2088-0522","authenticated-orcid":true,"given":"Hui","family":"Guo","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuhui","family":"Li","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guojing","family":"Hu","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guolin","family":"Wan","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruwen","family":"Wang","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guoyu","family":"Xian","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. 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China, 110870"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ke","family":"Zhu","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yechao","family":"Han","sequence":"additional","affiliation":[{"name":"University of Chinese Academy of Sciences , , ,","place":["Beijing, P. R. China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2942-892X","authenticated-orcid":true,"given":"Lihong","family":"Bao","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. China, 100190"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2490-4691","authenticated-orcid":true,"given":"Xiao","family":"Lin","sequence":"additional","affiliation":[{"name":"University of Chinese Academy of Sciences , , ,","place":["Beijing, P. R. China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9323-1307","authenticated-orcid":true,"given":"Shixuan","family":"Du","sequence":"additional","affiliation":[{"name":"Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences , ,","place":["Beijing, P. R. 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Rev. Lett."},{"key":"2026080409270174500_cit9","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.108.174430","article-title":"In-Plane\nCanted Ferromagnetism, Intrinsic\nWeyl Fermions, and Large Anomalous Hall Effect in the Kagome Semimetal\nRh3Sn2S2","volume":"108","author":"Wu","year":"2023","journal-title":"Phys.\nRev. B"},{"key":"2026080409270174500_cit10","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.101.115106","article-title":"Emerging Chiral Edge States from the Confinement of a Magnetic Weyl\nSemimetal in Co3Sn2S2","volume":"101","author":"Muechler","year":"2020","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit11","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.121.057202","article-title":"Quantum\nSpin Liquid with Even Ising Gauge Field Structure on Kagome Lattice","volume":"121","author":"Wang","year":"2018","journal-title":"Phys. Rev. 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Phys."},{"key":"2026080409270174500_cit15","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.99.094430","article-title":"Field-Induced Topological\nHall Effect in the Noncoplanar Triangular Antiferromagnetic Geometry\nof Mn3Sn","volume":"99","author":"Rout","year":"2019","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit16","doi-asserted-by":"publisher","DOI":"10.1007\/s11433-024-2553-3","article-title":"Anisotropic Transport\nProperties and Topological Hall Effect in the\nAnnealed Kagome Antiferromagnet FeGe","volume":"68","author":"Ma","year":"2025","journal-title":"Sci. China,\nSer. G:Phys., Mech. Astron."},{"key":"2026080409270174500_cit17","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202522151","article-title":"Large Room\nTemperature Anomalous Nernst Effect Coupled with Topological Nernst\nEffect from Incommensurate Spin Structure in a Kagome Antiferromagnet","volume":"13","author":"Ma","year":"2026","journal-title":"Adv. Sci."},{"key":"2026080409270174500_cit18","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.108.144435","article-title":"Planar\nHall Effect and Anisotropic\nMagnetoresistance in Thin Films of the Chiral Antiferromagnet Mn3Sn","volume":"108","author":"Sharma","year":"2023","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit19","doi-asserted-by":"publisher","first-page":"7860","DOI":"10.1021\/acs.nanolett.0c02219","article-title":"Field-Induced Anomalous Hall Conductivity\nand Planar Hall Effect in Co3Sn2S2 Nanoflakes","volume":"20","author":"Yang","year":"2020","journal-title":"Nano Lett."},{"key":"2026080409270174500_cit20","doi-asserted-by":"publisher","first-page":"2838","DOI":"10.1021\/acsaelm.3c00312","article-title":"Anisotropic Magnetoresistance\nand\nPlanar Hall Effect in Layered Room-Temperature Ferromagnet Cr1.2Te2","volume":"5","author":"Ma","year":"2023","journal-title":"ACS Appl. Electron.\nMater."},{"key":"2026080409270174500_cit21","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.96.041110","article-title":"Giant Planar\nHall Effect in Topological Metals","volume":"96","author":"Burkov","year":"2017","journal-title":"Phys. Rev.\nB"},{"key":"2026080409270174500_cit22","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.97.201110","article-title":"Giant Anisotropic\nMagnetoresistance and Planar Hall Effect in the Dirac Semimetal Cd3As2","volume":"97","author":"Li","year":"2018","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit23","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.1601742","article-title":"Butterfly\nMagnetoresistance, Quasi-2D\nDirac Fermi Surface and Topological Phase Transition in ZrSiS","volume":"2","author":"Ali","year":"2016","journal-title":"Sci. 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Mater."},{"key":"2026080409270174500_cit27","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-019-10624-z","article-title":"Orbital-Flop Induced\nMagnetoresistance Anisotropy in\nRare Earth Monopnictide CeSb","volume":"10","author":"Xu","year":"2019","journal-title":"Nat. Commun."},{"key":"2026080409270174500_cit28","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.100.180407","article-title":"Magnetization-Governed\nMagnetoresistance Anisotropy in the Topological Semimetal CeBi","volume":"100","author":"Lyu","year":"2019","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit29","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.106.235102","article-title":"Anomalous Symmetry Breaking in the Weyl Semimetal CeAlGe","volume":"106","author":"Hodovanets","year":"2022","journal-title":"Phys. Rev. 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Lett."},{"key":"2026080409270174500_cit33","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.96.125112","article-title":"Separation\nof Electron and Hole Dynamics in the Semimetal\nLaSb","volume":"96","author":"Han","year":"2017","journal-title":"Phys. Rev. B"},{"key":"2026080409270174500_cit34","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.107.085136","article-title":"Magnetoresistance and Kohler Rule\nin the Topological Chiral Semimetal CoSi","volume":"107","author":"Petrova","year":"2023","journal-title":"Phys.\nRev. B"},{"key":"2026080409270174500_cit35","doi-asserted-by":"publisher","first-page":"7476","DOI":"10.1021\/acs.nanolett.0c02962","article-title":"Topological\nKagome Magnet Co3Sn2S2 Thin Flakes\nwith High Electron Mobility and Large Anomalous Hall Effect","volume":"20","author":"Tanaka","year":"2020","journal-title":"Nano Lett."},{"key":"2026080409270174500_cit36","doi-asserted-by":"publisher","first-page":"2032","DOI":"10.1007\/s40843-022-2348-9","article-title":"Record-High Mobility and Extreme\nMagnetoresistance on Kagome-Lattice in Compensated Semimetal Ni3In2S2","volume":"66","author":"Fang","year":"2023","journal-title":"Sci. China\nMater."},{"key":"2026080409270174500_cit37","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.104.235139","article-title":"Electronic\nProperties of the Topological Kagome Metals YV6Sn6 and GdV6Sn6","volume":"104","author":"Pokharel","year":"2021","journal-title":"Phys. Rev.\nB"},{"key":"2026080409270174500_cit38","doi-asserted-by":"publisher","first-page":"1161","DOI":"10.1038\/nmat4684","article-title":"The Chiral\nAnomaly and Thermopower of Weyl Fermions in the Half-Heusler GdPtBi","volume":"15","author":"Hirschberger","year":"2016","journal-title":"Nat. Mater."},{"key":"2026080409270174500_cit39","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-25002-x","article-title":"Magnetic-Field-Induced\nRobust Zero Hall Plateau State in MnBi2Te4 Chern\nInsulator","volume":"12","author":"Liu","year":"2021","journal-title":"Nat. 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