{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,20]],"date-time":"2026-10-20T12:49:21Z","timestamp":1792500561065,"version":"4.5.0"},"reference-count":65,"publisher":"American Chemical Society (ACS)","issue":"41","license":[{"start":{"date-parts":[[2026,10,8]],"date-time":"2026-10-08T00:00:00Z","timestamp":1791417600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,10,8]],"date-time":"2026-10-08T00:00:00Z","timestamp":1791417600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,10,8]],"date-time":"2026-10-08T00:00:00Z","timestamp":1791417600000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100003977","name":"Israel Science Foundation","doi-asserted-by":"publisher","award":["4085\/25"],"award-info":[{"award-number":["4085\/25"]}],"id":[{"id":"10.13039\/501100003977","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100000015","name":"U.S. Department of Energy","doi-asserted-by":"publisher","award":["BES-ERCAP0032503"],"award-info":[{"award-number":["BES-ERCAP0032503"]}],"id":[{"id":"10.13039\/100000015","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100000015","name":"U.S. Department of Energy","doi-asserted-by":"publisher","award":["DE-AC02-05CH11231"],"award-info":[{"award-number":["DE-AC02-05CH11231"]}],"id":[{"id":"10.13039\/100000015","id-type":"DOI","asserted-by":"publisher"}]},{"name":"National Science Foundation (NSF)","award":["CHE-2449564"],"award-info":[{"award-number":["CHE-2449564"]}]},{"name":"National Science Foundation (NSF)","award":["DMR-2019444"],"award-info":[{"award-number":["DMR-2019444"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,20]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Quantum light provides opportunities for controlling multiphoton absorption beyond the classical limits. Here, we investigate biexciton generation in nanocrystal quantum dots driven by energy-time-entangled photon pairs generated via spontaneous parametric downconversion. We show that frequency\u2013time correlations between pairs of photons increase the population of biexcitons over excitons, thereby lending specificity to the excitation of many-body states. By employing a three-level model, we demonstrate that biexciton generation depends nontrivially on the photon entanglement time and pump bandwidth. We find that maximizing efficiency requires an optimally shaped entangled photon field rather than simply scaling parameters for a monotonic improvement. Extending to a realistic CdSe\/CdS core\u2013shell quantum dot containing many excitonic states coupled to the quantum field, we demonstrate that increasing the biphoton arrival-time entanglement (closer arrival time) enhances constructive pathway interference and expands accessible excitation channels while preserving better energy-conservation in excitation than classical light when generating biexcitons. Furthermore, tuning the time-correlation properties enables selective excitation of closely spaced biexciton states. These results establish entangled photons as tools for selective excitation and control of higher-order excited states in quantum-confined systems.<\/jats:p>","DOI":"10.1021\/acsnano.6c10075","type":"journal-article","created":{"date-parts":[[2026,10,8]],"date-time":"2026-10-08T21:01:52Z","timestamp":1791493312000},"page":"27807-27817","source":"Crossref","is-referenced-by-count":0,"title":["Selective Biexciton\nGeneration under Energy-Time Entangled\nQuantum Light in Quantum Dots"],"prefix":"10.1021","volume":"20","author":[{"ORCID":"https:\/\/orcid.org\/0009-0003-7697-2850","authenticated-orcid":true,"given":"Kaiyue","family":"Peng","sequence":"first","affiliation":[{"name":"University of California , , , ,","place":["Berkeley, California, United States, 94720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-8867-3387","authenticated-orcid":true,"given":"Chieh","family":"Tsao","sequence":"additional","affiliation":[{"name":"University of California , , , ,","place":["Berkeley, California, United States, 94720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2901-0141","authenticated-orcid":true,"given":"Hendrik","family":"Utzat","sequence":"additional","affiliation":[{"name":"University of California , , , ,","place":["Berkeley, California, United States, 94720"]},{"name":"Lawrence Berkeley National Laboratory , , , ,","place":["Berkeley, California, United States, 94720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2031-3525","authenticated-orcid":true,"given":"Eran","family":"Rabani","sequence":"additional","affiliation":[{"name":"University of California , , , ,","place":["Berkeley, California, United States, 94720"]},{"name":"Lawrence Berkeley National Laboratory , , , ,","place":["Berkeley, California, United States, 94720"]},{"name":"Hebrew University of Jerusalem , , ,","place":["Jerusalem, Israel, 91904"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,10,8]]},"reference":[{"issue":"2","key":"2026102008172942800_cit1","doi-asserted-by":"publisher","first-page":"021309","DOI":"10.1063\/5.0010193","article-title":"Progress in quantum-dot single photon sources for quantum\ninformation technologies: A broad spectrum overview","volume":"7","author":"Arakawa","year":"2020","journal-title":"Appl. Phys. Rev."},{"key":"2026102008172942800_cit2","doi-asserted-by":"publisher","first-page":"1091","DOI":"10.1038\/s41565-024-01606-4","article-title":"Engineering\ncolloidal semiconductor nanocrystals for\nquantum information processing","volume":"19","author":"Almutlaq","year":"2024","journal-title":"Nat. Nanotechnol."},{"key":"2026102008172942800_cit3","doi-asserted-by":"publisher","first-page":"1","DOI":"10.1146\/annurev.matsci.34.040203.111535","article-title":"Quantum dot\nopto-electronic devices","volume":"34","author":"Bhattacharya","year":"2004","journal-title":"Annu. Rev. Mater. Res."},{"key":"2026102008172942800_cit4","doi-asserted-by":"publisher","first-page":"3873","DOI":"10.1103\/PhysRevLett.77.3873","article-title":"Photoluminescence\nspectroscopy of\nsingle CdSe nanocrystallite quantum dots","volume":"77","author":"Empedocles","year":"1996","journal-title":"Phys.\nRev. Lett."},{"issue":"20","key":"2026102008172942800_cit5","doi-asserted-by":"publisher","first-page":"201104","DOI":"10.1063\/5.0143201","article-title":"Temperature\ndependence of photoluminescence spectrum\nof single lead halide perovskite nanocrystals: Effect of size on the\nphase transition temperature","volume":"158","author":"Cho","year":"2023","journal-title":"J. Chem. Phys."},{"issue":"1","key":"2026102008172942800_cit6","doi-asserted-by":"publisher","first-page":"4424","DOI":"10.1038\/s41467-025-58800-8","article-title":"Exciton-phonon coupling and phonon-assisted\nexciton relaxation dynamics in In1-xGaxP quantum dots","volume":"16","author":"Li","year":"2025","journal-title":"Nat. Commun."},{"key":"2026102008172942800_cit7","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202523678","article-title":"Phase-Pure\nand Size-Tunable Tin Halide Perovskite Quantum Dots","author":"Dressler","year":"2026","journal-title":"Adv. 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Phys."},{"key":"2026102008172942800_cit46","article-title":"Heralded Emission Detection in InAs\/ZnSe\nQuantum\nDot Solids Using Time-Correlated Photons","author":"Tsao","year":"2025","journal-title":"arXiv: 250911704"},{"issue":"8","key":"2026102008172942800_cit47","doi-asserted-by":"publisher","first-page":"081501","DOI":"10.1063\/5.0049338","article-title":"Entangled\ntwo-photon absorption by\natoms and molecules: A quantum optics tutorial","volume":"155","author":"Raymer","year":"2021","journal-title":"J. Chem. 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Rev.\nLett."},{"key":"2026102008172942800_cit51","doi-asserted-by":"publisher","first-page":"9640","DOI":"10.1364\/OE.20.009640","article-title":"A high-brightness source of polarization-entangled\nphotons optimized for applications in free space","volume":"20","author":"Steinlechner","year":"2012","journal-title":"Opt. Express"},{"issue":"1","key":"2026102008172942800_cit52","doi-asserted-by":"publisher","first-page":"48","DOI":"10.1038\/s42005-023-01169-1","article-title":"Ultrafast hole relaxation dynamics in quantum dots\nrevealed by two-dimensional electronic spectroscopy","volume":"6","author":"Brosseau","year":"2023","journal-title":"Commun. Phys."},{"issue":"10","key":"2026102008172942800_cit53","doi-asserted-by":"publisher","first-page":"104702","DOI":"10.1063\/5.0272621","article-title":"Atomistically\nresolved hot exciton relaxation dynamics in CdSe quantum dots: Experiment\nand theory","volume":"163","author":"Ghosh","year":"2025","journal-title":"J. Chem. 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