{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T19:46:52Z","timestamp":1792784812557,"version":"4.5.0"},"reference-count":52,"publisher":"American Chemical Society (ACS)","issue":"39","license":[{"start":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T00:00:00Z","timestamp":1789948800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T00:00:00Z","timestamp":1789948800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T00:00:00Z","timestamp":1789948800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"name":"National Basic Research Program of China (973 Program)","award":["2023YFB3809501"],"award-info":[{"award-number":["2023YFB3809501"]}]},{"name":"National Natural Science Foundation of China (NSFC)","award":["52472246"],"award-info":[{"award-number":["52472246"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"crossref"}]},{"name":"National Natural Science Foundation of China (NSFC)","award":["U25A20382"],"award-info":[{"award-number":["U25A20382"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"crossref"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,10,6]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Developing high-performance magnesium metal batteries is hindered by sluggish Mg2+ diffusion kinetics and the structural instability of conventional cathodes. Here, we propose a design principle for organic cathodes by regulating polymer spatial configurations, which facilitates multidirectional Mg2+ transport and enhances structural robustness. Three poly(perylene diimide) (PDI)-based polymers, namely linear pPDI, zigzag mPDI, and layered oPDI, were synthesized to systematically investigate the structure\u2013function relationship. The oPDI cathode, featuring a highly ordered two-dimensional layered configuration, forms an interconnected three-dimensional Mg2+ transport network, in striking contrast to the one-dimensional interchain hopping confined in pPDI and mPDI. By integrating multiscale experimental characterizations with density functional theory calculations, we reveal that oPDI enables rapid Mg2+ diffusion, minimizes structural distortion, and exhibits highly reversible carbonyl redox chemistry. Consequently, oPDI exhibits enhanced rate capability, durable cycling performance (92% retention over 1000 cycles), and wide-temperature adaptability from \u221220 to 50 \u00b0C. Furthermore, Mg||oPDI pouch cells also maintain stable cycling performance, demonstrating the potential for practical implementation. This work presents spatial configuration engineering as an effective strategy for designing high-performance organic cathodes and advances the development of safe, scalable, and temperature-resilient magnesium batteries.<\/jats:p>","DOI":"10.1021\/acsnano.6c13540","type":"journal-article","created":{"date-parts":[[2026,9,21]],"date-time":"2026-09-21T13:02:27Z","timestamp":1789995747000},"page":"26822-26832","source":"Crossref","is-referenced-by-count":0,"title":["Tailoring\nIon-Transport Networks for Wide-Temperature\nMg-Organic Batteries"],"prefix":"10.1021","volume":"20","author":[{"given":"Ge","family":"Zhang","sequence":"first","affiliation":[{"name":"Wuhan University of Technology , , ,","place":["Wuhan, P. R. China, 430070"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Meng","sequence":"additional","affiliation":[{"name":"The Hong Kong Polytechnic University , , Hung Hom , ,","place":["Hong Kong, P. R. China, 999077"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenwei","family":"Zhang","sequence":"additional","affiliation":[{"name":"Wuhan University of Technology , , ,","place":["Wuhan, P. R. China, 430070"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ze","family":"He","sequence":"additional","affiliation":[{"name":"University of Cambridge , , ,","place":["Cambridge, U.K., CB3 0FS"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianyong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Wuhan University of Technology , , ,","place":["Wuhan, P. R. China, 430070"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenxu","family":"Dong","sequence":"additional","affiliation":[{"name":"Wuhan University of Technology , , ,","place":["Wuhan, P. R. 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