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Conventional approaches rely on lithographically patterned metasurfaces with limited scalability, or on ultrathin materials with weak light\u2013matter interaction. Here, we show that cavity-coupled assemblies of sub-10 nm plasmonic tin-doped indium oxide nanocrystals function as dynamic metasurfaces with electrochemically switchable linear and nonlinear optical responses. By integrating colloidal nanocrystals into a photonic architecture, we colocate permittivity modulation and electromagnetic field confinement within the same nanoscale volume, achieving 77% absolute reflection modulation. Synthetic control of tin doping provides spectral selectivity across 2.5\u20134 \u03bcm, while solution processing yields centimeter-scale device uniformity. Beyond linear modulation, voltage-controlled near-field enhancement enables electrically switchable ultrafast nonlinear response with 100% relative reflection modulation (from an absolute 3 to 6%) and 0.25 ps recovery time, enabling dual-time scale optical control.<\/jats:p>","DOI":"10.1021\/acsnano.6c08804","type":"journal-article","created":{"date-parts":[[2026,7,20]],"date-time":"2026-07-20T06:54:12Z","timestamp":1784530452000},"page":"21435-21444","source":"Crossref","is-referenced-by-count":0,"title":["Electrochemical\nControl of Tunable Infrared Nanocrystal\nMetasurfaces"],"prefix":"10.1021","volume":"20","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0796-9271","authenticated-orcid":true,"given":"Woo Je","family":"Chang","sequence":"first","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78712"]},{"name":"University of Michigan , , , ,","place":["Ann Arbor, Michigan, United States, 48109"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3886-1378","authenticated-orcid":true,"given":"Zarko","family":"Sakotic","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78758"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Madeline","family":"Brown","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78758"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1256-9064","authenticated-orcid":true,"given":"Lauralee E.","family":"Hurst","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78712"]},{"name":"University of Michigan , , , ,","place":["Ann Arbor, Michigan, United States, 48109"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yonathan","family":"Magendzo Behar","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78758"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-8043-0584","authenticated-orcid":true,"given":"Yujin","family":"Park","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78712"]},{"name":"University of Michigan , , , ,","place":["Ann Arbor, Michigan, United States, 48109"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3234-0803","authenticated-orcid":true,"given":"Daniel","family":"Wasserman","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78758"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8737-451X","authenticated-orcid":true,"given":"Delia J.","family":"Milliron","sequence":"additional","affiliation":[{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78712"]},{"name":"University of Michigan , , , ,","place":["Ann Arbor, Michigan, United States, 48109"]},{"name":"University of Texas at Austin , , , ,","place":["Austin, Texas, United States, 78712"]},{"name":"University of Michigan , , , ,","place":["Ann Arbor, Michigan, United States, 48109"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,20]]},"reference":[{"key":"2026080409265371900_cit1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-35327-w","article-title":"High-capacity free-space\noptical communications using wavelength-and mode-division-multiplexing\nin the mid-infrared region","volume":"13","author":"Zou","year":"2022","journal-title":"Nat. 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